Local nematic susceptibility in stressed from NMR electric field gradient measurements
Abstract
The electric field gradient (EFG) tensor at the 75As site couples to the orbital occupations of the As p orbitals and is a sensitive probe of local nematicity in BaFe2As2. We use nuclear magnetic resonance to measure the nuclear quadrupolar splittings and find that the EFG asymmetry responds linearly to the presence of a strain field in the paramagnetic phase. We extract the nematic susceptibility from the slope of this linear response as a function of temperature and find that it diverges near the structural transition, in agreement with other measures of the bulk nematic susceptibility. Our work establishes an alternative method to extract the nematic susceptibility which, in contrast to transport methods, can be extended inside the superconducting state.
- Authors:
-
- Univ. of California, Davis, CA (United States). Dept. of Physics
- TU Dresden, Dresden (Germany). Inst. for Solid State Physics
- Ames Lab. and Iowa State Univ., Ames, IA (United States). Dept. of Physics and Astronomy
- Univ. of Minnesota, Minneapolis, MN (United States). School of Physics and Astronomy
- Publication Date:
- Research Org.:
- Ames Laboratory (AMES), Ames, IA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; National Science Foundation (NSF); German Research Foundation (DFG)
- OSTI Identifier:
- 1415857
- Alternate Identifier(s):
- OSTI ID: 1414039; OSTI ID: 1464798
- Report Number(s):
- IS-J-9544
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1800860
- Grant/Contract Number:
- DMR-1506961; DMR-1607139; NA0002908; SC0012336; AC02-07CH11358
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 96; Journal Issue: 24; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; antiferromagnetism; high-temperature superconductors; nuclear quadrupole resonance
Citation Formats
Kissikov, T., Sarkar, R., Lawson, M., Bush, B. T., Timmons, E. I., Tanatar, M. A., Prozorov, R., Bud'ko, S. L., Canfield, P. C., Fernandes, R. M., Goh, W. F., Pickett, W. E., and Curro, N. J. Local nematic susceptibility in stressed BaFe2As2 from NMR electric field gradient measurements. United States: N. p., 2017.
Web. doi:10.1103/PhysRevB.96.241108.
Kissikov, T., Sarkar, R., Lawson, M., Bush, B. T., Timmons, E. I., Tanatar, M. A., Prozorov, R., Bud'ko, S. L., Canfield, P. C., Fernandes, R. M., Goh, W. F., Pickett, W. E., & Curro, N. J. Local nematic susceptibility in stressed BaFe2As2 from NMR electric field gradient measurements. United States. https://doi.org/10.1103/PhysRevB.96.241108
Kissikov, T., Sarkar, R., Lawson, M., Bush, B. T., Timmons, E. I., Tanatar, M. A., Prozorov, R., Bud'ko, S. L., Canfield, P. C., Fernandes, R. M., Goh, W. F., Pickett, W. E., and Curro, N. J. Tue .
"Local nematic susceptibility in stressed BaFe2As2 from NMR electric field gradient measurements". United States. https://doi.org/10.1103/PhysRevB.96.241108. https://www.osti.gov/servlets/purl/1415857.
@article{osti_1415857,
title = {Local nematic susceptibility in stressed BaFe2As2 from NMR electric field gradient measurements},
author = {Kissikov, T. and Sarkar, R. and Lawson, M. and Bush, B. T. and Timmons, E. I. and Tanatar, M. A. and Prozorov, R. and Bud'ko, S. L. and Canfield, P. C. and Fernandes, R. M. and Goh, W. F. and Pickett, W. E. and Curro, N. J.},
abstractNote = {The electric field gradient (EFG) tensor at the 75As site couples to the orbital occupations of the As p orbitals and is a sensitive probe of local nematicity in BaFe2As2. We use nuclear magnetic resonance to measure the nuclear quadrupolar splittings and find that the EFG asymmetry responds linearly to the presence of a strain field in the paramagnetic phase. We extract the nematic susceptibility from the slope of this linear response as a function of temperature and find that it diverges near the structural transition, in agreement with other measures of the bulk nematic susceptibility. Our work establishes an alternative method to extract the nematic susceptibility which, in contrast to transport methods, can be extended inside the superconducting state.},
doi = {10.1103/PhysRevB.96.241108},
journal = {Physical Review B},
number = 24,
volume = 96,
place = {United States},
year = {Tue Dec 19 00:00:00 EST 2017},
month = {Tue Dec 19 00:00:00 EST 2017}
}
Web of Science
Figures / Tables:
Works referenced in this record:
Electronic nematic susceptibility of iron-based superconductors
journal, January 2016
- Böhmer, Anna E.; Meingast, Christoph
- Comptes Rendus Physique, Vol. 17, Issue 1-2
Antiferromagnetic order and spin dynamics in iron-based superconductors
journal, August 2015
- Dai, Pengcheng
- Reviews of Modern Physics, Vol. 87, Issue 3
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Anisotropic thermodynamic and transport properties of single-crystalline ( and 0.45)
journal, July 2008
- Ni, N.; Bud’ko, S. L.; Kreyssig, A.
