DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Observation of nanoscale magnetic fields using twisted electron beams

Abstract

Electron waves give an unprecedented enhancement to the field of microscopy by providing higher resolving power compared to their optical counterpart. Further information about a specimen, such as electric and magnetic features, can be revealed in electron microscopy because electrons possess both a magnetic moment and charge. In-plane magnetic structures in materials can be studied experimentally using the effect of the Lorentz force. On the other hand, full mapping of the magnetic field has hitherto remained challenging. Here we measure a nanoscale out-of-plane magnetic field by interfering a highly twisted electron vortex beam with a reference wave. We implement a recently developed holographic technique to manipulate the electron wavefunction, which gives free electrons an additional unbounded quantized magnetic moment along their propagation direction. Our finding demonstrates that full reconstruction of all three components of nanoscale magnetic fields is possible without tilting the specimen.

Authors:
 [1]; ORCiD logo [2]; ORCiD logo [3];  [2]; ORCiD logo [4];  [5];  [6]; ORCiD logo [7];  [8];  [9];  [8];  [10]; ORCiD logo [2]; ORCiD logo [11]
  1. CNR-Istituto Nanoscienze, Modena (Italy); CNR-IMEM Parco Area delle Scienze 37/A, Parma (Italy)
  2. Univ. of Oregon, Eugene, OR (United States). Department of Physics
  3. CNR-Istituto Nanoscienze, Modena (Italy); University of Modena and Reggio Emilia, Modena (Italy)
  4. CNR-IMM Bologna (Italy)
  5. University of Ottawa, ON (Canada). Department of Physics
  6. CNR-Istituto Nanoscienze, Modena (Italy)
  7. CNR-Istituto Nanoscienze, Modena (Italy); University of Modena and Reggio Emilia, Modena (Italy)
  8. Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons and Peter Grunberg Institute, Forschungszentrum, Julich (Germany)
  9. Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons and Peter Grunberg Institute, Forschungszentrum, Julich (Germany); Chinese Academy of Sciences (CAS), Beijing (China). Institute of Physics
  10. University of Ottawa, ON (Canada). Department of Physics; Univ. of Rochester, NY (United States). Institute of Optics; Univ. of Glasgow, Scotland (United Kingdom). School of Physics and Astronomy
  11. University of Ottawa, ON (Canada). Department of Physics; nstitute for Advanced Studies in Basic Sciences, Zanjan (Iran). Department of Physics
Publication Date:
Research Org.:
Univ. of Oregon, Eugene, OR (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1424912
Grant/Contract Number:  
SC0010466
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; 36 MATERIALS SCIENCE

Citation Formats

Grillo, Vincenzo, Harvey, Tyler R., Venturi, Federico, Pierce, Jordan S., Balboni, Roberto, Bouchard, Frédéric, Carlo Gazzadi, Gian, Frabboni, Stefano, Tavabi, Amir H., Li, Zi-An, Dunin-Borkowski, Rafal E., Boyd, Robert W., McMorran, Benjamin J., and Karimi, Ebrahim. Observation of nanoscale magnetic fields using twisted electron beams. United States: N. p., 2017. Web. doi:10.1038/s41467-017-00829-5.
Grillo, Vincenzo, Harvey, Tyler R., Venturi, Federico, Pierce, Jordan S., Balboni, Roberto, Bouchard, Frédéric, Carlo Gazzadi, Gian, Frabboni, Stefano, Tavabi, Amir H., Li, Zi-An, Dunin-Borkowski, Rafal E., Boyd, Robert W., McMorran, Benjamin J., & Karimi, Ebrahim. Observation of nanoscale magnetic fields using twisted electron beams. United States. https://doi.org/10.1038/s41467-017-00829-5
Grillo, Vincenzo, Harvey, Tyler R., Venturi, Federico, Pierce, Jordan S., Balboni, Roberto, Bouchard, Frédéric, Carlo Gazzadi, Gian, Frabboni, Stefano, Tavabi, Amir H., Li, Zi-An, Dunin-Borkowski, Rafal E., Boyd, Robert W., McMorran, Benjamin J., and Karimi, Ebrahim. Mon . "Observation of nanoscale magnetic fields using twisted electron beams". United States. https://doi.org/10.1038/s41467-017-00829-5. https://www.osti.gov/servlets/purl/1424912.
@article{osti_1424912,
title = {Observation of nanoscale magnetic fields using twisted electron beams},
author = {Grillo, Vincenzo and Harvey, Tyler R. and Venturi, Federico and Pierce, Jordan S. and Balboni, Roberto and Bouchard, Frédéric and Carlo Gazzadi, Gian and Frabboni, Stefano and Tavabi, Amir H. and Li, Zi-An and Dunin-Borkowski, Rafal E. and Boyd, Robert W. and McMorran, Benjamin J. and Karimi, Ebrahim},
abstractNote = {Electron waves give an unprecedented enhancement to the field of microscopy by providing higher resolving power compared to their optical counterpart. Further information about a specimen, such as electric and magnetic features, can be revealed in electron microscopy because electrons possess both a magnetic moment and charge. In-plane magnetic structures in materials can be studied experimentally using the effect of the Lorentz force. On the other hand, full mapping of the magnetic field has hitherto remained challenging. Here we measure a nanoscale out-of-plane magnetic field by interfering a highly twisted electron vortex beam with a reference wave. We implement a recently developed holographic technique to manipulate the electron wavefunction, which gives free electrons an additional unbounded quantized magnetic moment along their propagation direction. Our finding demonstrates that full reconstruction of all three components of nanoscale magnetic fields is possible without tilting the specimen.},
doi = {10.1038/s41467-017-00829-5},
journal = {Nature Communications},
number = 1,
volume = 8,
place = {United States},
year = {Mon Sep 25 00:00:00 EDT 2017},
month = {Mon Sep 25 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 36 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Highly efficient electron vortex beams generated by nanofabricated phase holograms
journal, January 2014

