Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts

Oh, Su Cheun; Wu, Yiqing; Tran, Dat T.; Lee, Ivan C.; Lei, Yu; Liu, Dongxia

doi:10.1016/j.fuel.2015.11.058

Title: Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts

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Authors:: Oh, Su Cheun; Wu, Yiqing; Tran, Dat T.; Lee, Ivan C.; Lei, Yu; Liu, Dongxia

Publication Date:: Tue Mar 01 00:00:00 EST 2016

Sponsoring Org.:: USDOE

OSTI Identifier:: 1422855

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Fuel

Additional Journal Information:: Journal Name: Fuel Journal Volume: 167 Journal Issue: C; Journal ID: ISSN 0016-2361

Publisher:: Elsevier

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Oh, Su Cheun, Wu, Yiqing, Tran, Dat T., Lee, Ivan C., Lei, Yu, and Liu, Dongxia. Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts.  United Kingdom: N. p., 2016. 
Web.  doi:10.1016/j.fuel.2015.11.058.

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                    Oh, Su Cheun, Wu, Yiqing, Tran, Dat T., Lee, Ivan C., Lei, Yu, & Liu, Dongxia. Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts.  United Kingdom.  https://doi.org/10.1016/j.fuel.2015.11.058

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                    Oh, Su Cheun, Wu, Yiqing, Tran, Dat T., Lee, Ivan C., Lei, Yu, and Liu, Dongxia. Tue .  
"Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts".  United Kingdom.  https://doi.org/10.1016/j.fuel.2015.11.058.

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@article{osti_1422855,

  title        = {Influences of cation and anion substitutions on oxidative coupling of methane over hydroxyapatite catalysts},

  author       = {Oh, Su Cheun and Wu, Yiqing and Tran, Dat T. and Lee, Ivan C. and Lei, Yu and Liu, Dongxia},

  abstractNote = {},

  doi          = {10.1016/j.fuel.2015.11.058},

  journal      = {Fuel},

  number       = C,

  volume       = 167,

  place        = {United Kingdom},

  year         = {Tue Mar 01 00:00:00 EST 2016},

  month        = {Tue Mar 01 00:00:00 EST 2016}

}

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https://doi.org/10.1016/j.fuel.2015.11.058

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Hydroxyapatites catalyze the partial oxidation of methane to carbon monoxide and hydrogen with molecular oxygen at a reaction temperature as low as 600[degrees]C. The predominant reactions can be stoichiometrically represented as CH[sub 4] + O[sub 2] [yields] CO[sub 2] + 2H[sub 2] and CH[sub 4] + O[sub 2] [yields] CO + H[sub 2] + H[sub 2]O. The former reaction is mainly catalyzed over stoichiometric apatite and the latter proceeds over the nonstoichiometric form. With oxygen as oxidant the H[sub 2]/CO[sub x] ratios produced are strongly dependent on the Ca/P ratio in the hydroxyapatite while with nitrous oxide little or nomore »« less
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