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Title: Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter

Authors:
ORCiD logo;  [1];  [2]; ;  [3]; ;  [4];
  1. Department of Civil and Environmental Engineering, Faculty of Science and Technology, University of Macau, Macau, China
  2. T. H. Chan School of Public Health, Harvard University, Boston, Massachusetts 02115, United States
  3. Aerodyne Research Inc., Billerica, Massachusetts 01821, United States
  4. Department of Chemistry, University of British Columbia, Vancouver, British Columbia, Canada
Publication Date:
Research Org.:
Harvard Univ., Cambridge, MA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1417220
Alternate Identifier(s):
OSTI ID: 1498677; OSTI ID: 1508596
Grant/Contract Number:  
SC0012792
Resource Type:
Published Article
Journal Name:
ACS Central Science
Additional Journal Information:
Journal Name: ACS Central Science Journal Volume: 4 Journal Issue: 2; Journal ID: ISSN 2374-7943
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 54 ENVIRONMENTAL SCIENCES

Citation Formats

Liu, Pengfei, Li, Yong Jie, Wang, Yan, Bateman, Adam P., Zhang, Yue, Gong, Zhaoheng, Bertram, Allan K., and Martin, Scot T. Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter. United States: N. p., 2018. Web. doi:10.1021/acscentsci.7b00452.
Liu, Pengfei, Li, Yong Jie, Wang, Yan, Bateman, Adam P., Zhang, Yue, Gong, Zhaoheng, Bertram, Allan K., & Martin, Scot T. Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter. United States. doi:10.1021/acscentsci.7b00452.
Liu, Pengfei, Li, Yong Jie, Wang, Yan, Bateman, Adam P., Zhang, Yue, Gong, Zhaoheng, Bertram, Allan K., and Martin, Scot T. Wed . "Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter". United States. doi:10.1021/acscentsci.7b00452.
@article{osti_1417220,
title = {Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter},
author = {Liu, Pengfei and Li, Yong Jie and Wang, Yan and Bateman, Adam P. and Zhang, Yue and Gong, Zhaoheng and Bertram, Allan K. and Martin, Scot T.},
abstractNote = {},
doi = {10.1021/acscentsci.7b00452},
journal = {ACS Central Science},
number = 2,
volume = 4,
place = {United States},
year = {2018},
month = {1}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1021/acscentsci.7b00452

Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

Figures / Tables:

Figure 1 Figure 1: (a) Schematic of ammonia reactive uptake for a highly viscous droplet in the left panel and a well-mixed liquid droplet in the right panel. The accessible reactive volume is highlighted in both panels. (b) A simplified mechanism of ammonia uptake and brown carbon production for SOM derived frommore » aromatic precursors. For instance, SOM carbonyls can react with ammonia to produce imines, which in turn oligomerize to yield conjugated light-absorbing organonitrogen compounds. This browning pathway competes with other reactions that may not produce chromophores, such as the NH3-neutralization of SOM carboxylic acids to form ammonium salts.« less

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Works referencing / citing this record:

Water diffusion measurements of single charged aerosols using H 2 O/D 2 O isotope exchange and Raman spectroscopy in an electrodynamic balance
journal, January 2019

  • Nadler, Katherine A.; Kim, Pyeongeun; Huang, Dao-Ling
  • Physical Chemistry Chemical Physics, Vol. 21, Issue 27
  • DOI: 10.1039/c8cp07052k

Water diffusion measurements of single charged aerosols using H 2 O/D 2 O isotope exchange and Raman spectroscopy in an electrodynamic balance
journal, January 2019

  • Nadler, Katherine A.; Kim, Pyeongeun; Huang, Dao-Ling
  • Physical Chemistry Chemical Physics, Vol. 21, Issue 27
  • DOI: 10.1039/c8cp07052k

    Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.