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Title: Mechanical properties of nanoporous gold in tension

Abstract

We report results of the tensile properties of nanoporous gold (NPG) as a function of the density and average ligament diameter. As-dealloyed tensile samples were thermally treated to coarsen the length scale of the NPG structure while increasing the sample density resulting from thickness reductions. The behaviors of samples with mean ligament diameters ranging from 30 to 750 nm and corresponding densities ranging from 0.30 to 0.57 that of bulk gold were examined. Digital image analysis was used to obtain ligament size histograms that were fit to the Weibull distribution. The Young's modulus was found to obey a power law, but with an exponent larger than that predicted by Gibson-Ashby scaling. The fracture behavior showed a brittle-ductile transition as a function of increasing ligament size. For samples characterized by a mean ligament diameter less than ~ 220 nm, the tensile behavior was linear elastic to sample fracture while samples with larger scale ligaments showed macroscopic yielding prior to fracture. These results are interpreted within the framework of extreme value statistics.

Authors:
 [1];  [1];  [1]
  1. Arizona State Univ., Tempe, AZ (United States). Ira A. Fulton School of Engineering
Publication Date:
Research Org.:
Arizona State Univ., Tempe, AZ (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1533469
Alternate Identifier(s):
OSTI ID: 1419114
Grant/Contract Number:  
SC0008677
Resource Type:
Accepted Manuscript
Journal Name:
Acta Materialia
Additional Journal Information:
Journal Volume: 129; Journal ID: ISSN 1359-6454
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; nanoporous gold; mechanical properties; digital image analysis; brittle-to-ductile transition; extreme value statistics

Citation Formats

Badwe, Nilesh, Chen, Xiying, and Sieradzki, Karl. Mechanical properties of nanoporous gold in tension. United States: N. p., 2017. Web. doi:10.1016/j.actamat.2017.02.040.
Badwe, Nilesh, Chen, Xiying, & Sieradzki, Karl. Mechanical properties of nanoporous gold in tension. United States. https://doi.org/10.1016/j.actamat.2017.02.040
Badwe, Nilesh, Chen, Xiying, and Sieradzki, Karl. Thu . "Mechanical properties of nanoporous gold in tension". United States. https://doi.org/10.1016/j.actamat.2017.02.040. https://www.osti.gov/servlets/purl/1533469.
@article{osti_1533469,
title = {Mechanical properties of nanoporous gold in tension},
author = {Badwe, Nilesh and Chen, Xiying and Sieradzki, Karl},
abstractNote = {We report results of the tensile properties of nanoporous gold (NPG) as a function of the density and average ligament diameter. As-dealloyed tensile samples were thermally treated to coarsen the length scale of the NPG structure while increasing the sample density resulting from thickness reductions. The behaviors of samples with mean ligament diameters ranging from 30 to 750 nm and corresponding densities ranging from 0.30 to 0.57 that of bulk gold were examined. Digital image analysis was used to obtain ligament size histograms that were fit to the Weibull distribution. The Young's modulus was found to obey a power law, but with an exponent larger than that predicted by Gibson-Ashby scaling. The fracture behavior showed a brittle-ductile transition as a function of increasing ligament size. For samples characterized by a mean ligament diameter less than ~ 220 nm, the tensile behavior was linear elastic to sample fracture while samples with larger scale ligaments showed macroscopic yielding prior to fracture. These results are interpreted within the framework of extreme value statistics.},
doi = {10.1016/j.actamat.2017.02.040},
journal = {Acta Materialia},
number = ,
volume = 129,
place = {United States},
year = {Thu Feb 16 00:00:00 EST 2017},
month = {Thu Feb 16 00:00:00 EST 2017}
}

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