  • Grillo, Vincenzo; Carlo Gazzadi, Gian; Karimi, Ebrahim
  • Applied Physics Letters, Vol. 104, Issue 4
  • DOI: 10.1063/1.4863564

Magnetic effects in the paraxial regime of elastic electron scattering
journal, November 2016


3D Magnetic Induction Maps of Nanoscale Materials Revealed by Electron Holographic Tomography
journal, September 2015


Sculpturing the electron wave function using nanoscale phase masks
journal, September 2014


Vector field electron tomography of magnetic materials: Theoretical development
journal, May 2008


Detection of magnetic circular dichroism using a transmission electron microscope
journal, May 2006

  • Schattschneider, P.; Rubino, S.; Hébert, C.
  • Nature, Vol. 441, Issue 7092
  • DOI: 10.1038/nature04778

Observation of the Larmor and Gouy Rotations with Electron Vortex Beams
journal, February 2013


Twisted photon entanglement through turbulent air across Vienna
journal, November 2015

  • Krenn, Mario; Handsteiner, Johannes; Fink, Matthias
  • Proceedings of the National Academy of Sciences, Vol. 112, Issue 46
  • DOI: 10.1073/pnas.1517574112

Generation of electron Airy beams
journal, February 2013

  • Voloch-Bloch, Noa; Lereah, Yossi; Lilach, Yigal
  • Nature, Vol. 494, Issue 7437
  • DOI: 10.1038/nature11840

Observation of Dirac monopoles in a synthetic magnetic field
journal, January 2014


Twisting of light around rotating black holes
journal, February 2011

  • Tamburini, Fabrizio; Thidé, Bo; Molina-Terriza, Gabriel
  • Nature Physics, Vol. 7, Issue 3
  • DOI: 10.1038/nphys1907

Electron tomography and holography in materials science
journal, April 2009

  • Midgley, Paul A.; Dunin-Borkowski, Rafal E.
  • Nature Materials, Vol. 8, Issue 4
  • DOI: 10.1038/nmat2406

Ultrasmall Functional Ferromagnetic Nanostructures Grown by Focused Electron-Beam-Induced Deposition
journal, September 2011

  • Serrano-Ramón, Luis; Córdoba, Rosa; Rodríguez, Luis Alfredo
  • ACS Nano, Vol. 5, Issue 10
  • DOI: 10.1021/nn201517r

Magnetic monopole field exposed by electrons
journal, December 2013

  • Béché, Armand; Van Boxem, Ruben; Van Tendeloo, Gustaaf
  • Nature Physics, Vol. 10, Issue 1
  • DOI: 10.1038/nphys2816

Structural transitions in electron beam deposited Co–carbonyl suspended nanowires at high electrical current densities
journal, January 2015

  • Gazzadi, Gian Carlo; Frabboni, Stefano
  • Beilstein Journal of Nanotechnology, Vol. 6
  • DOI: 10.3762/bjnano.6.134

Orbital angular momentum of light and the transformation of Laguerre-Gaussian laser modes
journal, June 1992


Lorentz phase microscopy of magnetic materials
journal, January 2004


Propagation of vortex electron wave functions in a magnetic field
journal, July 2012


Quantum walks and wavepacket dynamics on a lattice with twisted photons
journal, March 2015

  • Cardano, Filippo; Massa, Francesco; Qassim, Hammam
  • Science Advances, Vol. 1, Issue 2
  • DOI: 10.1126/sciadv.1500087

