Magnetic Resonance with Squeezed Microwaves
Abstract
Vacuum fluctuations of the electromagnetic field set a fundamental limit to the sensitivity of a variety of measurements, including magnetic resonance spectroscopy. We report the use of squeezed microwave fields, which are engineered quantum states of light for which fluctuations in one field quadrature are reduced below the vacuum level, to enhance the detection sensitivity of an ensemble of electronic spins at millikelvin temperatures. By shining a squeezed vacuum state on the input port of a microwave resonator containing the spins, we obtain a 1.2-dB noise reduction at the spectrometer output compared to the case of a vacuum input. This result constitutes a proof of principle of the application of quantum metrology to magnetic resonance spectroscopy.
- Authors:
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1399805
- Alternate Identifier(s):
- OSTI ID: 1421828
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Published Article
- Journal Name:
- Physical Review. X
- Additional Journal Information:
- Journal Name: Physical Review. X Journal Volume: 7 Journal Issue: 4; Journal ID: ISSN 2160-3308
- Publisher:
- American Physical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
Citation Formats
Bienfait, A., Campagne-Ibarcq, P., Kiilerich, A. H., Zhou, X., Probst, S., Pla, J. J., Schenkel, T., Vion, D., Esteve, D., Morton, J. J. L., Moelmer, K., and Bertet, P. Magnetic Resonance with Squeezed Microwaves. United States: N. p., 2017.
Web. doi:10.1103/PhysRevX.7.041011.
Bienfait, A., Campagne-Ibarcq, P., Kiilerich, A. H., Zhou, X., Probst, S., Pla, J. J., Schenkel, T., Vion, D., Esteve, D., Morton, J. J. L., Moelmer, K., & Bertet, P. Magnetic Resonance with Squeezed Microwaves. United States. https://doi.org/10.1103/PhysRevX.7.041011
Bienfait, A., Campagne-Ibarcq, P., Kiilerich, A. H., Zhou, X., Probst, S., Pla, J. J., Schenkel, T., Vion, D., Esteve, D., Morton, J. J. L., Moelmer, K., and Bertet, P. Tue .
"Magnetic Resonance with Squeezed Microwaves". United States. https://doi.org/10.1103/PhysRevX.7.041011.
@article{osti_1399805,
title = {Magnetic Resonance with Squeezed Microwaves},
author = {Bienfait, A. and Campagne-Ibarcq, P. and Kiilerich, A. H. and Zhou, X. and Probst, S. and Pla, J. J. and Schenkel, T. and Vion, D. and Esteve, D. and Morton, J. J. L. and Moelmer, K. and Bertet, P.},
abstractNote = {Vacuum fluctuations of the electromagnetic field set a fundamental limit to the sensitivity of a variety of measurements, including magnetic resonance spectroscopy. We report the use of squeezed microwave fields, which are engineered quantum states of light for which fluctuations in one field quadrature are reduced below the vacuum level, to enhance the detection sensitivity of an ensemble of electronic spins at millikelvin temperatures. By shining a squeezed vacuum state on the input port of a microwave resonator containing the spins, we obtain a 1.2-dB noise reduction at the spectrometer output compared to the case of a vacuum input. This result constitutes a proof of principle of the application of quantum metrology to magnetic resonance spectroscopy.},
doi = {10.1103/PhysRevX.7.041011},
journal = {Physical Review. X},
number = 4,
volume = 7,
place = {United States},
year = {Tue Oct 17 00:00:00 EDT 2017},
month = {Tue Oct 17 00:00:00 EDT 2017}
}
https://doi.org/10.1103/PhysRevX.7.041011
Web of Science
Works referenced in this record:
Electrical activation and electron spin resonance measurements of implanted bismuth in isotopically enriched silicon-28
journal, April 2012
- Weis, C. D.; Lo, C. C.; Lang, V.
- Applied Physics Letters, Vol. 100, Issue 17
Heisenberg-Limited Qubit Read-Out with Two-Mode Squeezed Light
journal, August 2015
- Didier, Nicolas; Kamal, Archana; Oliver, William D.
