DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Investigation of the short argon arc with hot anode. I. Numerical simulations of non-equilibrium effects in the near-electrode regions

Abstract

The atmospheric pressure arcs have recently found application in the production of nanoparticles. The distinguishing features of such arcs are small length and hot ablating anode characterized by intensive electron emission and radiation from its surface. We performed a one-dimensional modeling of argon arc, which shows that near-electrode effects of thermal and ionization non-equilibrium play an important role in the operation of a short arc, because the non-equilibrium regions are up to several millimeters long and are comparable to the arc length. The near-anode region is typically longer than the near-cathode region and its length depends more strongly on the current density. The model was extensively verified and validated against previous simulation results and experimental data. The Volt-Ampere characteristic (VAC) of the near-anode region depends on the anode cooling mechanism. The anode voltage is negative. In the case of strong anode cooling (water-cooled anode) when the anode is cold, temperature and plasma density gradients increase with current density, resulting in a decrease of the anode voltage (the absolute value increases). Falling VAC of the near-anode region suggests the arc constriction near the anode. Without anode cooling, the anode temperature increases significantly with the current density, leading to a drastic increasemore » in the thermionic emission current from the anode. Correspondingly, the anode voltage increases to suppress the emission, and the opposite trend in the VAC is observed. The results of simulations were found to be independent of sheath model used: collisional (fluid) or collisionless model gave the same plasma profiles for both near-anode and near-cathode regions.« less

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2];  [1]
  1. Princeton Plasma Physics Lab. (PPPL), Princeton, NJ (United States)
  2. Keiser Univ., Fort Lauderdale, FL (United States)
Publication Date:
Research Org.:
Princeton Plasma Physics Laboratory (PPPL), Princeton, NJ (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Fusion Energy Sciences (FES)
OSTI Identifier:
1419791
Alternate Identifier(s):
OSTI ID: 1417712
Grant/Contract Number:  
AC02-09CH11466
Resource Type:
Accepted Manuscript
Journal Name:
Physics of Plasmas
Additional Journal Information:
Journal Volume: 25; Journal Issue: 1; Journal ID: ISSN 1070-664X
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY

Citation Formats

Khrabry, A., Kaganovich, I. D., Nemchinsky, V., and Khodak, A. Investigation of the short argon arc with hot anode. I. Numerical simulations of non-equilibrium effects in the near-electrode regions. United States: N. p., 2018. Web. doi:10.1063/1.5007082.
Khrabry, A., Kaganovich, I. D., Nemchinsky, V., & Khodak, A. Investigation of the short argon arc with hot anode. I. Numerical simulations of non-equilibrium effects in the near-electrode regions. United States. https://doi.org/10.1063/1.5007082
Khrabry, A., Kaganovich, I. D., Nemchinsky, V., and Khodak, A. Mon . "Investigation of the short argon arc with hot anode. I. Numerical simulations of non-equilibrium effects in the near-electrode regions". United States. https://doi.org/10.1063/1.5007082. https://www.osti.gov/servlets/purl/1419791.
@article{osti_1419791,
title = {Investigation of the short argon arc with hot anode. I. Numerical simulations of non-equilibrium effects in the near-electrode regions},
author = {Khrabry, A. and Kaganovich, I. D. and Nemchinsky, V. and Khodak, A.},
abstractNote = {The atmospheric pressure arcs have recently found application in the production of nanoparticles. The distinguishing features of such arcs are small length and hot ablating anode characterized by intensive electron emission and radiation from its surface. We performed a one-dimensional modeling of argon arc, which shows that near-electrode effects of thermal and ionization non-equilibrium play an important role in the operation of a short arc, because the non-equilibrium regions are up to several millimeters long and are comparable to the arc length. The near-anode region is typically longer than the near-cathode region and its length depends more strongly on the current density. The model was extensively verified and validated against previous simulation results and experimental data. The Volt-Ampere characteristic (VAC) of the near-anode region depends on the anode cooling mechanism. The anode voltage is negative. In the case of strong anode cooling (water-cooled anode) when the anode is cold, temperature and plasma density gradients increase with current density, resulting in a decrease of the anode voltage (the absolute value increases). Falling VAC of the near-anode region suggests the arc constriction near the anode. Without anode cooling, the anode temperature increases significantly with the current density, leading to a drastic increase in the thermionic emission current from the anode. Correspondingly, the anode voltage increases to suppress the emission, and the opposite trend in the VAC is observed. The results of simulations were found to be independent of sheath model used: collisional (fluid) or collisionless model gave the same plasma profiles for both near-anode and near-cathode regions.},
doi = {10.1063/1.5007082},
journal = {Physics of Plasmas},
number = 1,
volume = 25,
place = {United States},
year = {Mon Jan 22 00:00:00 EST 2018},
month = {Mon Jan 22 00:00:00 EST 2018}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 33 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