- Physical Review B, Vol. 78, Issue 1
Nematic spin correlations in the tetragonal state of uniaxial-strained BaFe2-xNixAs2
journal, July 2014
- Lu, X.; Park, J. T.; Zhang, R.
- Science, Vol. 345, Issue 6197
Cu Substitution Effects on the Local Magnetic Properties of : A Site-Selective and NMR Study
journal, September 2014
- Takeda, Hikaru; Imai, Takashi; Tachibana, Makoto
- Physical Review Letters, Vol. 113, Issue 11
Nanoscale Electronic Order in Iron Pnictides
journal, March 2010
- Lang, G.; Grafe, H. -J.; Paar, D.
- Physical Review Letters, Vol. 104, Issue 9
Critical quadrupole fluctuations and collective modes in iron pnictide superconductors
journal, February 2016
- Thorsmølle, V. K.; Khodas, M.; Yin, Z. P.
- Physical Review B, Vol. 93, Issue 5
and NMR investigation of lightly doped
journal, April 2009
- Ning, F. L.; Ahilan, K.; Imai, T.
- Physical Review B, Vol. 79, Issue 14
Dichotomy between in-plane magnetic susceptibility and resistivity anisotropies in extremely strained BaFe2As2
journal, September 2017
- He, Mingquan; Wang, Liran; Ahn, Felix
- Nature Communications, Vol. 8, Issue 1
Enhancement of Superconductivity near a Nematic Quantum Critical Point
journal, March 2015
- Lederer, S.; Schattner, Y.; Berg, E.
- Physical Review Letters, Vol. 114, Issue 9
Critical behavior of the spin density wave transition in underdoped ( ): NMR investigation
journal, June 2014
- Ning, F. L.; Fu, M.; Torchetti, D. A.
- Physical Review B, Vol. 89, Issue 21
Local magnetic inhomogeneities in as seen via NMR
journal, October 2010
- Dioguardi, A. P.; apRoberts-Warren, N.; Shockley, A. C.
- Physical Review B, Vol. 82, Issue 14
Observation of Incipient Charge Nematicity in
journal, December 2013
- Gallais, Y.; Fernandes, R. M.; Paul, I.
- Physical Review Letters, Vol. 111, Issue 26
Electronic reconstruction through the structural and magnetic transitions in detwinned NaFeAs
journal, July 2012
- Yi, M.; Lu, D. H.; Moore, R. G.
- New Journal of Physics, Vol. 14, Issue 7
Superconductivity in FeSe Thin Films Driven by the Interplay between Nematic Fluctuations and Spin-Orbit Coupling
journal, November 2016
- Kang, Jian; Fernandes, Rafael M.
- Physical Review Letters, Vol. 117, Issue 21
Thermopower as a Sensitive Probe of Electronic Nematicity in Iron Pnictides
journal, February 2013
- Jiang, Shuai; Jeevan, H. S.; Dong, Jinkui
- Physical Review Letters, Vol. 110, Issue 6
Divergent Nematic Susceptibility in an Iron Arsenide Superconductor
journal, August 2012
- Chu, J. -H.; Kuo, H. -H.; Analytis, J. G.
- Science, Vol. 337, Issue 6095
FeAs-Based Superconductivity: A Case Study of the Effects of Transition Metal Doping on BaFe 2 As 2
journal, August 2010
- Canfield, Paul C.; Bud'ko, Sergey L.
- Annual Review of Condensed Matter Physics, Vol. 1, Issue 1
Nuclear magnetic resonance probe head design for precision strain control
journal, October 2017
- Kissikov, T.; Sarkar, R.; Bush, B. T.
- Review of Scientific Instruments, Vol. 88, Issue 10
Evidence of local disorder in the overdoped regime of Ba(Fe Co ) As
journal, July 2011
- Park, Keeseong; Louca, Despina; Llobet, Anna
- Physical Review B, Vol. 84, Issue 2
Electronic properties of LaO 1− x F x FeAs in the normal state probed by NMR/NQR
journal, March 2009
- Grafe, H-J; Lang, G.; Hammerath, F.
- New Journal of Physics, Vol. 11, Issue 3
Magnetic fluctuations and superconducting properties of studied by NMR
journal, September 2017
- Cui, J.; Ding, Q. -P.; Meier, W. R.
- Physical Review B, Vol. 96, Issue 10
Uniaxial-strain mechanical detwinning of and crystals: Optical and transport study
journal, May 2010
- Tanatar, M. A.; Blomberg, E. C.; Kreyssig, A.
- Physical Review B, Vol. 81, Issue 18
Electronic nematicity above the structural and superconducting transition in BaFe2(As1−xP x )2
journal, June 2012
- Kasahara, S.; Shi, H. J.; Hashimoto, K.
