Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells
- Authors:
-
[6]
- Univ. at Buffalo, NY (United States). Dept. of Chemical and Biological Engineering; East China Univ. of Science and Technology, Shanghai (China). School of Mechanical and Power Engineering
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials
- Oregon State Univ., Corvallis, OR (United States). School of Chemical, Biological, and Environmental Engineering
- Univ. at Buffalo, NY (United States). Dept. of Chemical and Biological Engineering
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States); Univ. at Buffalo, NY (United States); East China Univ. of Science and Technology, Shanghai (China); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office; USDOE Office of Science (SC); National Science Foundation (NSF); Shanghai Natural Science Foundation of China; USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1422592
- Alternate Identifier(s):
- OSTI ID: 1417922; OSTI ID: 1558078
- Report Number(s):
- LA-UR-19-27321
Journal ID: ISSN 0935-9648; TRN: US1801631
- Grant/Contract Number:
- AC05-00OR22725; AC02-06CH11357; SC0012704; CBET-1604392; 16ZR1408600; 89233218CNA000001
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; carbon nanocomposites; electrocatalysis; oxygen reduction; proton exchange membrane fuel cells; single atomic Co; Energy Sciences
Citation Formats
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., and Wu, Gang. Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells. United States: N. p., 2018.
Web. doi:10.1002/adma.201706758.
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., & Wu, Gang. Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells. United States. https://doi.org/10.1002/adma.201706758
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., and Wu, Gang. Wed .
"Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells". United States. https://doi.org/10.1002/adma.201706758. https://www.osti.gov/servlets/purl/1422592.
@article{osti_1422592,
title = {Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells},
author = {Wang, Xiao Xia and Cullen, David A. and Pan, Yung-Tin and Hwang, Sooyeon and Wang, Maoyu and Feng, Zhenxing and Wang, Jingyun and Engelhard, Mark H. and Zhang, Hanguang and He, Yanghua and Shao, Yuyan and Su, Dong and More, Karren L. and Spendelow, Jacob S. and Wu, Gang},
abstractNote = {},
doi = {10.1002/adma.201706758},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {2018},
month = {1}
}
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Figure 1: STEM images and element analysis for the best performing 20Co-NC-1100 catalysts. Aberration-corrected MAADF-STEM images (a-e) with accompanying EEL point spectra (e-f). The point spectrum in (f) was taken at the dark neighboring support area in (e) and only shows C and no any N and Co. The pointmore »
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- Zhang, Huabin; Liu, Yanyu; Chen, Tao
- Advanced Materials, Vol. 31, Issue 48
Two‐Dimensional Conjugated Aromatic Networks as High‐Site‐Density and Single‐Atom Electrocatalysts for the Oxygen Reduction Reaction
journal, September 2019
- Yang, Shaoxuan; Yu, Yihuan; Dou, Meiling
- Angewandte Chemie International Edition, Vol. 58, Issue 41
Rapid and energy-efficient microwave pyrolysis for high-yield production of highly-active bifunctional electrocatalysts for water splitting
journal, January 2020
- Huang, Huawei; Zhou, Si; Yu, Chang
- Energy & Environmental Science, Vol. 13, Issue 2
Cobalt‐based coordination polymer as high activity electrocatalyst for oxygen reduction reaction: Catalysis by novel active site CoO 4 N 2
journal, December 2019
- Chen, Xin; Ge, Fan; Lai, Nanjun
