Carbon-Nanotube-Based Thermoelectric Materials and Devices
Abstract
Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.
- Authors:
-
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Texas A & M Univ., College Station, TX (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), NREL Laboratory Directed Research and Development (LDRD)
- OSTI Identifier:
- 1419418
- Alternate Identifier(s):
- OSTI ID: 1417708
- Report Number(s):
- NREL/JA-5900-70041
Journal ID: ISSN 0935-9648; TRN: US1801347
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; carbon nanotubes; composite materials; energy harvesting; organic electronics; thermoelectrics
Citation Formats
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States: N. p., 2018.
Web. doi:10.1002/adma.201704386.
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, & Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States. https://doi.org/10.1002/adma.201704386
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Mon .
"Carbon-Nanotube-Based Thermoelectric Materials and Devices". United States. https://doi.org/10.1002/adma.201704386. https://www.osti.gov/servlets/purl/1419418.
@article{osti_1419418,
title = {Carbon-Nanotube-Based Thermoelectric Materials and Devices},
author = {Blackburn, Jeffrey L. and Ferguson, Andrew J. and Cho, Chungyeon and Grunlan, Jaime C.},
abstractNote = {Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity-generation sectors, and manufacturing processes. Thermal energy is also an abundant low-flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off-grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric-energy-harvesting devices. Carbon-based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source-materials, their amenability to high-throughput solution-phase fabrication routes, and the high specific energy (i.e., W g-1) enabled by their low mass. Single-walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric-energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube-based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon-nanotube-based materials and composites have for producing high-performance next-generation devices for thermoelectric-energy harvesting.},
doi = {10.1002/adma.201704386},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {2018},
month = {1}
}
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- Han, Weifang; Song, Wei; Shen, Yuxiang
- Journal of Materials Science, Vol. 54, Issue 8
Clinical Applications of Carbon Nanomaterials in Diagnostics and Therapy
journal, August 2018
- Loh, Kian Ping; Ho, Dean; Chiu, Gigi Ngar Chee
- Advanced Materials, Vol. 30, Issue 47
Thermoelectric Properties of PEDOT:PSS
journal, February 2019
- Fan, Zeng; Ouyang, Jianyong
- Advanced Electronic Materials, Vol. 5, Issue 11
Enhanced Phonon‐Drag Thermopower of Ballistic Semiconducting Single‐Walled Carbon Nanotubes Near the Second Subband Edge
journal, February 2019
- Tsaousidou, Margarita
- physica status solidi (b), Vol. 256, Issue 6
Semiconducting Single-Walled Carbon Nanotubes or Very Rigid Conjugated Polymers: A Comparison
journal, November 2018
- Zaumseil, Jana
- Advanced Electronic Materials, Vol. 5, Issue 2
Convenient but powerful method to dope single-walled carbon nanotube films with iodonium salts
journal, August 2019
- Kumanek, B.; Przypis, Ł.; Wróbel, P. S.
- Applied Nanoscience, Vol. 10, Issue 2
Thermally Enhanced n‐Type Thermoelectric Behavior in Completely Organic Graphene Oxide‐Based Thin Films
journal, October 2018
- Cho, Chungyeon; Bittner, Noah; Choi, Woongchul
- Advanced Electronic Materials, Vol. 5, Issue 11
A facile and efficient strategy for the functionalization of multiple-walled carbon nanotubes using well-defined polypropylene-grafted polystyrene
journal, July 2018
- Abbasian, Mojtaba; Ghaeminia, Haleh; Jaymand, Mehdi
- Applied Physics A, Vol. 124, Issue 8
Carbon nanotube fibers with enhanced longitudinal carrier mobility for high-performance all-carbon thermoelectric generators
