Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells
- Authors:
-
[6]
- Univ. at Buffalo, NY (United States). Dept. of Chemical and Biological Engineering; East China Univ. of Science and Technology, Shanghai (China). School of Mechanical and Power Engineering
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials
- Oregon State Univ., Corvallis, OR (United States). School of Chemical, Biological, and Environmental Engineering
- Univ. at Buffalo, NY (United States). Dept. of Chemical and Biological Engineering
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States); Univ. at Buffalo, NY (United States); East China Univ. of Science and Technology, Shanghai (China); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office (HFTO); USDOE Office of Science (SC); National Science Foundation (NSF); Shanghai Natural Science Foundation of China; USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1422592
- Alternate Identifier(s):
- OSTI ID: 1417922; OSTI ID: 1558078
- Report Number(s):
- LA-UR-19-27321
Journal ID: ISSN 0935-9648; TRN: US1801631
- Grant/Contract Number:
- AC05-00OR22725; AC02-06CH11357; SC0012704; CBET-1604392; 16ZR1408600; 89233218CNA000001
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; carbon nanocomposites; electrocatalysis; oxygen reduction; proton exchange membrane fuel cells; single atomic Co; Energy Sciences
Citation Formats
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., and Wu, Gang. Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells. United States: N. p., 2018.
Web. doi:10.1002/adma.201706758.
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., & Wu, Gang. Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells. United States. https://doi.org/10.1002/adma.201706758
Wang, Xiao Xia, Cullen, David A., Pan, Yung-Tin, Hwang, Sooyeon, Wang, Maoyu, Feng, Zhenxing, Wang, Jingyun, Engelhard, Mark H., Zhang, Hanguang, He, Yanghua, Shao, Yuyan, Su, Dong, More, Karren L., Spendelow, Jacob S., and Wu, Gang. Wed .
"Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells". United States. https://doi.org/10.1002/adma.201706758. https://www.osti.gov/servlets/purl/1422592.
@article{osti_1422592,
title = {Nitrogen-Coordinated Single Cobalt Atom Catalysts for Oxygen Reduction in Proton Exchange Membrane Fuel Cells},
author = {Wang, Xiao Xia and Cullen, David A. and Pan, Yung-Tin and Hwang, Sooyeon and Wang, Maoyu and Feng, Zhenxing and Wang, Jingyun and Engelhard, Mark H. and Zhang, Hanguang and He, Yanghua and Shao, Yuyan and Su, Dong and More, Karren L. and Spendelow, Jacob S. and Wu, Gang},
abstractNote = {},
doi = {10.1002/adma.201706758},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {Wed Jan 24 00:00:00 EST 2018},
month = {Wed Jan 24 00:00:00 EST 2018}
}
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Figures / Tables:
Figure 1: STEM images and element analysis for the best performing 20Co-NC-1100 catalysts. Aberration-corrected MAADF-STEM images (a-e) with accompanying EEL point spectra (e-f). The point spectrum in (f) was taken at the dark neighboring support area in (e) and only shows C and no any N and Co. The pointmore »
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Carbon-Rich Nanomaterials: Fascinating Hydrogen and Oxygen Electrocatalysts
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Unveiling the Activity Origin of Electrocatalytic Oxygen Evolution over Isolated Ni Atoms Supported on a N‐Doped Carbon Matrix
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Two‐Dimensional Conjugated Aromatic Networks as High‐Site‐Density and Single‐Atom Electrocatalysts for the Oxygen Reduction Reaction
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Rapid and energy-efficient microwave pyrolysis for high-yield production of highly-active bifunctional electrocatalysts for water splitting
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Cobalt‐based coordination polymer as high activity electrocatalyst for oxygen reduction reaction: Catalysis by novel active site CoO 4 N 2
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Carbon‐Based Metal‐Free ORR Electrocatalysts for Fuel Cells: Past, Present, and Future
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Thermally Driven Structure and Performance Evolution of Atomically Dispersed FeN 4 Sites for Oxygen Reduction
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Atomic‐Scale Insights into the Low‐Temperature Oxidation of Methanol over a Single‐Atom Pt 1 ‐Co 3 O 4 Catalyst
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Cobalt Nanoparticles and Atomic Sites in Nitrogen‐Doped Carbon Frameworks for Highly Sensitive Sensing of Hydrogen Peroxide
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Preparation of reduced graphite oxide loaded with cobalt(II) and nitrogen co-doped carbon polyhedrons from a metal-organic framework (type ZIF-67), and its application to electrochemical determination of metronidazole
