Application, Deactivation, and Regeneration of Heterogeneous Catalysts in Bio-Oil Upgrading

Cheng, Shouyun; Wei, Lin; Zhao, Xianhui; Julson, James

doi:10.3390/catal6120195

Title: Application, Deactivation, and Regeneration of Heterogeneous Catalysts in Bio-Oil Upgrading

Journal Article · 07 December 2016 · Catalysts

DOI: https://doi.org/10.3390/catal6120195 · OSTI ID:1419689

^[1]; Wei, Lin ^[1]; Zhao, Xianhui ^[1]; Julson, James ^[1]

South Dakota State Univ., Brookings, SD (United States)

The massive consumption of fossil fuels and associated environmental issues are leading to an increased interest in alternative resources such as biofuels. The renewable biofuels can be upgraded from bio-oils that are derived from biomass pyrolysis. Catalytic cracking and hydrodeoxygenation (HDO) are two of the most promising bio-oil upgrading processes for biofuel production. Heterogeneous catalysts are essential for upgrading bio-oil into hydrocarbon biofuel. Although advances have been achieved, the deactivation and regeneration of catalysts still remains a challenge. This review focuses on the current progress and challenges of heterogeneous catalyst application, deactivation, and regeneration. The technologies of catalysts deactivation, reduction, and regeneration for improving catalyst activity and stability are discussed. Some suggestions for future research including catalyst mechanism, catalyst development, process integration, and biomass modification for the production of hydrocarbon biofuels are provided.

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Research Organization:: South Dakota State Univ., Brookings, SD (United States)

Sponsoring Organization:: USDOE; Dept. of Transportation (DOT) (United States)

Grant/Contract Number:: SA0900160; SA0700149; SA1600799

OSTI ID:: 1419689

Alternate ID(s):: OSTI ID: 1395954

Journal Information:: Catalysts, Vol. 6, Issue 12; ISSN 2073-4344

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 98 works

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Overview of catalytic upgrading of biomass pyrolysis vapors toward the production of fuels and high-value chemicals Iliopoulou, Eleni F.; Triantafyllidis, Kostas S.; Lappas, Angelos A. Wiley Interdisciplinary Reviews: Energy and Environment, Vol. 8, Issue 1 https://doi.org/10.1002/wene.322	journal	August 2018
Efficient deoxygenation of waste cooking oil over Co ₃ O ₄ –La ₂ O ₃ -doped activated carbon for the production of diesel-like fuel Abdulkareem-Alsultan, G.; Asikin-Mijan, N.; Mustafa-Alsultan, G. RSC Advances, Vol. 10, Issue 9 https://doi.org/10.1039/c9ra09516k	journal	January 2020
Transition Metal Phosphides for the Catalytic Hydrodeoxygenation of Waste Oils into Green Diesel Alvarez-Galvan, M.; Campos-Martin, Jose; Fierro, Jose Catalysts, Vol. 9, Issue 3 https://doi.org/10.3390/catal9030293	journal	March 2019
Catalyst Performance in the HDPE Pyrolysis-Reforming under Reaction-Regeneration Cycles Barbarias, Itsaso; Artetxe, Maite; Lopez, Gartzen Catalysts, Vol. 9, Issue 5 https://doi.org/10.3390/catal9050414	journal	May 2019
Biomass Energy Technological Paradigm (BETP): Trends in This Sector Li, Meihui; Luo, Na; Lu, Yi Sustainability, Vol. 9, Issue 4 https://doi.org/10.3390/su9040567	journal	April 2017
Recent research progress on bio-oil conversion into bio-fuels and raw chemicals: a review: Research progress on bio-oil conversion Valle, Beatriz; Remiro, Aingeru; García-Gómez, Naiara Journal of Chemical Technology & Biotechnology, Vol. 94, Issue 3 https://doi.org/10.1002/jctb.5758	journal	July 2018
Bright Side of Lignin Depolymerization: Toward New Platform Chemicals Sun, Zhuohua; Fridrich, Bálint; de Santi, Alessandra Chemical Reviews, Vol. 118, Issue 2 https://doi.org/10.1021/acs.chemrev.7b00588	journal	January 2018

Figures / Tables (7)

Table 1(p. 3)

Table 2(p. 4)

Table 3 : Part 1(p. 4)

Table 3 : Part 2(p. 5)

Figure 1(p. 7)

Table 4 : Part 1(p. 10)

Table 4 : Part 2(p. 11)

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Related Subjects

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
09 BIOMASS FUELS
biomass
biofuel
pyrolysis
bio-oil
catalyst
catalytic cracking
hydrodeoxygenation
coking
deactivation
regeneration