- International Journal of Energy Research, Vol. 44, Issue 3
Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future
journal, January 2019
- Yang, Lijun; Shui, Jianglan; Du, Lei
- Advanced Materials, Vol. 31, Issue 13
Thermally Driven Structure and Performance Evolution of Atomically Dispersed FeN 4 Sites for Oxygen Reduction
journal, November 2019
- Li, Jiazhan; Zhang, Hanguang; Samarakoon, Widitha
- Angewandte Chemie, Vol. 131, Issue 52
Atomic‐Scale Insights into the Low‐Temperature Oxidation of Methanol over a Single‐Atom Pt 1 ‐Co 3 O 4 Catalyst
journal, April 2019
- Jiang, Zeyu; Feng, Xiangbo; Deng, Jianlin
- Advanced Functional Materials, Vol. 29, Issue 31
Cobalt Nanoparticles and Atomic Sites in Nitrogen‐Doped Carbon Frameworks for Highly Sensitive Sensing of Hydrogen Peroxide
journal, August 2019
- Li, Zehui; Liu, Rongji; Tang, Cheng
- Small, Vol. 16, Issue 15
Preparation of reduced graphite oxide loaded with cobalt(II) and nitrogen co-doped carbon polyhedrons from a metal-organic framework (type ZIF-67), and its application to electrochemical determination of metronidazole
journal, August 2019
- Chen, Han; Wu, Xingxing; Zhao, Rui
- Microchimica Acta, Vol. 186, Issue 9
Metal-Nitrogen-Carbon Catalysts for Oxygen Reduction in PEM Fuel Cells: Self-Template Synthesis Approach to Enhancing Catalytic Activity and Stability
journal, March 2019
- He, Yanghua; Tan, Qiang; Lu, Leilei
- Electrochemical Energy Reviews, Vol. 2, Issue 2
Boosting reversible oxygen electrocatalysis with enhanced interfacial pyridinic-N–Co bonding in cobalt oxide/mesoporous N-doped graphene hybrids
journal, January 2018
- Feng, Ting; Zhao, Xue-Ru; Dong, Cun-Ku
- Nanoscale, Vol. 10, Issue 47
Ultrathin‐Carbon‐Layer‐Protected PtCu Nanoparticles Encapsulated in Carbon Capsules: A Structure Engineering of the Anode Electrocatalyst for Direct Formic Acid Fuel Cells
journal, May 2019
- Xu, Min; Chen, Hong; Zhao, Yufei
- Particle & Particle Systems Characterization, Vol. 36, Issue 7
Core-Shell Polydopamine@Zr-Hemin MOFs Derived Fe-N-Doped Porous Carbon Nanospheres Electrocatalysts for the Oxygen Reduction
journal, January 2018
- Wang, Yinling; Wang, Juan; Zhang, Youliang
- Journal of The Electrochemical Society, Vol. 165, Issue 10
Direct fabrication of bimetallic AuPt nanobrick spherical nanoarchitectonics for the oxygen reduction reaction
journal, January 2019
- Narendra Kumar, Alam Venugopal; Yin, Shuli; Wang, Ziqiang
- New Journal of Chemistry, Vol. 43, Issue 24
Transition Metal–Nitrogen–Carbon (M–N–C) Catalysts for Oxygen Reduction Reaction. Insights on Synthesis and Performance in Polymer Electrolyte Fuel Cells
journal, February 2019
- Osmieri, Luigi
- ChemEngineering, Vol. 3, Issue 1
Bacterium, Fungus, and Virus Microorganisms for Energy Storage and Conversion
journal, October 2019
- Shen, Shenghui; Zhou, Rongfan; Li, Yahao
- Small Methods, Vol. 3, Issue 12
Molecular Design of Single‐Atom Catalysts for Oxygen Reduction Reaction
journal, February 2020
- Wan, Chengzhang; Duan, Xiangfeng; Huang, Yu
- Advanced Energy Materials, Vol. 10, Issue 14
Engineering Local Coordination Environments of Atomically Dispersed and Heteroatom‐Coordinated Single Metal Site Electrocatalysts for Clean Energy‐Conversion
journal, November 2019
- Zhu, Yuanzhi; Sokolowski, Joshua; Song, Xiancheng
- Advanced Energy Materials, Vol. 10, Issue 11
Single and double boron atoms doped nanoporous C 2 N– h 2D electrocatalysts for highly efficient N 2 reduction reaction: a density functional theory study
journal, May 2019
- Cao, Yongyong; Deng, Shengwei; Fang, Qiaojun
- Nanotechnology, Vol. 30, Issue 33
