In Situ TEM Multi-Beam Ion Irradiation as a Technique for Elucidating Synergistic Radiation Effects

Taylor, Caitlin Anne; Bufford, Daniel Charles; Muntifering, Brittany Rana; Senor, David; Steckbeck, Mackenzie; Davis, Justin; Doyle, Barney; Buller, Daniel; Hattar, Khalid

doi:10.3390/MA10101148

Title: In Situ TEM Multi-Beam Ion Irradiation as a Technique for Elucidating Synergistic Radiation Effects

Journal Article · 29 September 2017 · Materials

DOI: https://doi.org/10.3390/MA10101148 · OSTI ID:1418331

Taylor, Caitlin Anne ^[1]; Bufford, Daniel Charles ^[1]; Muntifering, Brittany Rana ^[1]; Senor, David ^[2]; Steckbeck, Mackenzie ^[1]; Davis, Justin ^[1]; Doyle, Barney ^[1]; Buller, Daniel ^[1];

^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

Materials designed for nuclear reactors undergo microstructural changes resulting from a combination of several environmental factors, including neutron irradiation damage, gas accumulation and elevated temperatures. Typical ion beam irradiation experiments designed for simulating a neutron irradiation environment involve irradiating the sample with a single ion beam and subsequent characterization of the resulting microstructure, often by transmission electron microscopy (TEM). This method does not allow for examination of microstructural effects due to simultaneous gas accumulation and displacement cascade damage, which occurs in a reactor. Sandia’s in situ ion irradiation TEM (I³TEM) offers the unique ability to observe microstructural changes due to irradiation damage caused by concurrent multi-beam ion irradiation in real time. This allows for time-dependent microstructure analysis. A plethora of additional in situ stages can be coupled with these experiments, e.g., for more accurately simulating defect kinetics at elevated reactor temperatures. As a result, this work outlines experiments showing synergistic effects in Au using in situ ion irradiation with various combinations of helium, deuterium and Au ions, as well as some initial work on materials utilized in tritium-producing burnable absorber rods (TPBARs): zirconium alloys and LiAlO₂.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC05-76RL01830; AC04-94AL85000

OSTI ID:: 1418331

Alternate ID(s):: OSTI ID: 1406365

Report Number(s):: PNNL-SA-131591; SAND-2017-11074J; MATEG9; PII: ma10101148; TRN: US1801270

Journal Information:: Materials, Vol. 10, Issue 10; ISSN 1996-1944

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 9 works

Citation information provided by
Web of Science

References (27)

