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Title: Magnetic properties of Sr 3 NiIrO 6 and Sr 3 CoIrO 6 : Magnetic hysteresis with coercive fields of up to 55 T

Here, we report extraordinarily large magnetic hysteresis loops in the iridates Sr 3NiIrO 5 and Sr 3CoIrO 6. We find coercive magnetic fields of up to 55 T with switched magnetic moments ≈1μ B per formula unit in Sr 3NiIrO 6 and coercive fields of up to 52 T with switched moments ≈3μ B per formula unit in Sr 3CoIrO 6. We propose that the magnetic hysteresis involves the field-induced evolution of quasi-one-dimensional chains in a frustrated triangular configuration. In conclusion, the striking magnetic behavior is likely to be linked to the unusual spin-orbit-entangled local state of the Ir 4+ ion and its potential for anisotropic exchange interactions.
Authors:
 [1] ;  [2] ;  [3] ;  [2] ;  [4] ;  [2] ;  [2] ;  [5] ;  [6] ;  [7] ;  [8] ;  [7] ;  [2]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Univ. of Oxford, Oxford (United Kingdom)
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  3. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Univ. of Oxford, Oxford (United Kingdom); Univ. of Edinburgh, Edinburgh (United Kingdom)
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Simon Fraser Univ., Burnaby, BC (Canada)
  5. Univ. of Oxford, Oxford (United Kingdom)
  6. Univ. of Warwick, Coventry (United Kingdom)
  7. Rutgers Univ., Piscataway, NJ (United States); Pohang Univ. of Science and Technology, Gyungbuk (Republic of Korea)
  8. Rutgers Univ., Piscataway, NJ (United States)
Publication Date:
Report Number(s):
LA-UR-17-28059
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1800998
Grant/Contract Number:
AC52-06NA25396
Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 94; Journal Issue: 22; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Research Org:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science
OSTI Identifier:
1417167
Alternate Identifier(s):
OSTI ID: 1334853

Singleton, John, Kim, Jae Wook, Topping, Craig V., Hansen, Anders, Mun, Eun -Deok, Chikara, S., Lakis, I., Ghannadzadeh, Saman, Goddard, Paul, Luo, Xuan, Oh, Yoon Seok, Cheong, Sang -Wook, and Zapf, Vivien S.. Magnetic properties of Sr3NiIrO6 and Sr3CoIrO6: Magnetic hysteresis with coercive fields of up to 55 T. United States: N. p., Web. doi:10.1103/PhysRevB.94.224408.
Singleton, John, Kim, Jae Wook, Topping, Craig V., Hansen, Anders, Mun, Eun -Deok, Chikara, S., Lakis, I., Ghannadzadeh, Saman, Goddard, Paul, Luo, Xuan, Oh, Yoon Seok, Cheong, Sang -Wook, & Zapf, Vivien S.. Magnetic properties of Sr3NiIrO6 and Sr3CoIrO6: Magnetic hysteresis with coercive fields of up to 55 T. United States. doi:10.1103/PhysRevB.94.224408.
Singleton, John, Kim, Jae Wook, Topping, Craig V., Hansen, Anders, Mun, Eun -Deok, Chikara, S., Lakis, I., Ghannadzadeh, Saman, Goddard, Paul, Luo, Xuan, Oh, Yoon Seok, Cheong, Sang -Wook, and Zapf, Vivien S.. 2016. "Magnetic properties of Sr3NiIrO6 and Sr3CoIrO6: Magnetic hysteresis with coercive fields of up to 55 T". United States. doi:10.1103/PhysRevB.94.224408. https://www.osti.gov/servlets/purl/1417167.
@article{osti_1417167,
title = {Magnetic properties of Sr3NiIrO6 and Sr3CoIrO6: Magnetic hysteresis with coercive fields of up to 55 T},
author = {Singleton, John and Kim, Jae Wook and Topping, Craig V. and Hansen, Anders and Mun, Eun -Deok and Chikara, S. and Lakis, I. and Ghannadzadeh, Saman and Goddard, Paul and Luo, Xuan and Oh, Yoon Seok and Cheong, Sang -Wook and Zapf, Vivien S.},
abstractNote = {Here, we report extraordinarily large magnetic hysteresis loops in the iridates Sr3NiIrO5 and Sr3CoIrO6. We find coercive magnetic fields of up to 55 T with switched magnetic moments ≈1μB per formula unit in Sr3NiIrO6 and coercive fields of up to 52 T with switched moments ≈3μB per formula unit in Sr3CoIrO6. We propose that the magnetic hysteresis involves the field-induced evolution of quasi-one-dimensional chains in a frustrated triangular configuration. In conclusion, the striking magnetic behavior is likely to be linked to the unusual spin-orbit-entangled local state of the Ir4+ ion and its potential for anisotropic exchange interactions.},
doi = {10.1103/PhysRevB.94.224408},
journal = {Physical Review B},
number = 22,
volume = 94,
place = {United States},
year = {2016},
month = {12}
}