Hierarchically porous Fe/N–C hollow spheres derived from melamine/Fe-incorporated polydopamine for efficient oxygen reduction reaction electrocatalysis
journal, January 2019
- Feng, Bomin; Wu, Xiuju; Niu, Yanli
- Sustainable Energy & Fuels, Vol. 3, Issue 12
Tailoring FeN 4 Sites with Edge Enrichment for Boosted Oxygen Reduction Performance in Proton Exchange Membrane Fuel Cell
journal, January 2019
- Fu, Xiaogang; Li, Na; Ren, Bohua
- Advanced Energy Materials, Vol. 9, Issue 11
Thermally Driven Structure and Performance Evolution of Atomically Dispersed FeN 4 Sites for Oxygen Reduction
journal, November 2019
- Li, Jiazhan; Zhang, Hanguang; Samarakoon, Widitha
- Angewandte Chemie International Edition, Vol. 58, Issue 52
A review of non-precious metal single atom confined nanomaterials in different structural dimensions (1D–3D) as highly active oxygen redox reaction electrocatalysts
journal, January 2020
- Liu, Jin; Zhang, Hao; Qiu, Ming
- Journal of Materials Chemistry A, Vol. 8, Issue 5
Direct Growth of Carbon Nanotubes Doped with Single Atomic Fe–N 4 Active Sites and Neighboring Graphitic Nitrogen for Efficient and Stable Oxygen Reduction Electrocatalysis
journal, September 2019
- Xia, Dongsheng; Yang, Xin; Xie, Lin
- Advanced Functional Materials, Vol. 29, Issue 49
Iron‐Free Cathode Catalysts for Proton‐Exchange‐Membrane Fuel Cells: Cobalt Catalysts and the Peroxide Mitigation Approach
journal, December 2018
- Wang, Xiao Xia; Prabhakaran, Venkateshkumar; He, Yanghua
- Advanced Materials, Vol. 31, Issue 31
Static Regulation and Dynamic Evolution of Single‐Atom Catalysts in Thermal Catalytic Reactions
journal, November 2018
- Li, Hongliang; Wang, Menglin; Luo, Laihao
- Advanced Science, Vol. 6, Issue 3
Efficient Oxygen Reduction Catalysts of Porous Carbon Nanostructures Decorated with Transition Metal Species
journal, June 2019
- Huang, Xiaoxiao; Shen, Tong; Zhang, Teng
- Advanced Energy Materials, Vol. 10, Issue 11
A Single‐Atom Iridium Heterogeneous Catalyst in Oxygen Reduction Reaction
journal, June 2019
- Xiao, Meiling; Zhu, Jianbing; Li, Gaoran
- Angewandte Chemie, Vol. 131, Issue 28
Efficient Oxygen Reduction Reaction (ORR) Catalysts Based on Single Iron Atoms Dispersed on a Hierarchically Structured Porous Carbon Framework
journal, June 2018
- Zhang, Zhengping; Sun, Junting; Wang, Feng
- Angewandte Chemie International Edition, Vol. 57, Issue 29
N, P, S/Fe‐codoped Carbon Derived from Feculae Bombycis as an Efficient Electrocatalyst for Oxygen Reduction Reaction
journal, June 2019
- Meng, Hongjie; Chen, Xiaohong; Gong, Tianle
- ChemCatChem, Vol. 11, Issue 24
Highly Dispersed Cu−N X Moieties Embedded in Graphene: A Promising Electrocatalyst towards the Oxygen Reduction Reaction
journal, August 2018
- Lu, Xiangyu; Du, Lei; Wang, Dan
- ChemElectroChem, Vol. 5, Issue 21
Electrochemical Energy Conversion and Storage with Zeolitic Imidazolate Framework Derived Materials: A Perspective
journal, October 2018
- Dutta, Soumen; Liu, Zhiming; Han, HyukSu
- ChemElectroChem, Vol. 5, Issue 23
Nitrogen/Cobalt Co‐doped Mesoporous Carbon Microspheres Derived from Amorphous Metal‐Organic Frameworks as a Catalyst for the Oxygen Reduction Reaction in Both Alkaline and Acidic Electrolytes
journal, March 2019
- Bai, Yafeng; Yang, Duanguang; Yang, Mei
- ChemElectroChem, Vol. 6, Issue 9
Surface and Interface Engineering: Molybdenum Carbide–Based Nanomaterials for Electrochemical Energy Conversion
journal, September 2019
- Ge, Riyue; Huo, Juanjuan; Sun, Mingjie
- Small
3D Hierarchical Porous Graphene-Based Energy Materials: Synthesis, Functionalization, and Application in Energy Storage and Conversion
journal, March 2019
- Tang, Cheng; Wang, Hao-Fan; Huang, Jia-Qi
