Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths

Xu, Xiaochuan; Zheng, Xiaorui; He, Feng; Wang, Zheng; Subbaraman, Harish; Wang, Yaguo; Jia, Baohua; Chen, Ray T.

doi:10.1038/s41598-017-09583-6

Title: Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths

Abstract

All-optical switches have been considered as a promising solution to overcome the fundamental speed limit of the current electronic switches. However, the lack of a suitable third-order nonlinear material greatly hinders the development of this technology. Here in this paper we report the observation of ultrahigh third-order nonlinearity about 0.45 cm²/GW in graphene oxide thin films at the telecommunication wavelength region, which is four orders of magnitude higher than that of single crystalline silicon. Besides, graphene oxide is water soluble and thus easy to process due to the existence of oxygen containing groups. These unique properties can potentially significantly advance the performance of alloptical switches.

Authors:

Xu, Xiaochuan ^[1]; Zheng, Xiaorui ^[2]; He, Feng ^[3];

^[4]; Subbaraman, Harish ^[5]; Wang, Yaguo ^[3];

^[2]; Chen, Ray T. ^[6]

Omega Optics, Inc., Austin, TX (United States)
Swinburne Univ. of Technology, Hawthorn, VIC (Australia)
Univ. of Texas, Austin, TX (United States). Dept. of Mechanical Engineering
Univ. of Texas, Austin, TX (United States). Texas Materials Inst., Materials Science and Engineering Program
Omega Optics, Inc., Austin, TX (United States); Boise State Univ., ID (United States). Dept. of Electrical and Computer Engineering
Omega Optics, Inc., Austin, TX (United States); Univ. of Texas, Austin, TX (United States). Dept. of Electrical and Computer Engineering

Publication Date:: 2017-08-29

Research Org.:: Omega Optics, Inc., Austin, TX (United States)

Sponsoring Org.:: USDOE; Australian Research Council (ARC); Defense Science Institute Australia

OSTI Identifier:: 1425666

Grant/Contract Number:: SC0013178

Resource Type:: Accepted Manuscript

Journal Name:: Scientific Reports

Additional Journal Information:: Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 2045-2322

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Materials for optics; Optical materials and structures

Citation Formats


                    Xu, Xiaochuan, Zheng, Xiaorui, He, Feng, Wang, Zheng, Subbaraman, Harish, Wang, Yaguo, Jia, Baohua, and Chen, Ray T. Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths.  United States: N. p., 2017. 
Web.  doi:10.1038/s41598-017-09583-6.

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                    Xu, Xiaochuan, Zheng, Xiaorui, He, Feng, Wang, Zheng, Subbaraman, Harish, Wang, Yaguo, Jia, Baohua, & Chen, Ray T. Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths.  United States.  https://doi.org/10.1038/s41598-017-09583-6

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                    Xu, Xiaochuan, Zheng, Xiaorui, He, Feng, Wang, Zheng, Subbaraman, Harish, Wang, Yaguo, Jia, Baohua, and Chen, Ray T. Tue .  
"Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths".  United States.  https://doi.org/10.1038/s41598-017-09583-6.  https://www.osti.gov/servlets/purl/1425666.

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@article{osti_1425666,

  title        = {Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths},

  author       = {Xu, Xiaochuan and Zheng, Xiaorui and He, Feng and Wang, Zheng and Subbaraman, Harish and Wang, Yaguo and Jia, Baohua and Chen, Ray T.},

  abstractNote = {All-optical switches have been considered as a promising solution to overcome the fundamental speed limit of the current electronic switches. However, the lack of a suitable third-order nonlinear material greatly hinders the development of this technology. Here in this paper we report the observation of ultrahigh third-order nonlinearity about 0.45 cm2/GW in graphene oxide thin films at the telecommunication wavelength region, which is four orders of magnitude higher than that of single crystalline silicon. Besides, graphene oxide is water soluble and thus easy to process due to the existence of oxygen containing groups. These unique properties can potentially significantly advance the performance of alloptical switches.},

  doi          = {10.1038/s41598-017-09583-6},

  journal      = {Scientific Reports},

  number       = 1,

  volume       = 7,

  place        = {United States},

  year         = {2017},

  month        = {8}

}

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Title: Observation of Third-order Nonlinearities in Graphene Oxide Film at Telecommunication Wavelengths