Magnetic Monopoles
journal, December 1984


Significance of Electromagnetic Potentials in the Quantum Theory
journal, August 1959


Elastic Scattering of Electron Vortex Beams in Magnetic Matter
journal, March 2016


High-dimensional quantum cloning and applications to quantum hacking
journal, February 2017

  • Bouchard, Frédéric; Fickler, Robert; Boyd, Robert W.
  • Science Advances, Vol. 3, Issue 2
  • DOI: 10.1126/sciadv.1601915

Efficient diffractive phase optics for electrons
journal, September 2014


Generation of electron beams carrying orbital angular momentum
journal, April 2010


Terabit-Scale Orbital Angular Momentum Mode Division Multiplexing in Fibers
journal, June 2013


Vacuum Faraday effect for electrons
journal, October 2012


Observation of isolated monopoles in a quantum field
journal, April 2015


Structured quantum waves
journal, July 2015

  • Harris, Jérémie; Grillo, Vincenzo; Mafakheri, Erfan
  • Nature Physics, Vol. 11, Issue 8
  • DOI: 10.1038/nphys3404

Semiclassical Dynamics of Electron Wave Packet States with Phase Vortices
journal, November 2007


Imaging the dynamics of free-electron Landau states
journal, August 2014

  • Schattschneider, P.; Schachinger, Th.; Stöger-Pollach, M.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5586

Production and application of electron vortex beams
journal, September 2010

  • Verbeeck, J.; Tian, H.; Schattschneider, P.
  • Nature, Vol. 467, Issue 7313
  • DOI: 10.1038/nature09366

Electron Vortex Beams with High Quanta of Orbital Angular Momentum
journal, January 2011

  • McMorran, B. J.; Agrawal, A.; Anderson, I. M.
  • Science, Vol. 331, Issue 6014, p. 192-195
  • DOI: 10.1126/science.1198804

Structure and bonding at the atomic scale by scanning transmission electron microscopy
journal, April 2009


Magnetic monopoles
journal, December 1984

  • Giacomelli, G.
  • La Rivista Del Nuovo Cimento Series 3, Vol. 7, Issue 12
  • DOI: 10.1007/bf02724347

Efficient Diffractive Phase Optics for Electrons
journal, August 2014

  • Pierce, Jordan; Harvey, Tyler; Agrawal, Amit
  • Microscopy and Microanalysis, Vol. 20, Issue S3
  • DOI: 10.1017/s143192761400350x

Magnetic Monopoles
book, January 2005


Twisting of light around rotating black holes
text, January 2011


Propagation of Vortex Electron Wave Functions in a Magnetic Field
text, January 2012


Vacuum Faraday effect for electrons
text, January 2012


Observation of the Larmor and Gouy Rotations with Electron Vortex Beams
text, January 2012


Observation of Dirac Monopoles in a Synthetic Magnetic Field
text, January 2014


Elastic scattering of electron vortex beams in magnetic matter
text, January 2015


Magnetic Effects in the Paraxial Regime of Elastic Electron Scattering
text, January 2016


High-dimensional quantum cloning and applications to quantum hacking
preprint, January 2016


Works referencing / citing this record:

Ultrafast generation and control of an electron vortex beam via chiral plasmonic near fields
journal, May 2019


A tunable path-separated electron interferometer with an amplitude-dividing grating beamsplitter
journal, December 2018

  • Yasin, Fehmi S.; Harada, Ken; Shindo, Daisuke
  • Applied Physics Letters, Vol. 113, Issue 23
  • DOI: 10.1063/1.5051380

Generation and detection of spin-orbit coupled neutron beams
journal, September 2019

  • Sarenac, Dusan; Kapahi, Connor; Chen, Wangchun
  • Proceedings of the National Academy of Sciences, Vol. 116, Issue 41
  • DOI: 10.1073/pnas.1906861116

‘Twisted’ electrons
journal, February 2018


Coiling free electron matter waves
journal, April 2019


Nanostructuring of electron beams
journal, January 2019


Intrinsic multipole moments of non-Gaussian wave packets
journal, February 2019


Relativistic Quantum Dynamics of Twisted Electron Beams in Arbitrary Electric and Magnetic Fields
journal, July 2018


Electric Quadrupole Moment and the Tensor Magnetic Polarizability of Twisted Electrons and a Potential for their Measurements
journal, February 2019


Magnetic characterization of cobalt nanowires and square nanorings fabricated by focused electron beam induced deposition
journal, January 2018

  • Venturi, Federico; Gazzadi, Gian Carlo; Tavabi, Amir H.
  • Beilstein Journal of Nanotechnology, Vol. 9
  • DOI: 10.3762/bjnano.9.97

Intrinsic multipole moments of the non-Gaussian wave packets
text, January 2018