- Electrochemical Energy Reviews, Vol. 2, Issue 2
Bimetallic carbide of Co 3 W 3 C enhanced non-noble-metal catalysts with high activity and stability for acidic oxygen reduction reaction
journal, January 2018
- Li, Bolin; Zhou, Jianmin; Zhang, Ling
- RSC Advances, Vol. 8, Issue 22
Colloidal Co single-atom catalyst: a facile synthesis strategy and high catalytic activity for hydrogen generation
journal, January 2020
- Wang, Junkai; Huang, Zhenxia; Lu, Lilin
- Green Chemistry, Vol. 22, Issue 4
MOF nanoleaves as new sacrificial templates for the fabrication of nanoporous Co–N x /C electrocatalysts for oxygen reduction
journal, January 2019
- Li, Jingjing; Xia, Wei; Tang, Jing
- Nanoscale Horizons, Vol. 4, Issue 4
3D interconnected nitrogen-self-doped carbon aerogels as efficient oxygen reduction electrocatalysts derived from biomass gelatin
journal, January 2019
- Yang, Haoqi; Kou, Shuqing; Li, Zhiyuan
- RSC Advances, Vol. 9, Issue 69
A dinuclear cobalt cluster as electrocatalyst for oxygen reduction reaction
journal, January 2019
- Li, Yun-Wu; Zhang, Wen-Jie; Li, Chun-Xia
- RSC Advances, Vol. 9, Issue 72
Atomically Dispersed Iron Cathode Catalysts Derived from Binary Ligand-Based Zeolitic Imidazolate Frameworks with Enhanced Stability for PEM Fuel Cells
journal, January 2019
- Zhang, Hanguang; Ding, Shuo; Hwang, Sooyeon
- Journal of The Electrochemical Society, Vol. 166, Issue 7
Experimental and Theoretical Trends of PGM-Free Electrocatalysts for the Oxygen Reduction Reaction with Different Transition Metals
journal, January 2019
- Martinez, Ulises; Holby, Edward F.; Babu, Siddharth Komini
- Journal of The Electrochemical Society, Vol. 166, Issue 7
The Challenge of Achieving a High Density of Fe-Based Active Sites in a Highly Graphitic Carbon Matrix
journal, February 2019
- Li, Jingkun; Jia, Qingying; Mukerjee, Sanjeev
- Catalysts, Vol. 9, Issue 2
Carbon-Supported Single Atom Catalysts for Electrochemical Energy Conversion and Storage
journal, August 2018
- Peng, Yi; Lu, Bingzhang; Chen, Shaowei
- Advanced Materials, Vol. 30, Issue 48
X‐Ray Absorption Spectroscopy Characterizations on PGM‐Free Electrocatalysts: Justification, Advantages, and Limitations
journal, December 2018
- Jia, Qingying; Liu, Ershuai; Jiao, Li
- Advanced Materials, Vol. 31, Issue 31
PGM‐Free Cathode Catalysts for PEM Fuel Cells: A Mini‐Review on Stability Challenges
journal, December 2018
- Shao, Yuyan; Dodelet, Jean‐Pol; Wu, Gang
- Advanced Materials, Vol. 31, Issue 31
Fabricating Single‐Atom Catalysts from Chelating Metal in Open Frameworks
journal, February 2019
- Lin, Yichao; Liu, Pingying; Velasco, Ever
- Advanced Materials, Vol. 31, Issue 18
Atomic Fe‐Doped MOF‐Derived Carbon Polyhedrons with High Active‐Center Density and Ultra‐High Performance toward PEM Fuel Cells
journal, February 2019
- Deng, Yijie; Chi, Bin; Li, Jing
- Advanced Energy Materials, Vol. 9, Issue 13
Oxygen Reduction Reactions on Single‐ or Few‐Atom Discrete Active Sites for Heterogeneous Catalysis
journal, September 2019
- Sharifi, Tiva; Gracia‐Espino, Eduardo; Chen, Anran
- Advanced Energy Materials, Vol. 10, Issue 11
Efficient Oxygen Reduction Reaction (ORR) Catalysts Based on Single Iron Atoms Dispersed on a Hierarchically Structured Porous Carbon Framework
journal, June 2018
- Zhang, Zhengping; Sun, Junting; Wang, Feng
- Angewandte Chemie, Vol. 130, Issue 29
Die facettenreiche Reaktivität heterogener Einzelatom‐Katalysatoren
journal, November 2018
- Mitchell, Sharon; Vorobyeva, Evgeniya; Pérez‐Ramírez, Javier
- Angewandte Chemie, Vol. 130, Issue 47
Ultrathin Nitrogen-Doped Holey Carbon@Graphene Bifunctional Electrocatalyst for Oxygen Reduction and Evolution Reactions in Alkaline and Acidic Media
