Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces
Abstract
All-dielectric metasurfaces, two-dimensional arrays of subwavelength low loss dielectric inclusions, can be used not only to control the amplitude and phase of optical beams, but also to generate new wavelengths through enhanced nonlinear optical processes that are free from some of the constraints dictated by the use of bulk materials. Recently, high quality factor (Q) resonances in these metasurfaces have been revealed and utilized for applications such as sensing and lasing. The origin of these resonances stems from the interference of two nanoresonator modes with vastly different Q. Here we show that nonlinear optical processes can be further enhanced by utilizing these high-Q resonances in broken symmetry all-dielectric metasurfaces. As a result, we study second harmonic generation from broken symmetry metasurfaces made from III–V semiconductors and observe nontrivial spectral shaping of second-harmonic and multifold efficiency enhancement induced by high field localization and enhancement inside the nanoresonators.
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1421766
- Report Number(s):
- SAND-2018-1266J
Journal ID: ISSN 2330-4022; 660514
- Grant/Contract Number:
- AC04-94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Photonics
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 5; Journal ID: ISSN 2330-4022
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; dielectric metasurfaces; Fano resonances; III−V semiconductors; second-harmonic generation
Citation Formats
Vabishchevich, Polina P., Liu, Sheng, Sinclair, Michael B., Keeler, Gordon A., Peake, Gregory M., and Brener, Igal. Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces. United States: N. p., 2018.
Web. doi:10.1021/acsphotonics.7b01478.
Vabishchevich, Polina P., Liu, Sheng, Sinclair, Michael B., Keeler, Gordon A., Peake, Gregory M., & Brener, Igal. Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces. United States. https://doi.org/10.1021/acsphotonics.7b01478
Vabishchevich, Polina P., Liu, Sheng, Sinclair, Michael B., Keeler, Gordon A., Peake, Gregory M., and Brener, Igal. Sat .
"Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces". United States. https://doi.org/10.1021/acsphotonics.7b01478. https://www.osti.gov/servlets/purl/1421766.
@article{osti_1421766,
title = {Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces},
author = {Vabishchevich, Polina P. and Liu, Sheng and Sinclair, Michael B. and Keeler, Gordon A. and Peake, Gregory M. and Brener, Igal},
abstractNote = {All-dielectric metasurfaces, two-dimensional arrays of subwavelength low loss dielectric inclusions, can be used not only to control the amplitude and phase of optical beams, but also to generate new wavelengths through enhanced nonlinear optical processes that are free from some of the constraints dictated by the use of bulk materials. Recently, high quality factor (Q) resonances in these metasurfaces have been revealed and utilized for applications such as sensing and lasing. The origin of these resonances stems from the interference of two nanoresonator modes with vastly different Q. Here we show that nonlinear optical processes can be further enhanced by utilizing these high-Q resonances in broken symmetry all-dielectric metasurfaces. As a result, we study second harmonic generation from broken symmetry metasurfaces made from III–V semiconductors and observe nontrivial spectral shaping of second-harmonic and multifold efficiency enhancement induced by high field localization and enhancement inside the nanoresonators.},
doi = {10.1021/acsphotonics.7b01478},
journal = {ACS Photonics},
number = 5,
volume = 5,
place = {United States},
year = {2018},
month = {1}
}
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Figure 1: Symmetry broken GaAs metasurface used to create high-Q Fano resonances. (a) Schematic of a Fano-resonant metasurface design, based on a cube with a ∼300 nm side that has a notch cut from the corner. Inset top: a top-view SEM image of the fabricated Fano metasurface. Inset bottom: amore »
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Works referenced in this record:
Colloquium : Nonlinear metamaterials
journal, September 2014
- Lapine, Mikhail; Shadrivov, Ilya V.; Kivshar, Yuri S.
- Reviews of Modern Physics, Vol. 86, Issue 3
Nonlinear photonic metasurfaces
journal, March 2017
- Li, Guixin; Zhang, Shuang; Zentgraf, Thomas
- Nature Reviews Materials, Vol. 2, Issue 5
Nonlinear metasurfaces: a paradigm shift in nonlinear optics
journal, January 2018
- Krasnok, Alexander; Tymchenko, Mykhailo; Alù, Andrea
- Materials Today, Vol. 21, Issue 1
Nonlinear plasmonics
journal, November 2012
- Kauranen, Martti; Zayats, Anatoly V.
- Nature Photonics, Vol. 6, Issue 11
Magnetic light
journal, July 2012
- Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Fu, Yuan Hsing
- Scientific Reports, Vol. 2, Issue 1
Optically resonant dielectric nanostructures
journal, November 2016
- Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L.
- Science, Vol. 354, Issue 6314
Resonantly Enhanced Second-Harmonic Generation Using III–V Semiconductor All-Dielectric Metasurfaces
journal, August 2016
- Liu, Sheng; Sinclair, Michael B.; Saravi, Sina
- Nano Letters, Vol. 16, Issue 9, p. 5426-5432
Nonlinear Generation of Vector Beams From AlGaAs Nanoantennas
journal, October 2016
- Camacho-Morales, Rocio; Rahmani, Mohsen; Kruk, Sergey
- Nano Letters, Vol. 16, Issue 11, p. 7191-7197
Monolithic AlGaAs second-harmonic nanoantennas
journal, January 2016
- Gili, V. F.; Carletti, L.; Locatelli, A.