journal, January 2019
- Lee, Taemin; Park, Kyung Tae; Ku, Bon-Cheol
- Nanoscale, Vol. 11, Issue 36
Conjugated Polymer Blends for Organic Thermoelectrics
journal, January 2019
- Zuo, Guangzheng; Abdalla, Hassan; Kemerink, Martijn
- Advanced Electronic Materials, Vol. 5, Issue 11
Balancing the electrical conductivity and Seebeck coefficient by controlled interfacial doping towards high performance benzothienobenzothiophene-based organic thermoelectric materials
journal, January 2019
- Tan, Jingjuan; Chen, Zhanhua; Wang, Dagang
- Journal of Materials Chemistry A, Vol. 7, Issue 43
A convenient and highly tunable way to n-type carbon nanotube thermoelectric composite film using common alkylammonium cationic surfactant
journal, January 2018
- Cheng, Xuejiang; Wang, Xin; Chen, Guangming
- Journal of Materials Chemistry A, Vol. 6, Issue 39
Multifunctional inorganic nanomaterials for energy applications
journal, January 2020
- Wang, Huilin; Liang, Xitong; Wang, Jiutian
- Nanoscale, Vol. 12, Issue 1
Thermoelectric fibers from well-dispersed carbon nanotube/poly(vinyliedene fluoride) pastes for fiber-based thermoelectric generators
journal, January 2018
- Kim, Jae-Yeop; Mo, Jun-Hyun; Kang, Young Hun
- Nanoscale, Vol. 10, Issue 42
Doping engineering of thermoelectric transport in BNC heteronanotubes
journal, January 2019
- Medrano Sandonas, Leonardo; Cuba-Supanta, Gustavo; Gutierrez, Rafael
- Physical Chemistry Chemical Physics, Vol. 21, Issue 4
Electromagnetic Response and Energy Conversion for Functions and Devices in Low‐Dimensional Materials
journal, April 2019
- Cao, Mao‐Sheng; Wang, Xi‐Xi; Zhang, Min
- Advanced Functional Materials, Vol. 29, Issue 25
Molecular Patching Engineering to Drive Energy Conversion as Efficient and Environment‐Friendly Cell toward Wireless Power Transmission
journal, January 2020
- Shu, Jin‐Cheng; Cao, Mao‐Sheng; Zhang, Min
- Advanced Functional Materials, Vol. 30, Issue 10
A Novel Way to Enhance the Thermoelectric Efficiency of Carbon Nanotube through Cobaltocene‐decamethyl Cobaltocene Encapsulation
journal, January 2020
- Koley, Sayantanu; Sen, Sabyasachi; Chakrabarti, Swapan
- ChemistrySelect, Vol. 5, Issue 4
Construction of cobaltous oxide/nickel–iron oxide electrodes with great cycle stability and high energy density for advanced asymmetry supercapacitor
journal, November 2019
- Zhao, Yan; Chen, Yuan; Liu, Qingqing
- Journal of Materials Science: Materials in Electronics, Vol. 30, Issue 24
Annular flexible thermoelectric devices with integrated-module architecture
journal, January 2020
- Qu, Dawei; Huang, Xuan; Li, Xin
- npj Flexible Electronics, Vol. 4, Issue 1
Effect of nanotube coupling on exciton transport in polymer-free monochiral semiconducting carbon nanotube networks
journal, January 2019
- Arias, Dylan H.; Sulas-Kern, Dana B.; Hart, Stephanie M.
- Nanoscale, Vol. 11, Issue 44
Anthanthrene-based conjugated polymers for the dispersion of single-walled carbon nanotubes
journal, January 2019
- Aumaitre, Cyril; Fong, Darryl; Adronov, Alex
- Polymer Chemistry, Vol. 10, Issue 47
Macroscopically aligned carbon nanotubes for flexible and high-temperature electronics, optoelectronics, and thermoelectrics
journal, December 2019
- Gao, Weilu; Komatsu, Natsumi; Taylor, Lauren W.
- Journal of Physics D: Applied Physics, Vol. 53, Issue 6
Poly(3,4-Ethylenedioxythiophene) Nanoparticles as Building Blocks for Hybrid Thermoelectric Flexible Films
journal, December 2019
- Serrano-Claumarchirant, Jose F.; Culebras, Mario; Cantarero, Andrés
- Coatings, Vol. 10, Issue 1
Preparation and Thermoelectric Properties of Graphite/poly(3,4-ethyenedioxythiophene) Nanocomposites
journal, October 2018
- Du, Yong; Li, Haixia; Jia, Xuechen
- Energies, Vol. 11, Issue 10
Impact of Synthesis Parameters of Multi-Walled Carbon Nanotubes on their Thermoelectric Properties
journal, October 2019
- Kumanek, Bogumiła; Stando, Grzegorz; Wróbel, Paweł S.