One-dimensional analysis of the anode boundary layer in free-burning argon arcs
journal, January 1999

  • Tanaka, Manabu; Ushio, Masao; Wu, Chuan Song
  • Journal of Physics D: Applied Physics, Vol. 32, Issue 5
  • DOI: 10.1088/0022-3727/32/5/016

Prediction of anode temperatures of free burning arcs
journal, July 1995


Current density at the refractory cathode of a high-current high-pressure arc (two modes of cathode spot attachment)
journal, November 2003


Investigation of the short argon arc with hot anode. II. Analytical model
journal, January 2018

  • Khrabry, A.; Kaganovich, I. D.; Nemchinsky, V.
  • Physics of Plasmas, Vol. 25, Issue 1
  • DOI: 10.1063/1.5007084

Transport coefficients of ionized argon
journal, January 1973


A self-consistent three-dimensional model of the arc, electrode and weld pool in gas–metal arc welding
journal, April 2011


A model of the cathode region of atmospheric pressure arcs
journal, September 1995


Detection of nanoparticles in carbon arc discharge with laser-induced incandescence
journal, June 2017


Numerical model of the anode region of high-current electric arcs
journal, January 1997

  • Jenista, J.; Heberlein, V. R.; Pfender, E.
  • IEEE Transactions on Plasma Science, Vol. 25, Issue 5
  • DOI: 10.1109/27.649585

Gas Discharge Physics
book, January 1991


Ionization layer at the edge of a fully ionized plasma
journal, February 1998


Complex structure of the carbon arc discharge for synthesis of nanotubes
journal, June 2017

  • Vekselman, V.; Feurer, M.; Huang, T.
  • Plasma Sources Science and Technology, Vol. 26, Issue 6
  • DOI: 10.1088/1361-6595/aa7158

Prediction of properties of free burning arcs including effects of ambipolar diffusion
journal, December 1999

  • Sansonnens, L.; Haidar, J.; Lowke, J. J.
  • Journal of Physics D: Applied Physics, Vol. 33, Issue 2
  • DOI: 10.1088/0022-3727/33/2/309

Arc discharge with a vaporizable anode: Why is the fullerene formation process affected by the kind of buffer gas?
journal, October 2001

  • Alekseyev, N. I.; Dyuzhev, G. A.
  • Technical Physics, Vol. 46, Issue 10
  • DOI: 10.1134/1.1412058

Simulation of the layer of non-equilibrium ionization in a high-pressure argon plasma with multiply-charged ions
journal, March 2000

  • Almeida, R. M. S.; Benilov, M. S.; Naidis, G. V.
  • Journal of Physics D: Applied Physics, Vol. 33, Issue 8
  • DOI: 10.1088/0022-3727/33/8/312

Large-scale production of single-walled carbon nanotubes by the electric-arc technique
journal, August 1997

  • Journet, C.; Maser, W. K.; Bernier, P.
  • Nature, Vol. 388, Issue 6644, p. 756-758
  • DOI: 10.1038/41972

3D modelling of heating of thermionic cathodes by high-pressure arc plasmas
journal, May 2006


Numerical modelling of high-pressure arc discharges: matching the LTE arc core with the electrodes
journal, July 2017

  • Lisnyak, M.; Cunha, M. D.; Bauchire, J-M
  • Journal of Physics D: Applied Physics, Vol. 50, Issue 31
  • DOI: 10.1088/1361-6463/aa76d3

Modeling the anode boundary layer of high-intensity argon arcs
journal, August 1999


Numerical study of the anode boundary layer in atmospheric pressure arc discharges
journal, February 2016


Anode attachment modes and their formation in a high intensity argon arc
journal, June 2007


Unified modelling of near-cathode plasma layers in high-pressure arc discharges
journal, November 2008


Anode sheath transition in an anodic arc for synthesis of nanomaterials
journal, March 2016


A computational investigation of the effectiveness of different shielding gas mixtures for arc welding
journal, May 2009