Heavy ion cratering of gold Donnelly, S. E.; Birtcher, R. C. Physical Review B, Vol. 56, Issue 21 https://doi.org/10.1103/PhysRevB.56.13599	journal	December 1997
Materials challenges in nuclear energy Zinkle, S. J.; Was, G. S. Acta Materialia, Vol. 61, Issue 3 https://doi.org/10.1016/j.actamat.2012.11.004	journal	February 2013
A review of in situ observation of defect production with energetic heavy ions Ishino, Shiori Journal of Nuclear Materials, Vol. 251 https://doi.org/10.1016/S0022-3115(97)00247-X	journal	November 1997
Direct observation of radiation damage produced in copper, gold and aluminum during ion bombardments at low temperatures in the electron microscope Howe, L. M.; McGurn, J. F.; Gilbert, R. W. Acta Metallurgica, Vol. 14, Issue 7 https://doi.org/10.1016/0001-6160(66)90001-0	journal	July 1966
Ion irradiation and radiation effect characterization at the JANNUS-Saclay triple beam facility Beck, Lucile; Serruys, Yves; Miro, Sandrine Journal of Materials Research, Vol. 30, Issue 9 https://doi.org/10.1557/jmr.2014.414	journal	February 2015
Concurrent in situ ion irradiation transmission electron microscope Hattar, K.; Bufford, D. C.; Buller, D. L. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338 https://doi.org/10.1016/j.nimb.2014.08.002	journal	November 2014
Synergistic effect of helium and hydrogen for defect evolution under multi-ion irradiation of Fe–Cr ferritic alloys Tanaka, T.; Oka, K.; Ohnuki, S. Journal of Nuclear Materials, Vol. 329-333 https://doi.org/10.1016/j.jnucmat.2004.04.051	journal	August 2004
Migration behavior of helium under displacive irradiation in stainless steel, nickel, iron and zirconium Lewis, M. B.; Farrell, K. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 16, Issue 2-3 https://doi.org/10.1016/0168-583X(86)90008-X	journal	June 1986
A heavy-ion accelerator-electron microscope link for the direct observation of ion irradiation effects Whitmell, D. S.; Kennedy, W. A. D.; Mazey, D. J. Radiation Effects, Vol. 22, Issue 3 https://doi.org/10.1080/10420157408230774	journal	January 1974
In Situ TEM Concurrent and Successive Au Self-Ion Irradiation and He Implantation Chisholm, Claire; Hattar, Khalid; Minor, Andrew M. MATERIALS TRANSACTIONS, Vol. 55, Issue 3 https://doi.org/10.2320/matertrans.MD201316	journal	January 2014
Nucleation and growth theory of cavity evolution under conditions of cascade damage and high helium generation Ghoniem, N. M. Journal of Nuclear Materials, Vol. 174, Issue 2-3 https://doi.org/10.1016/0022-3115(90)90231-B	journal	November 1990
In situ Transmission Electron Microscopy Investigation of Radiation Effects Birtcher, R. C.; Kirk, M. A.; Furuya, K. Journal of Materials Research, Vol. 20, Issue 7 https://doi.org/10.1557/JMR.2005.0242	journal	July 2005
In situ transmission electron microscopy and ion irradiation of ferritic materials Kirk, Marquis A.; Baldo, Peter M.; Liu, Amelia C. Y. Microscopy Research and Technique, Vol. 72, Issue 3 https://doi.org/10.1002/jemt.20670	journal	March 2009
Irradiation Facilities of the Takasaki Advanced Radiation Research Institute Kurashima, Satoshi; Satoh, Takahiro; Saitoh, Yuichi Quantum Beam Science, Vol. 1, Issue 1 https://doi.org/10.3390/qubs1010002	journal	March 2017
Ion damage to metal films inside an electron microscope Pashley, D. W.; Presland, A. E. B. Philosophical Magazine, Vol. 6, Issue 68 https://doi.org/10.1080/14786436108243360	journal	August 1961
A review of transmission electron microscopes with in situ ion irradiation Hinks, J. A. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 267, Issue 23-24 https://doi.org/10.1016/j.nimb.2009.09.014	journal	December 2009
In situ experiments in the transmission electron microscope Butler, E. P. Reports on Progress in Physics, Vol. 42, Issue 5 https://doi.org/10.1088/0034-4885/42/5/002	journal	May 1979
In situ transmission electron microscopy and ion irradiation of ferritic materials Kirk, Marquis A.; Baldo, Peter M.; Liu, Amelia C. Y. Microscopy Research and Technique, Vol. 72, Issue 3 https://doi.org/10.1002/jemt.20670	journal	March 2009
Direct observation of radiation damage produced in copper, gold and aluminum during ion bombardments at low temperatures in the electron microscope Howe, L. M.; McGurn, J. F.; Gilbert, R. W. Acta Metallurgica, Vol. 14, Issue 7 https://doi.org/10.1016/0001-6160(66)90001-0	journal	July 1966
Concurrent in situ ion irradiation transmission electron microscope Hattar, K.; Bufford, D. C.; Buller, D. L. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338 https://doi.org/10.1016/j.nimb.2014.08.002	journal	November 2014
New evaluation of displacement damage and gas production for breeder ceramics under IFMIF, fusion and fission neutron irradiation Lizunov, Yu; Möslang, A.; Ryazanov, A. Journal of Nuclear Materials, Vol. 307-311 https://doi.org/10.1016/s0022-3115(02)01275-8	journal	December 2002
A heavy-ion accelerator-electron microscope link for the direct observation of ion irradiation effects Whitmell, D. S.; Kennedy, W. A. D.; Mazey, D. J. Radiation Effects, Vol. 22, Issue 3 https://doi.org/10.1080/10420157408230774	journal	January 1974
In situ experiments in the transmission electron microscope Butler, E. P. Reports on Progress in Physics, Vol. 42, Issue 5 https://doi.org/10.1088/0034-4885/42/5/002	journal	May 1979
Response of helium bubbles in gold to displacement-cascade damage Donnelly, S. E.; Birtcher, R. C.; Templier, C. Physical Review B, Vol. 52, Issue 6 https://doi.org/10.1103/physrevb.52.3970	journal	August 1995
Nanoparticle Ejection from Au Induced by Single Xe Ion Impacts Birtcher, Robert C.; Donnelly, S. E.; Schlutig, S. Physical Review Letters, Vol. 85, Issue 23 https://doi.org/10.1103/physrevlett.85.4968	journal	December 2000
Ion irradiation and radiation effect characterization at the JANNUS-Saclay triple beam facility Beck, Lucile; Serruys, Yves; Miro, Sandrine Journal of Materials Research, Vol. 30, Issue 9 https://doi.org/10.1557/jmr.2014.414	journal	February 2015
Irradiation Facilities of the Takasaki Advanced Radiation Research Institute Kurashima, Satoshi; Satoh, Takahiro; Saitoh, Yuichi Quantum Beam Science, Vol. 1, Issue 1 https://doi.org/10.3390/qubs1010002	journal	March 2017

Cited By (2)

Application of In Situ TEM to Investigate Irradiation Creep in Nanocrystalline Zirconium Bufford, Daniel C.; Barr, Christopher M.; Wang, Baoming JOM, Vol. 71, Issue 10 https://doi.org/10.1007/s11837-019-03701-7	journal	August 2019
A study of irradiation effects in TiO ₂ using molecular dynamics simulation and complementary in situ transmission electron microscopy Cowen, Benjamin J.; El-Genk, Mohamed S.; Hattar, Khalid Journal of Applied Physics, Vol. 124, Issue 9 https://doi.org/10.1063/1.5045491	journal	September 2018