- Optics Express, Vol. 24, Issue 14, p. 15965-15971
Nonlinear Optical Magnetism Revealed by Second-Harmonic Generation in Nanoantennas
journal, May 2017
- Kruk, Sergey S.; Camacho-Morales, Rocio; Xu, Lei
- Nano Letters, Vol. 17, Issue 6, p. 3914-3918
III–V Semiconductor Nanoresonators—A New Strategy for Passive, Active, and Nonlinear All‐Dielectric Metamaterials
journal, June 2016
- Liu, Sheng; Keeler, Gordon A.; Reno, John L.
- Advanced Optical Materials, Vol. 4, Issue 10
Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response
journal, October 2014
- Shcherbakov, Maxim R.; Neshev, Dragomir N.; Hopkins, Ben
- Nano Letters, Vol. 14, Issue 11, p. 6488-6492
Efficient Third Harmonic Generation and Nonlinear Subwavelength Imaging at a Higher-Order Anapole Mode in a Single Germanium Nanodisk
journal, December 2016
- Grinblat, Gustavo; Li, Yi; Nielsen, Michael P.
- ACS Nano, Vol. 11, Issue 1
Degenerate Four-Wave Mixing in a Multiresonant Germanium Nanodisk
journal, August 2017
- Grinblat, Gustavo; Li, Yi; Nielsen, Michael P.
- ACS Photonics, Vol. 4, Issue 9
Third-harmonic generation from Mie-type resonances of isolated all-dielectric nanoparticles
journal, March 2017
- Melik-Gaykazyan, Elizaveta V.; Shcherbakov, Maxim R.; Shorokhov, Alexander S.
- Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 375, Issue 2090
Nonlinear Fano-Resonant Dielectric Metasurfaces
journal, October 2015
- Yang, Yuanmu; Wang, Wenyi; Boulesbaa, Abdelaziz
- Nano Letters, Vol. 15, Issue 11, p. 7388-7393
Multifold Enhancement of Third-Harmonic Generation in Dielectric Nanoparticles Driven by Magnetic Fano Resonances
journal, July 2016
- Shorokhov, Alexander S.; Melik-Gaykazyan, Elizaveta V.; Smirnova, Daria A.
- Nano Letters, Vol. 16, Issue 8
Fano resonances in nanoscale structures
journal, August 2010
- Miroshnichenko, Andrey E.; Flach, Sergej; Kivshar, Yuri S.
- Reviews of Modern Physics, Vol. 82, Issue 3
Optical Fano resonance of an individual semiconductor nanostructure
journal, April 2014
- Fan, Pengyu; Yu, Zongfu; Fan, Shanhui
- Nature Materials, Vol. 13, Issue 5
The Fano resonance in plasmonic nanostructures and metamaterials
journal, August 2010
- Luk'yanchuk, Boris; Zheludev, Nikolay I.; Maier, Stefan A.
- Nature Materials, Vol. 9, Issue 9
Spectrally selective chiral silicon metasurfaces based on infrared Fano resonances
journal, May 2014
- Wu, Chihhui; Arju, Nihal; Kelp, Glen
- Nature Communications, Vol. 5, Article No. 3892
Fano Resonances in All-Dielectric Oligomers
journal, February 2012
- Miroshnichenko, Andrey E.; Kivshar, Yuri S.
- Nano Letters, Vol. 12, Issue 12
Observation of Fano Resonances in All-Dielectric Nanoparticle Oligomers
journal, February 2014
- Chong, Katie E.; Hopkins, Ben; Staude, Isabelle
- Small, Vol. 10, Issue 10
Broken Symmetry Dielectric Resonators for High Quality Factor Fano Metasurfaces
journal, November 2016
- Campione, Salvatore; Liu, Sheng; Basilio, Lorena I.
- ACS Photonics, Vol. 3, Issue 12, p. 2362-2367
Works referencing / citing this record:
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation
journal, January 2019
- Huang, Zhijin; Lu, Huihui; Xiong, Hanqing
- Nanomaterials, Vol. 9, Issue 1
Second harmonic generation in monolithic lithium niobate metasurfaces
journal, January 2019
- Carletti, Luca; Li, Cheng; Sautter, Jürgen
- Optics Express, Vol. 27, Issue 23
Spontaneous photon-pair generation from a dielectric nanoantenna
journal, January 2019
- Marino, Giuseppe; Solntsev, Alexander S.; Xu, Lei
- Optica, Vol. 6, Issue 11
Recent Progress in Active Optical Metasurfaces
journal, April 2019
- Kang, Lei; Jenkins, Ronald P.; Werner, Douglas H.
- Advanced Optical Materials, Vol. 7, Issue 14
Resonant dielectric metasurfaces: active tuning and nonlinear effects
journal, July 2019
- Zou, Chengjun; Sautter, Jürgen; Setzpfandt, Frank
- Journal of Physics D: Applied Physics, Vol. 52, Issue 37
Asymmetric Metasurfaces with High- Resonances Governed by Bound States in the Continuum
journal, November 2018
- Koshelev, Kirill; Lepeshov, Sergey; Liu, Mingkai
- Physical Review Letters, Vol. 121, Issue 19
Fano-resonant silicon photonic crystal slab for efficient third-harmonic generation
journal, December 2018
- Ban, Guoxun; Gong, Cheng; Zhou, Chaobiao
- Optics Letters, Vol. 44, Issue 1
Tailored Nonlinear Anisotropy in Mie‐Resonant Dielectric Oligomers
journal, July 2019
- Kroychuk, Maria K.; Yagudin, Damir F.; Shorokhov, Alexander S.
- Advanced Optical Materials, Vol. 7, Issue 20
All‐Dielectric Silicon Metasurface with Strong Subterahertz Toroidal Dipole Resonance
journal, July 2019
- Zografopoulos, Dimitrios C.; Ferraro, Antonio; Algorri, José Francisco
- Advanced Optical Materials, Vol. 7, Issue 19
Interaction of semiconductor metasurfaces with short laser pulses: From nonlinear-optical response toward spatiotemporal shaping
journal, August 2019
- Shcherbakov, M. R.; Eilenberger, F.; Staude, I.
- Journal of Applied Physics, Vol. 126, Issue 8
Resonant harmonic generation in AlGaAs nanoantennas probed by cylindrical vector beams
journal, January 2019
- Camacho-Morales, Rocio; Bautista, Godofredo; Zang, Xiaorun
- Nanoscale, Vol. 11, Issue 4
Nonradiating photonics with resonant dielectric nanostructures
journal, March 2019
- Koshelev, Kirill; Favraud, Gael; Bogdanov, Andrey
- Nanophotonics, Vol. 8, Issue 5
Second-harmonic generation in Mie-resonant dielectric nanoparticles made of noncentrosymmetric materials
journal, February 2019
- Frizyuk, Kristina; Volkovskaya, Irina; Smirnova, Daria
- Physical Review B, Vol. 99, Issue 7
Trapping and filtering of light by single Si nanospheres in a GaAs nanocavity
journal, January 2019
- Huang, Yingcong; Yan, Jiahao; Ma, Churong
- Nanoscale, Vol. 11, Issue 35
Fano resonant behaviour of waveguide mode in all-dielectric multilayer structure directly monitored by fluorescence of embedded dye molecules
journal, September 2019
- Kang, Byungjun; Motokura, Kengo; Fujii, Minoru
- Journal of Optics, Vol. 21, Issue 10
Boosting Second Harmonic Radiation from AlGaAs Nanoantennas with Epsilon-Near-Zero Materials
journal, November 2018
- Rocco, Davide; Vincenti, Maria; De Angelis, Costantino
- Applied Sciences, Vol. 8, Issue 11
Highly-Efficient Longitudinal Second-Harmonic Generation from Doubly-Resonant AlGaAs Nanoantennas
journal, September 2018
- Xu, Lei; Rahmani, Mohsen; Smirnova, Daria
- Photonics, Vol. 5, Issue 3
Symmetry‐Protected Dual Bound States in the Continuum in Metamaterials
journal, May 2019
- Cong, Longqing; Singh, Ranjan
- Advanced Optical Materials
Toroidal metasurface resonances in microwave waveguides
journal, May 2019
- Zografopoulos, Dimitrios C.; Algorri, José Francisco; Ferraro, Antonio
- Scientific Reports, Vol. 9, Issue 1
Active tuning of the Fano resonance from a Si nanosphere dimer by the substrate effect
journal, January 2019
- Huang, Yingcong; Yan, Jiahao; Ma, Churong
- Nanoscale Horizons, Vol. 4, Issue 1
All-optical tuning of symmetry protected quasi bound states in the continuum
journal, September 2019
- Karl, Nicholas; Vabishchevich, Polina P.; Liu, Sheng
- Applied Physics Letters, Vol. 115, Issue 14
Symmetry-protected bound states in the continuum supported by all-dielectric metasurfaces
journal, December 2019
- Li, Shiyu; Zhou, Chaobiao; Liu, Tingting
- Physical Review A, Vol. 100, Issue 6
Overcoming the efficiency-bandwidth tradeoff for optical harmonics generation using nonlinear time-variant resonators
journal, December 2019
- Shcherbakov, Maxim R.; Shafirin, Pavel; Shvets, Gennady
- Physical Review A, Vol. 100, Issue 6
Second-harmonic generation in Mie-resonant dielectric nanoparticles made of noncentrosymmetric materials
text, January 2018
- Frizyuk, Kristina; Volkovskaya, Irina; Smirnova, Daria
- arXiv
Toroidal metasurface resonances in microwave waveguides
journal, May 2019
- Zografopoulos, Dimitrios C.; Algorri, José Francisco; Ferraro, Antonio
- Scientific Reports, Vol. 9, Issue 1
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation
journal, January 2019
- Huang, Zhijin; Lu, Huihui; Xiong, Hanqing
- Nanomaterials, Vol. 9, Issue 1
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