- Materials, Vol. 12, Issue 21
Recent Progress in Flexible Organic Thermoelectrics
journal, November 2018
- Culebras, Mario; Choi, Kyungwho; Cho, Chungyeon
- Micromachines, Vol. 9, Issue 12
Carbon Nanotube-Based Organic Thermoelectric Materials for Energy Harvesting
journal, October 2018
- Wang, Xiaodong; Wang, Hong; Liu, Bing
- Polymers, Vol. 10, Issue 11
Printable Semiconductors for Backplane TFTs of Flexible OLED Displays
journal, August 2019
- Zhu, Huihui; Shin, Eun‐Sol; Liu, Ao
- Advanced Functional Materials, Vol. 30, Issue 20
Flexible Thermoelectric Materials and Generators: Challenges and Innovations
journal, May 2019
- Wang, Yuan; Yang, Lei; Shi, Xiao‐Lei
- Advanced Materials, Vol. 31, Issue 29
Shape Conformal and Thermal Insulative Organic Solar Absorber Sponge for Photothermal Water Evaporation and Thermoelectric Power Generation
journal, April 2019
- Zhu, Liangliang; Ding, Tianpeng; Gao, Minmin
- Advanced Energy Materials, Vol. 9, Issue 22
Solar Harvesting: a Unique Opportunity for Organic Thermoelectrics?
journal, October 2019
- Jurado, José P.; Dörling, Bernhard; Zapata‐Arteaga, Osnat
- Advanced Energy Materials, Vol. 9, Issue 45
Farming thermoelectric paper
journal, January 2019
- Abol-Fotouh, Deyaa; Dörling, Bernhard; Zapata-Arteaga, Osnat
- Energy & Environmental Science, Vol. 12, Issue 2
Interplay between synthetic conditions and micromorphology in poly(3,4-ethylenedioxythiophene):tosylate (PEDOT:Tos): an atomistic investigation
journal, January 2019
- Cappai, A.; Antidormi, A.; Bosin, A.
- Physical Chemistry Chemical Physics, Vol. 21, Issue 16
A practical field guide to thermoelectrics: Fundamentals, synthesis, and characterization
journal, June 2018
- Zevalkink, Alex; Smiadak, David M.; Blackburn, Jeff L.
- Applied Physics Reviews, Vol. 5, Issue 2
Polyvinyl alcohol covalently grafted CNT for free-standing, flexible, and high-performance thermoelectric generator film
journal, February 2019
- Ha, Jae Un; Cho, Jangwhan; Yoon, Seongwon
- Nanotechnology, Vol. 30, Issue 14
Effect of Nonionic Conjugated Matrix Polymer and P-Dopant on Carbon Nanotube Aggregation and Thermoelectric Properties
journal, September 2018
- Li, Hui; Huang, Jiyuan; Sato, Toshiyuki
- MRS Advances, Vol. 3, Issue 60
Recent Progress in Thermoelectric Materials Based on Conjugated Polymers
journal, January 2019
- Yao, Chang-Jiang; Zhang, Hao-Li; Zhang, Qichun
- Polymers, Vol. 11, Issue 1
Thermoelectric properties of sorted semiconducting single-walled carbon nanotube sheets
text, January 2019
- Huang, Wenxin; Tokunaga, Eriko; Nakashima, Yuki
- Taylor & Francis
Donor-doped ZnO thin films on mica for fully-inorganic flexible thermoelectrics
journal, March 2019
- Paul, Biplab; Khranovskyy, Volodymyr; Yakimova, Rositsa
- Materials Research Letters, Vol. 7, Issue 6
Organic Thermoelectric Multilayers with High Stretchiness
journal, December 2019
- Cho, Chungyeon; Son, Jihun
- Nanomaterials, Vol. 10, Issue 1
Fiber‐Based Energy Conversion Devices for Human‐Body Energy Harvesting
journal, June 2019
- Huang, Liang; Lin, Shizhe; Xu, Zisheng
- Advanced Materials, Vol. 32, Issue 5
Freely Shapable and 3D Porous Carbon Nanotube Foam Using Rapid Solvent Evaporation Method for Flexible Thermoelectric Power Generators
journal, June 2019
- Lee, Min‐Hye; Kang, Young Hun; Kim, Jungwon
- Advanced Energy Materials, Vol. 9, Issue 29
A tool box to ascertain the nature of doping and photoresponse in single-walled carbon nanotubes
journal, January 2019
- Santidrián, Ana; González-Domínguez, José M.; Diez-Cabanes, Valentin
- Physical Chemistry Chemical Physics, Vol. 21, Issue 7
Will organic thermoelectrics get hot?
journal, July 2019
- Campoy-Quiles, Mariano
- Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2152