- Nature, Vol. 486, Issue 7403
Origin of the Resistive Anisotropy in the Electronic Nematic Phase of Revealed by Optical Spectroscopy
journal, September 2015
- Mirri, C.; Dusza, A.; Bastelberger, S.
- Physical Review Letters, Vol. 115, Issue 10
NMR Evidence for Inhomogeneous Nematic Fluctuations in
journal, March 2016
- Dioguardi, A. P.; Kissikov, T.; Lin, C. H.
- Physical Review Letters, Vol. 116, Issue 10
Emergence of Orbital Nematicity in the Tetragonal Phase of BaFe 2 (As 1− x P x ) 2
journal, April 2015
- Iye, Tetsuya; Julien, Marc-Henri; Mayaffre, Hadrien
- Journal of the Physical Society of Japan, Vol. 84, Issue 4
In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor
journal, August 2010
- Chu, J. -H.; Analytis, J. G.; De Greve, K.
- Science, Vol. 329, Issue 5993
Effects of Nematic Fluctuations on the Elastic Properties of Iron Arsenide Superconductors
journal, October 2010
- Fernandes, R. M.; VanBebber, L. H.; Bhattacharya, S.
- Physical Review Letters, Vol. 105, Issue 15
Commensurate Itinerant Antiferromagnetism in BaFe 2 As 2 : 75 As-NMR Studies on a Self-Flux Grown Single Crystal
journal, November 2008
- Kitagawa, Kentaro; Katayama, Naoyuki; Ohgushi, Kenya
- Journal of the Physical Society of Japan, Vol. 77, Issue 11
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors
journal, May 2016
- Kuo, H. -H.; Chu, J. -H.; Palmstrom, J. C.
- Science, Vol. 352, Issue 6288
Origin of the Tetragonal-to-Orthorhombic Phase Transition in FeSe: A Combined Thermodynamic and NMR Study of Nematicity
journal, January 2015
- Böhmer, A. E.; Arai, T.; Hardy, F.
- Physical Review Letters, Vol. 114, Issue 2
Ambient- and low-temperature synchrotron x-ray diffraction study of BaFe As and CaFe As at high pressures up to 56 GPa
journal, February 2011
- Mittal, R.; Mishra, S. K.; Chaplot, S. L.
- Physical Review B, Vol. 83, Issue 5
Preemptive nematic order, pseudogap, and orbital order in the iron pnictides
journal, January 2012
- Fernandes, R. M.; Chubukov, A. V.; Knolle, J.
- Physical Review B, Vol. 85, Issue 2
Visualization of electron nematicity and unidirectional antiferroic fluctuations at high temperatures in NaFeAs
journal, February 2014
- Rosenthal, E. P.; Andrade, E. F.; Arguello, C. J.
- Nature Physics, Vol. 10, Issue 3
Electronic nematic correlations in the stress-free tetragonal state of
journal, October 2015
- Man, Haoran; Lu, Xingye; Chen, Justin S.
- Physical Review B, Vol. 92, Issue 13
Dichotomy between in-plane magnetic susceptibility and resistivity anisotropies in extremely strained BaFe₂As₂
text, January 2017
- He, Mingquan; Wang, Liran; Ahn, Felix
- Karlsruhe
Commensurate Itinerant Antiferromagnetism in BaFe2As2: 75As-NMR Studies on a Self-Flux Grown Single Crystal
text, January 2008
- Kitagawa, Kentaro; Katayama, Naoyuki; Ohgushi, Kenya
- arXiv
FeAs-based superconductivity: a case study of the effects of transition metal doping on BaFe2As2
text, January 2010
- Canfield, Paul C.; Bud'ko, Sergey L.
- arXiv
Preemptive nematic order, pseudogap, and orbital order in the iron pnictides
text, January 2011
- Fernandes, R. M.; Chubukov, A. V.; Knolle, J.
- arXiv
Effect of tensile stress on the in-plane resistivity anisotropy in BaFe2As2
text, January 2011
- Blomberg, E. C.; Kreyssig, A.; Tanatar, M. A.
- arXiv
Thermopower as sensitive probe of electronic nematicity in iron pnictides
text, January 2012
- Jiang, Shuai; Jeevan, H. S.; Dong, Jinkui
- arXiv
Visualization of Electron Nematicity and Unidirectional Antiferroic Fluctuations at High Temperatures in NaFeAs
text, January 2013
- Rosenthal, E. P.; Andrade, E. F.; Arguello, C. J.
- arXiv
Antiferromagnetic order and spin dynamics in iron-based superconductors
text, January 2015
- Dai, Pengcheng
- arXiv
Superconductivity in FeSe thin films driven by the interplay between nematic fluctuations and spin-orbit coupling
text, January 2016
- Kang, Jian; Fernandes, Rafael M.
- arXiv
Figures / Tables found in this record: