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This content will become publicly available on January 29, 2019

Title: Four-Wave-Mixing Approach to In Situ Detection of Nanoparticles

Here, we report on the development and experimental validation of a laser-based technique which uses coherent Rayleigh-Brillouin scattering (CRBS) to detect nanoparticles with characteristic sizes ranging from the atomic scale to tens of nanometers. This technique is aimed (nonexclusively) at the detection of nanoparticles produced by volumetric nanoparticle synthesis methods. Using CRBS, carbon nanoparticles of dimensions less than 10 nm and concentrations of 10 10 cm –3 are detected in situ in a carbon arc discharge with graphite electrodes. This four-wave-mixing approach should enable advances in the understanding of nanoparticle growth that could potentially lead to improved modeling of the growth mechanisms, and thus to improve synthesis selectivity of nanoparticles and yield.
Authors:
 [1] ;  [2] ;  [2] ;  [1] ;  [1] ;  [1]
  1. Princeton Plasma Physics Lab. (PPPL), Princeton, NJ (United States)
  2. Princeton Univ., Princeton, NJ (United States)
Publication Date:
Grant/Contract Number:
AC02-09CH11466
Type:
Accepted Manuscript
Journal Name:
Physical Review Applied
Additional Journal Information:
Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2331-7019
Publisher:
American Physical Society (APS)
Research Org:
Princeton Plasma Physics Lab. (PPPL), Princeton, NJ (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
OSTI Identifier:
1420375
Alternate Identifier(s):
OSTI ID: 1418392