Carbon-Nanotube-Based Thermoelectric Materials and Devices
Abstract
Abstract Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity‐generation sectors, and manufacturing processes. Thermal energy is also an abundant low‐flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off‐grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric‐energy‐harvesting devices. Carbon‐based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source‐materials, their amenability to high‐throughput solution‐phase fabrication routes, and the high specific energy (i.e., W g −1 ) enabled by their low mass. Single‐walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric‐energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube‐based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon‐nanotube‐based materials and composites have for producing high‐performance next‐generation devices for thermoelectric‐energy harvesting.
- Authors:
-
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Texas A & M Univ., College Station, TX (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), NREL Laboratory Directed Research and Development (LDRD)
- OSTI Identifier:
- 1419418
- Alternate Identifier(s):
- OSTI ID: 1417708
- Report Number(s):
- NREL/JA-5900-70041
Journal ID: ISSN 0935-9648; TRN: US1801347
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 11; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; carbon nanotubes; composite materials; energy harvesting; organic electronics; thermoelectrics
Citation Formats
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States: N. p., 2018.
Web. doi:10.1002/adma.201704386.
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, & Grunlan, Jaime C. Carbon-Nanotube-Based Thermoelectric Materials and Devices. United States. https://doi.org/10.1002/adma.201704386
Blackburn, Jeffrey L., Ferguson, Andrew J., Cho, Chungyeon, and Grunlan, Jaime C. Mon .
"Carbon-Nanotube-Based Thermoelectric Materials and Devices". United States. https://doi.org/10.1002/adma.201704386. https://www.osti.gov/servlets/purl/1419418.
@article{osti_1419418,
title = {Carbon-Nanotube-Based Thermoelectric Materials and Devices},
author = {Blackburn, Jeffrey L. and Ferguson, Andrew J. and Cho, Chungyeon and Grunlan, Jaime C.},
abstractNote = {Abstract Conversion of waste heat to voltage has the potential to significantly reduce the carbon footprint of a number of critical energy sectors, such as the transportation and electricity‐generation sectors, and manufacturing processes. Thermal energy is also an abundant low‐flux source that can be harnessed to power portable/wearable electronic devices and critical components in remote off‐grid locations. As such, a number of different inorganic and organic materials are being explored for their potential in thermoelectric‐energy‐harvesting devices. Carbon‐based thermoelectric materials are particularly attractive due to their use of nontoxic, abundant source‐materials, their amenability to high‐throughput solution‐phase fabrication routes, and the high specific energy (i.e., W g −1 ) enabled by their low mass. Single‐walled carbon nanotubes (SWCNTs) represent a unique 1D carbon allotrope with structural, electrical, and thermal properties that enable efficient thermoelectric‐energy conversion. Here, the progress made toward understanding the fundamental thermoelectric properties of SWCNTs, nanotube‐based composites, and thermoelectric devices prepared from these materials is reviewed in detail. This progress illuminates the tremendous potential that carbon‐nanotube‐based materials and composites have for producing high‐performance next‐generation devices for thermoelectric‐energy harvesting.},
doi = {10.1002/adma.201704386},
journal = {Advanced Materials},
number = 11,
volume = 30,
place = {United States},
year = {Mon Jan 22 00:00:00 EST 2018},
month = {Mon Jan 22 00:00:00 EST 2018}
}
Web of Science
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Enhanced Phonon‐Drag Thermopower of Ballistic Semiconducting Single‐Walled Carbon Nanotubes Near the Second Subband Edge
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Semiconducting Single-Walled Carbon Nanotubes or Very Rigid Conjugated Polymers: A Comparison
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Convenient but powerful method to dope single-walled carbon nanotube films with iodonium salts
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Thermally Enhanced n‐Type Thermoelectric Behavior in Completely Organic Graphene Oxide‐Based Thin Films
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A facile and efficient strategy for the functionalization of multiple-walled carbon nanotubes using well-defined polypropylene-grafted polystyrene
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Carbon nanotube fibers with enhanced longitudinal carrier mobility for high-performance all-carbon thermoelectric generators
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Conjugated Polymer Blends for Organic Thermoelectrics
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A convenient and highly tunable way to n-type carbon nanotube thermoelectric composite film using common alkylammonium cationic surfactant