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Metal-Nitrogen-Carbon Catalysts for Oxygen Reduction in PEM Fuel Cells: Self-Template Synthesis Approach to Enhancing Catalytic Activity and Stability
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Boosting reversible oxygen electrocatalysis with enhanced interfacial pyridinic-N–Co bonding in cobalt oxide/mesoporous N-doped graphene hybrids
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Ultrathin‐Carbon‐Layer‐Protected PtCu Nanoparticles Encapsulated in Carbon Capsules: A Structure Engineering of the Anode Electrocatalyst for Direct Formic Acid Fuel Cells
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Core-Shell Polydopamine@Zr-Hemin MOFs Derived Fe-N-Doped Porous Carbon Nanospheres Electrocatalysts for the Oxygen Reduction
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Direct fabrication of bimetallic AuPt nanobrick spherical nanoarchitectonics for the oxygen reduction reaction
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Transition Metal–Nitrogen–Carbon (M–N–C) Catalysts for Oxygen Reduction Reaction. Insights on Synthesis and Performance in Polymer Electrolyte Fuel Cells
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Bacterium, Fungus, and Virus Microorganisms for Energy Storage and Conversion
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Molecular Design of Single‐Atom Catalysts for Oxygen Reduction Reaction
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Engineering Local Coordination Environments of Atomically Dispersed and Heteroatom‐Coordinated Single Metal Site Electrocatalysts for Clean Energy‐Conversion
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Single and double boron atoms doped nanoporous C 2 N– h 2D electrocatalysts for highly efficient N 2 reduction reaction: a density functional theory study
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Hierarchically porous Fe/N–C hollow spheres derived from melamine/Fe-incorporated polydopamine for efficient oxygen reduction reaction electrocatalysis
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Tailoring FeN 4 Sites with Edge Enrichment for Boosted Oxygen Reduction Performance in Proton Exchange Membrane Fuel Cell
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Thermally Driven Structure and Performance Evolution of Atomically Dispersed FeN 4 Sites for Oxygen Reduction
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A review of non-precious metal single atom confined nanomaterials in different structural dimensions (1D–3D) as highly active oxygen redox reaction electrocatalysts
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Direct Growth of Carbon Nanotubes Doped with Single Atomic Fe–N 4 Active Sites and Neighboring Graphitic Nitrogen for Efficient and Stable Oxygen Reduction Electrocatalysis
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Iron‐Free Cathode Catalysts for Proton‐Exchange‐Membrane Fuel Cells: Cobalt Catalysts and the Peroxide Mitigation Approach
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Static Regulation and Dynamic Evolution of Single‐Atom Catalysts in Thermal Catalytic Reactions
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Efficient Oxygen Reduction Catalysts of Porous Carbon Nanostructures Decorated with Transition Metal Species
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A Single‐Atom Iridium Heterogeneous Catalyst in Oxygen Reduction Reaction
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Efficient Oxygen Reduction Reaction (ORR) Catalysts Based on Single Iron Atoms Dispersed on a Hierarchically Structured Porous Carbon Framework
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Transition Metal‐Nitrogen‐Carbon Active Site for Oxygen Reduction Electrocatalysis: Beyond the Fascinations of TM‐N4
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N, P, S/Fe‐codoped Carbon Derived from Feculae Bombycis as an Efficient Electrocatalyst for Oxygen Reduction Reaction
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Highly Dispersed Cu−N X Moieties Embedded in Graphene: A Promising Electrocatalyst towards the Oxygen Reduction Reaction
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Electrochemical Energy Conversion and Storage with Zeolitic Imidazolate Framework Derived Materials: A Perspective
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Nitrogen/Cobalt Co‐doped Mesoporous Carbon Microspheres Derived from Amorphous Metal‐Organic Frameworks as a Catalyst for the Oxygen Reduction Reaction in Both Alkaline and Acidic Electrolytes
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Surface and Interface Engineering: Molybdenum Carbide–Based Nanomaterials for Electrochemical Energy Conversion
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Bimetallic carbide of Co 3 W 3 C enhanced non-noble-metal catalysts with high activity and stability for acidic oxygen reduction reaction
