Carbon-Nanotube-Based Thermoelectric Materials and Devices
Abstract
Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.
- Authors:
-
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Texas A & M Univ., College Station, TX (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE Office of Energy Efficiency and Renewable Energy (EERE), NREL Laboratory Directed Research and Development (LDRD)
- OSTI Identifier:
- 1419418
- Alternate Identifier(s):
- OSTI ID: 1417708
- Report Number(s):
- NREL/JA-5900-70041
Journal ID: ISSN 0935-9648; TRN: US1801347
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; carbon nanotubes; composite materials; energy harvesting; organic electronics; thermoelectrics
Citation Formats
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States: N. p., 2018.
Web. doi:10.1002/adma.201704386.
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, & Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States. doi:10.1002/adma.201704386.
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Mon .
"Carbon-Nanotube-Based Thermoelectric Materials and Devices". United States. doi:10.1002/adma.201704386. https://www.osti.gov/servlets/purl/1419418.
@article{osti_1419418,
title = {Carbon-Nanotube-Based Thermoelectric Materials and Devices},
author = {Blackburn, Jeffrey L. and Ferguson, Andrew J. and Cho, Chungyeon and Grunlan, Jaime C.},
abstractNote = {Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.},
doi = {10.1002/adma.201704386},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {2018},
month = {1}
}
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