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Thermoelectric fibers from well-dispersed carbon nanotube/poly(vinyliedene fluoride) pastes for fiber-based thermoelectric generators
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Doping engineering of thermoelectric transport in BNC heteronanotubes
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Electromagnetic Response and Energy Conversion for Functions and Devices in Low‐Dimensional Materials
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Molecular Patching Engineering to Drive Energy Conversion as Efficient and Environment‐Friendly Cell toward Wireless Power Transmission
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A Novel Way to Enhance the Thermoelectric Efficiency of Carbon Nanotube through Cobaltocene‐decamethyl Cobaltocene Encapsulation
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Construction of cobaltous oxide/nickel–iron oxide electrodes with great cycle stability and high energy density for advanced asymmetry supercapacitor
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Annular flexible thermoelectric devices with integrated-module architecture
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Macroscopically aligned carbon nanotubes for flexible and high-temperature electronics, optoelectronics, and thermoelectrics
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Poly(3,4-Ethylenedioxythiophene) Nanoparticles as Building Blocks for Hybrid Thermoelectric Flexible Films
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Preparation and Thermoelectric Properties of Graphite/poly(3,4-ethyenedioxythiophene) Nanocomposites
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Impact of Synthesis Parameters of Multi-Walled Carbon Nanotubes on their Thermoelectric Properties
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Recent Progress in Flexible Organic Thermoelectrics
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Carbon Nanotube-Based Organic Thermoelectric Materials for Energy Harvesting
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Printable Semiconductors for Backplane TFTs of Flexible OLED Displays
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Flexible Thermoelectric Materials and Generators: Challenges and Innovations
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Shape Conformal and Thermal Insulative Organic Solar Absorber Sponge for Photothermal Water Evaporation and Thermoelectric Power Generation
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Solar Harvesting: a Unique Opportunity for Organic Thermoelectrics?
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Interplay between synthetic conditions and micromorphology in poly(3,4-ethylenedioxythiophene):tosylate (PEDOT:Tos): an atomistic investigation
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A practical field guide to thermoelectrics: Fundamentals, synthesis, and characterization
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Polyvinyl alcohol covalently grafted CNT for free-standing, flexible, and high-performance thermoelectric generator film
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Effect of Nonionic Conjugated Matrix Polymer and P-Dopant on Carbon Nanotube Aggregation and Thermoelectric Properties
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Recent Progress in Thermoelectric Materials Based on Conjugated Polymers
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Thermoelectric properties of sorted semiconducting single-walled carbon nanotube sheets
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Organic Thermoelectric Multilayers with High Stretchiness
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Fiber‐Based Energy Conversion Devices for Human‐Body Energy Harvesting
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Freely Shapable and 3D Porous Carbon Nanotube Foam Using Rapid Solvent Evaporation Method for Flexible Thermoelectric Power Generators
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A tool box to ascertain the nature of doping and photoresponse in single-walled carbon nanotubes
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Will organic thermoelectrics get hot?
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Thermal conductivity of carbon nanotube networks: a review
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Effect of Functional Groups on the Thermoelectric Performance of Carbon Nanotubes
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Breaking the Nanoparticle Loading–Dispersion Dichotomy in Polymer Nanocomposites with the Art of Croissant-Making
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Will organic thermoelectrics get hot?
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Manipulation of p-/n-Type Thermoelectric Thin Films through a Layer-by-Layer Assembled Carbonaceous Multilayer Structure
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Carbon Nanotube-Based Organic Thermoelectric Materials for Energy Harvesting
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Recent Progress in Thermoelectric Materials Based on Conjugated Polymers
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