Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces

Vabishchevich, Polina P.; Liu, Sheng; Sinclair, Michael B.; Keeler, Gordon A.; Peake, Gregory M.; Brener, Igal

doi:10.1021/acsphotonics.7b01478

Title: Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces

Journal Article · 27 January 2018 · ACS Photonics

DOI: https://doi.org/10.1021/acsphotonics.7b01478 · OSTI ID:1421766

^[1]; Liu, Sheng ^[1]; Sinclair, Michael B. ^[1]; Keeler, Gordon A. ^[1]; Peake, Gregory M. ^[1];

^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

All-dielectric metasurfaces, two-dimensional arrays of subwavelength low loss dielectric inclusions, can be used not only to control the amplitude and phase of optical beams, but also to generate new wavelengths through enhanced nonlinear optical processes that are free from some of the constraints dictated by the use of bulk materials. Recently, high quality factor (Q) resonances in these metasurfaces have been revealed and utilized for applications such as sensing and lasing. The origin of these resonances stems from the interference of two nanoresonator modes with vastly different Q. Here we show that nonlinear optical processes can be further enhanced by utilizing these high-Q resonances in broken symmetry all-dielectric metasurfaces. As a result, we study second harmonic generation from broken symmetry metasurfaces made from III–V semiconductors and observe nontrivial spectral shaping of second-harmonic and multifold efficiency enhancement induced by high field localization and enhancement inside the nanoresonators.

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1421766

Report Number(s):: SAND-2018-1266J; 660514

Journal Information:: ACS Photonics, Vol. 5, Issue 5; ISSN 2330-4022

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 176 works

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