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Title: Drivers of Seasonal Variability in Marine Boundary Layer Aerosol Number Concentration Investigated Using a Steady State Approach

Marine boundary layer (MBL) aerosol particles affect the climate through their interaction with MBL clouds. Although both MBL clouds and aerosol particles have pronounced seasonal cycles, the factors controlling seasonal variability of MBL aerosol particle concentration are not well-constrained. In this paper an aerosol budget is constructed representing the effects of wet deposition, free-tropospheric entrainment, primary surface sources, and advection on the MBL accumulation mode aerosol number concentration (N a). These terms are further parameterized, and by assuming that on seasonal timescales N a is in steady state, the budget equation is rearranged to form a diagnostic equation for N a based on observable variables. Using data primarily collected in the subtropical northeast Pacific during the MAGIC campaign (Marine ARM (Atmospheric Radiation Measurement) GPCI (GCSS Pacific Cross-section Intercomparison) Investigation of Clouds), estimates of both mean summer and winter N a concentrations are made using the simplified steady-state model and seasonal mean observed variables, and are found to match well with the observed N a. To attribute the modeled difference between summer and winter aerosol concentrations to individual observed variables (e.g. precipitation rate, free-tropospheric aerosol number concentration), a local sensitivity analysis is combined with the seasonal difference in observed variables. Thismore » analysis shows that despite wintertime precipitation frequency being lower than summer, the higher winter precipitation rate accounted for approximately 60% of the modeled seasonal difference in N a, which emphasizes the importance of marine stratocumulus precipitation in determining MBL aerosol concentrations on longer time scales.« less
Authors:
ORCiD logo [1] ; ORCiD logo [1] ; ORCiD logo [1] ;  [1] ;  [2]
  1. Univ. of Washington, Seattle, WA (United States). Dept. of Atmospheric Sciences
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Report Number(s):
BNL-114844-2017-JAAM
Journal ID: ISSN 2169-897X
Grant/Contract Number:
SC0012704; SC0013489; SC0011602; AGS-1445813
Type:
Accepted Manuscript
Journal Name:
Journal of Geophysical Research: Atmospheres
Additional Journal Information:
Journal Volume: 123; Journal Issue: 2; Journal ID: ISSN 2169-897X
Publisher:
American Geophysical Union
Research Org:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org:
USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23); Univ. of Washington, Seattle, WA (United States)
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES
OSTI Identifier:
1424973

Mohrmann, Johannes, Wood, Robert, McGibbon, Jeremy, Eastman, Ryan, and Luke, Edward. Drivers of Seasonal Variability in Marine Boundary Layer Aerosol Number Concentration Investigated Using a Steady State Approach. United States: N. p., Web. doi:10.1002/2017JD027443.
Mohrmann, Johannes, Wood, Robert, McGibbon, Jeremy, Eastman, Ryan, & Luke, Edward. Drivers of Seasonal Variability in Marine Boundary Layer Aerosol Number Concentration Investigated Using a Steady State Approach. United States. doi:10.1002/2017JD027443.
Mohrmann, Johannes, Wood, Robert, McGibbon, Jeremy, Eastman, Ryan, and Luke, Edward. 2018. "Drivers of Seasonal Variability in Marine Boundary Layer Aerosol Number Concentration Investigated Using a Steady State Approach". United States. doi:10.1002/2017JD027443.
@article{osti_1424973,
title = {Drivers of Seasonal Variability in Marine Boundary Layer Aerosol Number Concentration Investigated Using a Steady State Approach},
author = {Mohrmann, Johannes and Wood, Robert and McGibbon, Jeremy and Eastman, Ryan and Luke, Edward},
abstractNote = {Marine boundary layer (MBL) aerosol particles affect the climate through their interaction with MBL clouds. Although both MBL clouds and aerosol particles have pronounced seasonal cycles, the factors controlling seasonal variability of MBL aerosol particle concentration are not well-constrained. In this paper an aerosol budget is constructed representing the effects of wet deposition, free-tropospheric entrainment, primary surface sources, and advection on the MBL accumulation mode aerosol number concentration (Na). These terms are further parameterized, and by assuming that on seasonal timescales Na is in steady state, the budget equation is rearranged to form a diagnostic equation for Na based on observable variables. Using data primarily collected in the subtropical northeast Pacific during the MAGIC campaign (Marine ARM (Atmospheric Radiation Measurement) GPCI (GCSS Pacific Cross-section Intercomparison) Investigation of Clouds), estimates of both mean summer and winter Na concentrations are made using the simplified steady-state model and seasonal mean observed variables, and are found to match well with the observed Na. To attribute the modeled difference between summer and winter aerosol concentrations to individual observed variables (e.g. precipitation rate, free-tropospheric aerosol number concentration), a local sensitivity analysis is combined with the seasonal difference in observed variables. This analysis shows that despite wintertime precipitation frequency being lower than summer, the higher winter precipitation rate accounted for approximately 60% of the modeled seasonal difference in Na, which emphasizes the importance of marine stratocumulus precipitation in determining MBL aerosol concentrations on longer time scales.},
doi = {10.1002/2017JD027443},
journal = {Journal of Geophysical Research: Atmospheres},
number = 2,
volume = 123,
place = {United States},
year = {2018},
month = {1}
}