Abstract

Citation Formats

Polarization dependence of Z-scan measurement: theory and experiment journal, January 2009

Capacity Trends and Limits of Optical Communication Networks journal, May 2012

Graphene oxide as a chemically tunable platform for optical applications journal, November 2010

Broadband nonlinear optical response in multi-layer black phosphorus: an emerging infrared and mid-infrared optical material journal, January 2015

Two-photon absorption as a limitation to all-optical switching journal, January 1989

All-optical switching with 1-ps response time in a DDMEBT enabled silicon grating coupler/resonator hybrid device journal, January 2014

Transient thermal effect, nonlinear refraction and nonlinear absorption properties of graphene oxide sheets in dispersion journal, January 2013

Thermal and Kerr nonlinear properties of plasma-deposited silicon nitride/ silicon dioxide waveguides journal, January 2008

Recent advances in silicon-based passive and active optical interconnects journal, January 2015

Flexible Single-Crystal Silicon Nanomembrane Photonic Crystal Cavity journal, November 2014

Processable aqueous dispersions of graphene nanosheets journal, January 2008

New CMOS-compatible platforms based on silicon nitride and Hydex for nonlinear optics journal, July 2013

Graphene and Graphene Oxide: Synthesis, Properties, and Applications journal, June 2010

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Ultra-high-density spatial division multiplexing with a few-mode multicore fibre journal, October 2014

Complementary metal–oxide–semiconductor compatible high efficiency subwavelength grating couplers for silicon integrated photonics journal, July 2012

Graphene Oxides as Tunable Broadband Nonlinear Optical Materials for Femtosecond Laser Pulses journal, March 2012

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Nonlinear silicon photonics journal, July 2010

Large energy soliton erbium-doped fiber laser with a graphene-polymer composite mode locker journal, October 2009

Ultrafast Dynamics and Nonlinear Optical Responses from sp 2 - and sp 3 -Hybridized Domains in Graphene Oxide journal, July 2011

False nonlinear effect in z-scan measurement based on semiconductor laser devices: theory and experiments journal, January 2014

Z-scan measurement of the nonlinear refractive index of graphene journal, January 2012

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Third order nonlinear optical property of Bi_2Se_3 journal, January 2013

Ultrafast nonlinear absorption and nonlinear refraction in few-layer oxidized black phosphorus journal, January 2016

In Situ Third-Order Non-linear Responses During Laser Reduction of Graphene Oxide Thin Films Towards On-Chip Non-linear Photonic Devices journal, March 2014

Atomic-Layer Graphene as a Saturable Absorber for Ultrafast Pulsed Lasers journal, October 2009

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Polarization dependence of Z-scan measurement: theory and experiment
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Capacity Trends and Limits of Optical Communication Networks
journal, May 2012

Graphene oxide as a chemically tunable platform for optical applications
journal, November 2010

Broadband nonlinear optical response in multi-layer black phosphorus: an emerging infrared and mid-infrared optical material
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Two-photon absorption as a limitation to all-optical switching
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All-optical switching with 1-ps response time in a DDMEBT enabled silicon grating coupler/resonator hybrid device
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Processable aqueous dispersions of graphene nanosheets
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Ultrafast Dynamics and Nonlinear Optical Responses from sp ² - and sp ³ -Hybridized Domains in Graphene Oxide
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False nonlinear effect in z-scan measurement based on semiconductor laser devices: theory and experiments
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Z-scan measurement of the nonlinear refractive index of graphene
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Amorphous silicon nanowires combining high nonlinearity, FOM and optical stability
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Third order nonlinear optical property of Bi_2Se_3
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Ultrafast nonlinear absorption and nonlinear refraction in few-layer oxidized black phosphorus
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