Self-organisation processes in the carbon arc for nanosynthesis
journal, February 2015

  • Ng, J.; Raitses, Y.
  • Journal of Applied Physics, Vol. 117, Issue 6
  • DOI: 10.1063/1.4906784

Numerical simulation of carbon arc discharge for nanoparticle synthesis
journal, July 2012

  • Kundrapu, M.; Keidar, M.
  • Physics of Plasmas, Vol. 19, Issue 7
  • DOI: 10.1063/1.4737153

Determining synthesis region of the single wall carbon nanotubes in arc plasma volume
journal, October 2016


The anode region of electric arcs: a survey
journal, December 2009


Stable synthesis of few-layered boron nitride nanotubes by anodic arc discharge
journal, June 2017


Account of near-cathode sheath in numerical models of high-pressure arc discharges
journal, May 2016


Non-equilibrium modelling of transferred arcs
journal, January 1999


Plasma-aided nanofabrication: where is the cutting edge?
journal, April 2007


Two forms of attachment of an atmospheric-pressure direct-current arc in argon to a thermionic cathode
journal, June 2007


“Synthesis-on” and “synthesis-off” modes of carbon arc operation during synthesis of carbon nanotubes
journal, December 2017


Novel non-equilibrium modelling of a DC electric arc in argon
journal, May 2016


Formation of self-organized anode patterns in arc discharge simulations
journal, March 2013


Investigating near-anode plasma layers of very high-pressure arc discharges
journal, January 2009


Boundary conditions at the walls with thermionic electron emission in two temperature modeling of “thermal” plasmas
journal, August 2015

  • Pekker, Leonid; Hussary, Nakhleh
  • Physics of Plasmas, Vol. 22, Issue 8
  • DOI: 10.1063/1.4928882

Non-equilibrium Modeling of Tungsten-Inert Gas Arcs
journal, January 2017


Anode phenomena in arc discharges: a review
journal, January 2011


Gas discharge physics
journal, August 1993


Investigation of the Short Argon Arc with Hot Anode, Part II: Analytical Model
text, January 2017


Works referencing / citing this record:

Plasma parameters of microarcs towards minuscule discharge gap
journal, June 2020

  • Baeva, Margarita; Loffhagen, Detlef; Becker, Markus M.
  • Contributions to Plasma Physics
  • DOI: 10.1002/ctpp.202000033

Fluid Modelling of DC Argon Microplasmas: Effects of the Electron Transport Description
journal, April 2019

  • Baeva, M.; Loffhagen, D.; Becker, M. M.
  • Plasma Chemistry and Plasma Processing, Vol. 39, Issue 4
  • DOI: 10.1007/s11090-019-09994-5

Unified Non-equilibrium Modelling of Tungsten-Inert Gas Microarcs in Atmospheric Pressure Argon
journal, July 2019


Investigation of the short argon arc with hot anode. II. Analytical model
journal, January 2018

  • Khrabry, A.; Kaganovich, I. D.; Nemchinsky, V.
  • Physics of Plasmas, Vol. 25, Issue 1
  • DOI: 10.1063/1.5007084

Model for the operation of an emissive cathode in a large magnetized-plasma
journal, February 2019


Features of the arc binding region structure on the surface of the thoriated cathode in atmospheric pressured argon
journal, February 2020

  • Sargsyan, M. A.; Tereshonok, D. V.; Valyano, G. E.
  • Physics of Plasmas, Vol. 27, Issue 2
  • DOI: 10.1063/1.5142800

Modeling the physics of interaction of high-pressure arcs with their electrodes: advances and challenges
journal, October 2019


Quantitative imaging of carbon dimer precursor for nanomaterial synthesis in the carbon arc
journal, February 2018

  • Vekselman, V.; Khrabry, A.; Kaganovich, I.
  • Plasma Sources Science and Technology, Vol. 27, Issue 2
  • DOI: 10.1088/1361-6595/aaa735

3D numerical investigation of a free-burning argon arc with metal electrodes using a novel sheath coupling procedure
journal, November 2019


Synthesis of nanoparticles in carbon arc: measurements and modeling
journal, May 2018

  • Yatom, Shurik; Khrabry, Alexander; Mitrani, James
  • MRS Communications, Vol. 8, Issue 03
  • DOI: 10.1557/mrc.2018.91

Investigation of the Short Argon Arc with Hot Anode, Part II: Analytical Model
text, January 2017