- Physical Review Letters, Vol. 115, Issue 9
Biological measurement beyond the quantum limit
journal, February 2013
- Taylor, Michael A.; Janousek, Jiri; Daria, Vincent
- Nature Photonics, Vol. 7, Issue 3
Observing single quantum trajectories of a superconducting quantum bit
journal, October 2013
- Murch, K. W.; Weber, S. J.; Macklin, C.
- Nature, Vol. 502, Issue 7470
Fast Quantum Nondemolition Readout by Parametric Modulation of Longitudinal Qubit-Oscillator Interaction
journal, November 2015
- Didier, Nicolas; Bourassa, Jérôme; Blais, Alexandre
- Physical Review Letters, Vol. 115, Issue 20
Input and output in damped quantum systems: Quantum stochastic differential equations and the master equation
journal, June 1985
- Gardiner, C. W.; Collett, M. J.
- Physical Review A, Vol. 31, Issue 6
Nuclear-spin noise
journal, October 1985
- Sleator, Tycho; Hahn, Erwin L.; Hilbert, Claude
- Physical Review Letters, Vol. 55, Issue 17
Quantum-Enhanced Measurements: Beating the Standard Quantum Limit
journal, November 2004
- Giovannetti, V.
- Science, Vol. 306, Issue 5700
Spectroscopy with squeezed light
journal, May 1992
- Polzik, E. S.; Carri, J.; Kimble, H. J.
- Physical Review Letters, Vol. 68, Issue 20
Broadband parametric amplification with impedance engineering: Beyond the gain-bandwidth product
journal, December 2015
- Roy, Tanay; Kundu, Suman; Chand, Madhavi
- Applied Physics Letters, Vol. 107, Issue 26
Inhibition of Atomic Phase Decays by Squeezed Light: A Direct Effect of Squeezing
journal, May 1986
- Gardiner, C. W.
- Physical Review Letters, Vol. 56, Issue 18
Strong environmental coupling in a Josephson parametric amplifier
journal, June 2014
- Mutus, J. Y.; White, T. C.; Barends, R.
- Applied Physics Letters, Vol. 104, Issue 26
Reduction of the radiative decay of atomic coherence in squeezed vacuum
journal, July 2013
- Murch, K. W.; Weber, S. J.; Beck, K. M.
- Nature, Vol. 499, Issue 7456
Quantum State Tomography of an Itinerant Squeezed Microwave Field
journal, June 2011
- Mallet, F.; Castellanos-Beltran, M. A.; Ku, H. S.
- Physical Review Letters, Vol. 106, Issue 22
Field Dependence of the Intrinsic Domain Magnetization of a Ferromagnet
journal, December 1940
- Holstein, T.; Primakoff, H.
- Physical Review, Vol. 58, Issue 12
Reaching the quantum limit of sensitivity in electron spin resonance
journal, December 2015
- Bienfait, A.; Pla, J. J.; Kubo, Y.
- Nature Nanotechnology, Vol. 11, Issue 3
A near-quantum-limited Josephson traveling-wave parametric amplifier
journal, September 2015
- Macklin, C.; O'Brien, K.; Hover, D.
- Science, Vol. 350, Issue 6258
High-gain weakly nonlinear flux-modulated Josephson parametric amplifier using a SQUID array
journal, June 2014
- Zhou, X.; Schmitt, V.; Bertet, P.
- Physical Review B, Vol. 89, Issue 21
Observation of zero-point noise squeezing via a Josephson-parametric amplifier
journal, September 1990
- Movshovich, R.; Yurke, B.; Kaminsky, P. G.
- Physical Review Letters, Vol. 65, Issue 12
Phase-preserving amplification near the quantum limit with a Josephson ring modulator
journal, May 2010
- Bergeal, N.; Schackert, F.; Metcalfe, M.
- Nature, Vol. 465, Issue 7294
Squeezed-light – enhanced polarization interferometer
journal, November 1987
- Grangier, P.; Slusher, R. E.; Yurke, B.
- Physical Review Letters, Vol. 59, Issue 19
Electron spin coherence exceeding seconds in high-purity silicon
journal, December 2011
- Tyryshkin, Alexei M.; Tojo, Shinichi; Morton, John J. L.
- Nature Materials, Vol. 11, Issue 2
Enhanced sensitivity of the LIGO gravitational wave detector by using squeezed states of light
journal, July 2013
- Aasi, J.; Abadie, J.; Abbott, B. P.
