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Title: Small influence of magnetic ordering on lattice dynamics in TaFe 1.25 Te 3

Raman scattering spectra of zigzag spin chain TaFe 1.25Te 3 single crystal are presented in a temperature range from 80 to 300 K. Nine Raman active modes of A g and B g symmetry are clearly observed and assigned by probing different scattering channels, which is confirmed by lattice dynamics calculations. Temperature dependence of the Raman modes linewidth is mainly governed by the lattice anharmonicity. The only deviation from the conventional behavior is observed for A g symmetry modes in a vicinity of the magnetic phase transition at T N ≈ 200 K. This implies that the electron-phonon interaction weakly changes with temperature and magnetic ordering, whereas small changes in the spectra near the critical temperature can be ascribed to spin fluctuations.
Authors:
 [1] ;  [1] ;  [1] ;  [1] ;  [1] ;  [2] ;  [3] ;  [1]
  1. Univ. of Belgrade (Serbia)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States); Tianjin Univ. of Technology (China)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Report Number(s):
BNL-200078-2018-JAAM
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1802023
Grant/Contract Number:
SC0012704
Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 96; Journal Issue: 17; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Research Org:
Brookhaven National Laboratory (BNL), Upton, NY (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
OSTI Identifier:
1425061
Alternate Identifier(s):
OSTI ID: 1409139

Opačić, M., Lazarević, N., Tanasković, D., Radonjić, M. M., Milosavljević, A., Ma, Yongchang, Petrovic, C., and Popović, Z. V.. Small influence of magnetic ordering on lattice dynamics in TaFe1.25Te3. United States: N. p., Web. doi:10.1103/PhysRevB.96.174303.
Opačić, M., Lazarević, N., Tanasković, D., Radonjić, M. M., Milosavljević, A., Ma, Yongchang, Petrovic, C., & Popović, Z. V.. Small influence of magnetic ordering on lattice dynamics in TaFe1.25Te3. United States. doi:10.1103/PhysRevB.96.174303.
Opačić, M., Lazarević, N., Tanasković, D., Radonjić, M. M., Milosavljević, A., Ma, Yongchang, Petrovic, C., and Popović, Z. V.. 2017. "Small influence of magnetic ordering on lattice dynamics in TaFe1.25Te3". United States. doi:10.1103/PhysRevB.96.174303. https://www.osti.gov/servlets/purl/1425061.
@article{osti_1425061,
title = {Small influence of magnetic ordering on lattice dynamics in TaFe1.25Te3},
author = {Opačić, M. and Lazarević, N. and Tanasković, D. and Radonjić, M. M. and Milosavljević, A. and Ma, Yongchang and Petrovic, C. and Popović, Z. V.},
abstractNote = {Raman scattering spectra of zigzag spin chain TaFe1.25Te3 single crystal are presented in a temperature range from 80 to 300 K. Nine Raman active modes of Ag and Bg symmetry are clearly observed and assigned by probing different scattering channels, which is confirmed by lattice dynamics calculations. Temperature dependence of the Raman modes linewidth is mainly governed by the lattice anharmonicity. The only deviation from the conventional behavior is observed for Ag symmetry modes in a vicinity of the magnetic phase transition at T N ≈ 200 K. This implies that the electron-phonon interaction weakly changes with temperature and magnetic ordering, whereas small changes in the spectra near the critical temperature can be ascribed to spin fluctuations.},
doi = {10.1103/PhysRevB.96.174303},
journal = {Physical Review B},
number = 17,
volume = 96,
place = {United States},
year = {2017},
month = {11}
}

Works referenced in this record:

QUANTUM ESPRESSO: a modular and open-source software project for quantum simulations of materials
journal, September 2009
  • Giannozzi, Paolo; Baroni, Stefano; Bonini, Nicola
  • Journal of Physics: Condensed Matter, Vol. 21, Issue 39, Article No. 395502
  • DOI: 10.1088/0953-8984/21/39/395502