Multidimensional photon correlation spectroscopy of cavity polaritons

Dorfman, Konstantin E.; Mukamel, Shaul

doi:10.1073/pnas.1719443115

Title: Multidimensional photon correlation spectroscopy of cavity polaritons

Journal Article · 31 January 2018 · Proceedings of the National Academy of Sciences of the United States of America

DOI: https://doi.org/10.1073/pnas.1719443115 · OSTI ID:1418899

Dorfman, Konstantin E. ^[1];

^[2]

East China Normal Univ. (ECNU), Shanghai (China)
Univ. of California, Irvine, CA (United States)

The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We introduce a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are indicated by solving the Jaynes–Cummings model.

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Research Organization:: Univ. of California, Irvine, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division; National Science Foundation (NSF)

Grant/Contract Number:: FG02-04ER15571; CHE-1663822

OSTI ID:: 1418899

Alternate ID(s):: OSTI ID: 1527163

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Vol. 115, Issue 7; ISSN 0027-8424

Publisher:: National Academy of SciencesCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 22 works

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