- Nature Photonics, Vol. 7, Issue 8
Proposal for detecting a single electron spin in a microwave resonator
journal, February 2017
- Haikka, P.; Kubo, Y.; Bienfait, A.
- Physical Review A, Vol. 95, Issue 2
Observation of Squeezed States Generated by Four-Wave Mixing in an Optical Cavity
journal, November 1985
- Slusher, R. E.; Hollberg, L. W.; Yurke, B.
- Physical Review Letters, Vol. 55, Issue 22
Squeezed-light spin noise spectroscopy
journal, May 2016
- Lucivero, Vito Giovanni; Jiménez-Martínez, Ricardo; Kong, Jia
- Physical Review A, Vol. 93, Issue 5
Generation of Squeezed States by Parametric Down Conversion
journal, November 1986
- Wu, Ling-An; Kimble, H. J.; Hall, J. L.
- Physical Review Letters, Vol. 57, Issue 20
A sensitive electrometer based on a Rydberg atom in a Schrödinger-cat state
journal, July 2016
- Facon, Adrien; Dietsche, Eva-Katharina; Grosso, Dorian
- Nature, Vol. 535, Issue 7611
Enhanced qubit readout using locally generated squeezing and inbuilt Purcell-decay suppression
journal, February 2017
- Govia, Luke C. G.; Clerk, Aashish A.
- New Journal of Physics, Vol. 19, Issue 2
Observation of strong radiation pressure forces from squeezed light on a mechanical oscillator
journal, March 2016
- Clark, Jeremy B.; Lecocq, Florent; Simmonds, Raymond W.
- Nature Physics, Vol. 12, Issue 7
Nonreciprocal Microwave Signal Processing with a Field-Programmable Josephson Amplifier
journal, February 2017
- Lecocq, F.; Ranzani, L.; Peterson, G. A.
- Physical Review Applied, Vol. 7, Issue 2
Controlling spin relaxation with a cavity
journal, February 2016
- Bienfait, A.; Pla, J. J.; Kubo, Y.
- Nature, Vol. 531, Issue 7592
Superconducting Circuits for Quantum Information: An Outlook
journal, March 2013
- Devoret, M. H.; Schoelkopf, R. J.
- Science, Vol. 339, Issue 6124
Atomic clock transitions in silicon-based spin qubits
journal, June 2013
- Wolfowicz, Gary; Tyryshkin, Alexei M.; George, Richard E.
- Nature Nanotechnology, Vol. 8, Issue 8
Quantum-mechanical noise in an interferometer
journal, April 1981
- Caves, Carlton M.
- Physical Review D, Vol. 23, Issue 8
Sideband cooling beyond the quantum backaction limit with squeezed light
journal, January 2017
- Clark, Jeremy B.; Lecocq, Florent; Simmonds, Raymond W.
- Nature, Vol. 541, Issue 7636
Parametric resonance in tunable superconducting cavities
journal, May 2013
- Wustmann, Waltraut; Shumeiko, Vitaly
- Physical Review B, Vol. 87, Issue 18
Reconfigurable Josephson Circulator/Directional Amplifier
journal, November 2015
- Sliwa, K. M.; Hatridge, M.; Narla, A.
- Physical Review X, Vol. 5, Issue 4
Widely tunable parametric amplifier based on a superconducting quantum interference device array resonator
journal, August 2007
- Castellanos-Beltran, M. A.; Lehnert, K. W.
- Applied Physics Letters, Vol. 91, Issue 8
Resonance Fluorescence from an Artificial Atom in Squeezed Vacuum
journal, July 2016
- Toyli, D. M.; Eddins, A. W.; Boutin, S.
- Physical Review X, Vol. 6, Issue 3
Precision measurement beyond the shot-noise limit
journal, July 1987
- Xiao, Min; Wu, Ling-An; Kimble, H. J.
- Physical Review Letters, Vol. 59, Issue 3
On-Chip Superconducting Microwave Circulator from Synthetic Rotation
journal, September 2015
- Kerckhoff, Joseph; Lalumière, Kevin; Chapman, Benjamin J.
- Physical Review Applied, Vol. 4, Issue 3