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Colloidal Co single-atom catalyst: a facile synthesis strategy and high catalytic activity for hydrogen generation
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MOF nanoleaves as new sacrificial templates for the fabrication of nanoporous Co–N x /C electrocatalysts for oxygen reduction
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3D interconnected nitrogen-self-doped carbon aerogels as efficient oxygen reduction electrocatalysts derived from biomass gelatin
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A dinuclear cobalt cluster as electrocatalyst for oxygen reduction reaction
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Atomically Dispersed Iron Cathode Catalysts Derived from Binary Ligand-Based Zeolitic Imidazolate Frameworks with Enhanced Stability for PEM Fuel Cells
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Experimental and Theoretical Trends of PGM-Free Electrocatalysts for the Oxygen Reduction Reaction with Different Transition Metals
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The Challenge of Achieving a High Density of Fe-Based Active Sites in a Highly Graphitic Carbon Matrix
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Carbon-Supported Single Atom Catalysts for Electrochemical Energy Conversion and Storage
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X‐Ray Absorption Spectroscopy Characterizations on PGM‐Free Electrocatalysts: Justification, Advantages, and Limitations
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PGM‐Free Cathode Catalysts for PEM Fuel Cells: A Mini‐Review on Stability Challenges
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Fabricating Single‐Atom Catalysts from Chelating Metal in Open Frameworks
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Atomic Fe‐Doped MOF‐Derived Carbon Polyhedrons with High Active‐Center Density and Ultra‐High Performance toward PEM Fuel Cells
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Oxygen Reduction Reactions on Single‐ or Few‐Atom Discrete Active Sites for Heterogeneous Catalysis
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Efficient Oxygen Reduction Reaction (ORR) Catalysts Based on Single Iron Atoms Dispersed on a Hierarchically Structured Porous Carbon Framework
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Die facettenreiche Reaktivität heterogener Einzelatom‐Katalysatoren
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Ultrathin Nitrogen-Doped Holey Carbon@Graphene Bifunctional Electrocatalyst for Oxygen Reduction and Evolution Reactions in Alkaline and Acidic Media
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Single Atom Catalysts on Carbon-Based Materials
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Electronic and Physical Property Manipulations: Recent Achievements towards Heterogeneous Carbon‐based Catalysts for Oxygen Reduction Reaction
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Insights Into the Effect of Nickel Doping on ZIF‐Derived Oxygen Reduction Catalysts for Zinc−Air Batteries
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Recent Progress in Precious Metal‐Free Carbon‐Based Materials towards the Oxygen Reduction Reaction: Activity, Stability, and Anti‐Poisoning
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Probing the Active Sites of Carbon‐Encapsulated Cobalt Nanoparticles for Oxygen Reduction
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In Situ X-ray Absorption Spectroscopy Studies of Nanoscale Electrocatalysts
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The Multifaceted Reactivity of Single-Atom Heterogeneous Catalysts
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Atomic‐ and Molecular‐Level Design of Functional Metal–Organic Frameworks (MOFs) and Derivatives for Energy and Environmental Applications
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Two‐Dimensional Conjugated Aromatic Networks as High‐Site‐Density and Single‐Atom Electrocatalysts for the Oxygen Reduction Reaction
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The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring
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Hollow Loofah‐Like N, O‐Co‐Doped Carbon Tube for Electrocatalysis of Oxygen Reduction
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The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring
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Fe-doped mayenite electride composite with 2D reduced Graphene Oxide: As a non-platinum based, highly durable electrocatalyst for Oxygen Reduction Reaction
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Novel Two-Dimensional Carbon–Chromium Nitride-Based Composite as an Electrocatalyst for Oxygen Reduction Reaction
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Alloyed Pt 3 M (M = Co, Ni) nanoparticles supported on S- and N-doped carbon nanotubes for the oxygen reduction reaction
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