Carbon-Nanotube-Based Thermoelectric Materials and Devices
Abstract
Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.
- Authors:
-
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Texas A & M Univ., College Station, TX (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), NREL Laboratory Directed Research and Development (LDRD)
- OSTI Identifier:
- 1419418
- Alternate Identifier(s):
- OSTI ID: 1417708
- Report Number(s):
- NREL/JA-5900-70041
Journal ID: ISSN 0935-9648; TRN: US1801347
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; carbon nanotubes; composite materials; energy harvesting; organic electronics; thermoelectrics
Citation Formats
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States: N. p., 2018.
Web. doi:10.1002/adma.201704386.
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, & Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States. https://doi.org/10.1002/adma.201704386
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Mon .
"Carbon-Nanotube-Based Thermoelectric Materials and Devices". United States. https://doi.org/10.1002/adma.201704386. https://www.osti.gov/servlets/purl/1419418.
@article{osti_1419418,
title = {Carbon-Nanotube-Based Thermoelectric Materials and Devices},
author = {Blackburn, Jeffrey L. and Ferguson, Andrew J. and Cho, Chungyeon and Grunlan, Jaime C.},
abstractNote = {Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.},
doi = {10.1002/adma.201704386},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {2018},
month = {1}
}
Web of Science
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Thermoelectric Properties of PEDOT:PSS
journal, February 2019
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Enhanced Phonon‐Drag Thermopower of Ballistic Semiconducting Single‐Walled Carbon Nanotubes Near the Second Subband Edge
journal, February 2019
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Semiconducting Single-Walled Carbon Nanotubes or Very Rigid Conjugated Polymers: A Comparison
journal, November 2018
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Convenient but powerful method to dope single-walled carbon nanotube films with iodonium salts
journal, August 2019
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Thermally Enhanced n‐Type Thermoelectric Behavior in Completely Organic Graphene Oxide‐Based Thin Films
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- Advanced Electronic Materials, Vol. 5, Issue 11
A facile and efficient strategy for the functionalization of multiple-walled carbon nanotubes using well-defined polypropylene-grafted polystyrene
journal, July 2018
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Carbon nanotube fibers with enhanced longitudinal carrier mobility for high-performance all-carbon thermoelectric generators
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Conjugated Polymer Blends for Organic Thermoelectrics
journal, January 2019
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- Advanced Electronic Materials, Vol. 5, Issue 11
Balancing the electrical conductivity and Seebeck coefficient by controlled interfacial doping towards high performance benzothienobenzothiophene-based organic thermoelectric materials
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- Journal of Materials Chemistry A, Vol. 7, Issue 43
A convenient and highly tunable way to n-type carbon nanotube thermoelectric composite film using common alkylammonium cationic surfactant
journal, January 2018
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Multifunctional inorganic nanomaterials for energy applications
journal, January 2020
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Thermoelectric fibers from well-dispersed carbon nanotube/poly(vinyliedene fluoride) pastes for fiber-based thermoelectric generators
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Doping engineering of thermoelectric transport in BNC heteronanotubes
journal, January 2019
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Electromagnetic Response and Energy Conversion for Functions and Devices in Low‐Dimensional Materials
journal, April 2019
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Molecular Patching Engineering to Drive Energy Conversion as Efficient and Environment‐Friendly Cell toward Wireless Power Transmission
journal, January 2020
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A Novel Way to Enhance the Thermoelectric Efficiency of Carbon Nanotube through Cobaltocene‐decamethyl Cobaltocene Encapsulation
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Construction of cobaltous oxide/nickel–iron oxide electrodes with great cycle stability and high energy density for advanced asymmetry supercapacitor
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Annular flexible thermoelectric devices with integrated-module architecture
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Effect of nanotube coupling on exciton transport in polymer-free monochiral semiconducting carbon nanotube networks
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Anthanthrene-based conjugated polymers for the dispersion of single-walled carbon nanotubes
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Macroscopically aligned carbon nanotubes for flexible and high-temperature electronics, optoelectronics, and thermoelectrics
journal, December 2019
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Poly(3,4-Ethylenedioxythiophene) Nanoparticles as Building Blocks for Hybrid Thermoelectric Flexible Films
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Preparation and Thermoelectric Properties of Graphite/poly(3,4-ethyenedioxythiophene) Nanocomposites
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Impact of Synthesis Parameters of Multi-Walled Carbon Nanotubes on their Thermoelectric Properties
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Recent Progress in Flexible Organic Thermoelectrics
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Carbon Nanotube-Based Organic Thermoelectric Materials for Energy Harvesting
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Printable Semiconductors for Backplane TFTs of Flexible OLED Displays
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Flexible Thermoelectric Materials and Generators: Challenges and Innovations
journal, May 2019
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Shape Conformal and Thermal Insulative Organic Solar Absorber Sponge for Photothermal Water Evaporation and Thermoelectric Power Generation
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Solar Harvesting: a Unique Opportunity for Organic Thermoelectrics?
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Farming thermoelectric paper
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Interplay between synthetic conditions and micromorphology in poly(3,4-ethylenedioxythiophene):tosylate (PEDOT:Tos): an atomistic investigation
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A practical field guide to thermoelectrics: Fundamentals, synthesis, and characterization
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Polyvinyl alcohol covalently grafted CNT for free-standing, flexible, and high-performance thermoelectric generator film
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Effect of Nonionic Conjugated Matrix Polymer and P-Dopant on Carbon Nanotube Aggregation and Thermoelectric Properties
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Recent Progress in Thermoelectric Materials Based on Conjugated Polymers
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Thermoelectric properties of sorted semiconducting single-walled carbon nanotube sheets
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Donor-doped ZnO thin films on mica for fully-inorganic flexible thermoelectrics
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Organic Thermoelectric Multilayers with High Stretchiness
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Fiber‐Based Energy Conversion Devices for Human‐Body Energy Harvesting
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Freely Shapable and 3D Porous Carbon Nanotube Foam Using Rapid Solvent Evaporation Method for Flexible Thermoelectric Power Generators
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A tool box to ascertain the nature of doping and photoresponse in single-walled carbon nanotubes
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Will organic thermoelectrics get hot?
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