Three-dimensional magnetic critical behavior in CrI3

Liu, Yu; Petrovic, C.

doi:10.1103/PhysRevB.97.014420

Title: Three-dimensional magnetic critical behavior in ${CrI}_{3}$

Abstract

CrI₃ is a promising candidate for the van der Waals bonded ferromagnetic devices since its ferromagnetism can be maintained upon exfoliating of bulk crystals down to single layer. In this work we studied critical properties of bulk CrI₃ single crystals around the paramagnetic to ferromagnetic phase transition. Critical exponents β= 0.260(4) with a critical temperature T_c= 60.05(13) K and γ= 1.136(6) with T_c= 60.43(4) K are obtained by the Kouvel-Fisher method, whereas δ= 5.32(2) is obtained by a critical isotherm analysis at T_c= 60 K. In conclusion, the critical exponents determined in bulk CrI₃ single crystals suggest a three-dimensional long-range magnetic coupling with the exchange distance decaying as J(r)≈r^-4:69

Authors:

Liu, Yu ^[1]; Petrovic, C. ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.

Publication Date:: Thu Jan 18 00:00:00 EST 2018

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

OSTI Identifier:: 1426456

Alternate Identifier(s):: OSTI ID: 1417417

Report Number(s):: BNL-203345-2018-JAAM
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1802286

Grant/Contract Number:: SC0012704

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 97; Journal Issue: 1; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 30 DIRECT ENERGY CONVERSION; ferromagnetism; magnetism; magnetic semiconductors; single crystal materials; magnetization measurements; x-ray diffraction

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                    Liu, Yu, and Petrovic, C. Three-dimensional magnetic critical behavior in CrI3.  United States: N. p., 2018. 
Web.  doi:10.1103/PhysRevB.97.014420.

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                    Liu, Yu, & Petrovic, C. Three-dimensional magnetic critical behavior in CrI3.  United States.  https://doi.org/10.1103/PhysRevB.97.014420

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                    Liu, Yu, and Petrovic, C. Thu .  
"Three-dimensional magnetic critical behavior in CrI3".  United States.  https://doi.org/10.1103/PhysRevB.97.014420.  https://www.osti.gov/servlets/purl/1426456.

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@article{osti_1426456,

  title        = {Three-dimensional magnetic critical behavior in CrI3},

  author       = {Liu, Yu and Petrovic, C.},

  abstractNote = {CrI3 is a promising candidate for the van der Waals bonded ferromagnetic devices since its ferromagnetism can be maintained upon exfoliating of bulk crystals down to single layer. In this work we studied critical properties of bulk CrI3 single crystals around the paramagnetic to ferromagnetic phase transition. Critical exponents β= 0.260(4) with a critical temperature Tc= 60.05(13) K and γ= 1.136(6) with Tc= 60.43(4) K are obtained by the Kouvel-Fisher method, whereas δ= 5.32(2) is obtained by a critical isotherm analysis at Tc= 60 K. In conclusion, the critical exponents determined in bulk CrI3 single crystals suggest a three-dimensional long-range magnetic coupling with the exchange distance decaying as J(r)≈r-4:69},

  doi          = {10.1103/PhysRevB.97.014420},

  journal      = {Physical Review B},

  number       = 1,

  volume       = 97,

  place        = {United States},

  year         = {Thu Jan 18 00:00:00 EST 2018},

  month        = {Thu Jan 18 00:00:00 EST 2018}

}

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https://doi.org/10.1103/PhysRevB.97.014420

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Cited by: 66 works

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FIG. 1: (a) Crystal structure of CrI₃ at room temperature. (b) Image of representative single crystals. (c) Single-crystal x-ray diffraction (XRD) and (d) powder XRD patterns of CrI₃ at room temperature. The vertical tick marks represent Bragg reflections of the C2/m space group.

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VI ₃ —a New Layered Ferromagnetic Semiconductor
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Title: Three-dimensional magnetic critical behavior in CrI 3

Abstract

Citation Formats

Figures / Tables:

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Title: Three-dimensional magnetic critical behavior in ${CrI}_{3}$

Critical scaling in the cubic helimagnet ${Cu}_{2}$ ${OSeO}_{3}$
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Critical exponents from field theory
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Detailed Magnetic Behavior of Nickel Near its Curie Point
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Magnetic behavior and spin-lattice coupling in cleavable van der Waals layered ${CrCl}_{3}$ crystals
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Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals
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Magnetic structure of the new layered ferromagnetic chromium hexatellurosilicate Cr2Si2Te6
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Critical magnetic properties of disordered polycrystalline ${Cr}_{75} {Fe}_{25}$ and ${Cr}_{70} {Fe}_{30}$ alloys
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Critical Exponents for Long-Range Interactions
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Approximate Equation of State For Nickel Near its Critical Temperature
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On a generalised approach to first and second order magnetic transitions
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