journal, November 2018
- Sun, Jiqing; Lowe, Sean E.; Zhang, Lijuan
- Angewandte Chemie, Vol. 130, Issue 50
Single Atom Catalysts on Carbon-Based Materials
journal, November 2018
- Rivera-Cárcamo, Camila; Serp, Philippe
- ChemCatChem, Vol. 10, Issue 22
Electronic and Physical Property Manipulations: Recent Achievements towards Heterogeneous Carbon‐based Catalysts for Oxygen Reduction Reaction
journal, October 2019
- Nie, Yao; Wei, Zidong
- ChemCatChem, Vol. 11, Issue 24
Insights Into the Effect of Nickel Doping on ZIF‐Derived Oxygen Reduction Catalysts for Zinc−Air Batteries
journal, February 2019
- Asokan, Arunchander; Lee, Hansol; Gwon, Ohhun
- ChemElectroChem, Vol. 6, Issue 4
Recent Progress in Precious Metal‐Free Carbon‐Based Materials towards the Oxygen Reduction Reaction: Activity, Stability, and Anti‐Poisoning
journal, November 2019
- Zhang, Ling; Li, Li; Chen, Hongmei
- Chemistry – A European Journal
Probing the Active Sites of Carbon‐Encapsulated Cobalt Nanoparticles for Oxygen Reduction
journal, February 2019
- Yan, Xuecheng; Dong, Chung‐Li; Huang, Yu‐Cheng
- Small Methods, Vol. 3, Issue 9
Metal-organic framework based nanomaterials for electrocatalytic oxygen redox reaction
journal, March 2019
- Zhang, Kexin; Guo, Wenhan; Liang, Zibin
- Science China Chemistry, Vol. 62, Issue 4
In Situ X-ray Absorption Spectroscopy Studies of Nanoscale Electrocatalysts
journal, June 2019
- Wang, Maoyu; Árnadóttir, Líney; Xu, Zhichuan J.
- Nano-Micro Letters, Vol. 11, Issue 1
Atomically dispersed manganese catalysts for oxygen reduction in proton-exchange membrane fuel cells
journal, October 2018
- Li, Jiazhan; Chen, Mengjie; Cullen, David A.
- Nature Catalysis, Vol. 1, Issue 12
The Multifaceted Reactivity of Single-Atom Heterogeneous Catalysts
text, January 2018
- Mitchell, Sharon; Vorobyeva, Evgeniya; Pérez-Ramírez, Javier
- ETH Zurich
Atomic‐ and Molecular‐Level Design of Functional Metal–Organic Frameworks (MOFs) and Derivatives for Energy and Environmental Applications
journal, August 2019
- Yilmaz, Gamze; Peh, Shing Bo; Zhao, Dan
- Advanced Science, Vol. 6, Issue 21
Two‐Dimensional Conjugated Aromatic Networks as High‐Site‐Density and Single‐Atom Electrocatalysts for the Oxygen Reduction Reaction
journal, September 2019
- Yang, Shaoxuan; Yu, Yihuan; Dou, Meiling
- Angewandte Chemie, Vol. 131, Issue 41
The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring
journal, April 2019
- Zhang, Zhiqi; Chen, Yugang; Zhou, Liqi
- Nature Communications, Vol. 10, Issue 1
Hollow Loofah‐Like N, O‐Co‐Doped Carbon Tube for Electrocatalysis of Oxygen Reduction
journal, February 2019
- Dong, Yuanyuan; Zhou, Mengwei; Tu, Wenzhe
- Advanced Functional Materials, Vol. 29, Issue 18
The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring
journal, April 2019
- Zhang, Zhiqi; Chen, Yugang; Zhou, Liqi
- Nature Communications, Vol. 10, Issue 1
Fe-doped mayenite electride composite with 2D reduced Graphene Oxide: As a non-platinum based, highly durable electrocatalyst for Oxygen Reduction Reaction
journal, December 2019
- Khan, Karim; Tareen, Ayesha Khan; Aslam, Muhammad
- Scientific Reports, Vol. 9, Issue 1
Novel Two-Dimensional Carbon–Chromium Nitride-Based Composite as an Electrocatalyst for Oxygen Reduction Reaction
journal, November 2019
- Khan, Karim; Tareen, Ayesha Khan; Aslam, Muhammad
- Frontiers in Chemistry, Vol. 7
Alloyed Pt 3 M (M = Co, Ni) nanoparticles supported on S- and N-doped carbon nanotubes for the oxygen reduction reaction
journal, January 2019
- Louisia, Stéphane; Thomas, Yohann R. J.; Lecante, Pierre
- Beilstein Journal of Nanotechnology, Vol. 10
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