Importance of filter’s microstructure in dynamic filtration modeling of gasoline particulate filters (GPFs): Inhomogeneous porosity and pore size distribution
Abstract
The state-of-the-art multiscale modeling of gasoline particulate filter (GPF) including channel scale, wall scale, and pore scale is described. The microstructures of two GPFs were experimentally characterized. The pore size distributions of the GPFs were determined by mercury porosimetry. The porosity was measured by X-ray computed tomography (CT) and found to be inhomogeneous across the substrate wall. The significance of pore size distribution with respect to filtration performance was analyzed. The predictions of filtration efficiency were improved by including the pore size distribution in the filtration model. A dynamic heterogeneous multiscale filtration (HMF) model was utilized to simulate particulate filtration on a single channel particulate filter with realistic particulate emissions from a spark-ignition direct-injection (SIDI) gasoline engine. The dynamic evolution of filter’s microstructure and macroscopic filtration characteristics including mass- and number-based filtration efficiencies and pressure drop were predicted and discussed. In conclusion, the microstructure of the GPF substrate including inhomogeneous porosity and pore size distribution is found to significantly influence local particulate deposition inside the substrate and macroscopic filtration performance and is recommended to be resolved in the filtration model to simulate and evaluate the filtration performance of GPFs.
- Authors:
-
- Univ. of Wisconsin, Madison, WI (United States). Engine Research Center
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Texas A & M Univ., College Station, TX (United States). Dept. of Mechanical Engineering
- Publication Date:
- Research Org.:
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); USDOE Office of Science (SC), Biological and Environmental Research (BER)
- OSTI Identifier:
- 1415777
- Alternate Identifier(s):
- OSTI ID: 1548885
- Report Number(s):
- PNNL-SA-131440
Journal ID: ISSN 1385-8947; PII: S1385894718300068; TRN: US1800849
- Grant/Contract Number:
- AC0576RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Engineering Journal
- Additional Journal Information:
- Journal Volume: 338; Journal Issue: C; Journal ID: ISSN 1385-8947
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 42 ENGINEERING; Gasoline particulate filter; Particle filtration; Numerical simulation; Substrate microstructure; Particle number; Particle mass
Citation Formats
Gong, Jian, Stewart, Mark L., Zelenyuk, Alla, Strzelec, Andrea, Viswanathan, Sandeep, Rothamer, David A., Foster, David E., and Rutland, Christopher J. Importance of filter’s microstructure in dynamic filtration modeling of gasoline particulate filters (GPFs): Inhomogeneous porosity and pore size distribution. United States: N. p., 2018.
Web. doi:10.1016/J.CEJ.2018.01.006.
Gong, Jian, Stewart, Mark L., Zelenyuk, Alla, Strzelec, Andrea, Viswanathan, Sandeep, Rothamer, David A., Foster, David E., & Rutland, Christopher J. Importance of filter’s microstructure in dynamic filtration modeling of gasoline particulate filters (GPFs): Inhomogeneous porosity and pore size distribution. United States. https://doi.org/10.1016/J.CEJ.2018.01.006
Gong, Jian, Stewart, Mark L., Zelenyuk, Alla, Strzelec, Andrea, Viswanathan, Sandeep, Rothamer, David A., Foster, David E., and Rutland, Christopher J. Wed .
"Importance of filter’s microstructure in dynamic filtration modeling of gasoline particulate filters (GPFs): Inhomogeneous porosity and pore size distribution". United States. https://doi.org/10.1016/J.CEJ.2018.01.006. https://www.osti.gov/servlets/purl/1415777.
@article{osti_1415777,
title = {Importance of filter’s microstructure in dynamic filtration modeling of gasoline particulate filters (GPFs): Inhomogeneous porosity and pore size distribution},
author = {Gong, Jian and Stewart, Mark L. and Zelenyuk, Alla and Strzelec, Andrea and Viswanathan, Sandeep and Rothamer, David A. and Foster, David E. and Rutland, Christopher J.},
abstractNote = {The state-of-the-art multiscale modeling of gasoline particulate filter (GPF) including channel scale, wall scale, and pore scale is described. The microstructures of two GPFs were experimentally characterized. The pore size distributions of the GPFs were determined by mercury porosimetry. The porosity was measured by X-ray computed tomography (CT) and found to be inhomogeneous across the substrate wall. The significance of pore size distribution with respect to filtration performance was analyzed. The predictions of filtration efficiency were improved by including the pore size distribution in the filtration model. A dynamic heterogeneous multiscale filtration (HMF) model was utilized to simulate particulate filtration on a single channel particulate filter with realistic particulate emissions from a spark-ignition direct-injection (SIDI) gasoline engine. The dynamic evolution of filter’s microstructure and macroscopic filtration characteristics including mass- and number-based filtration efficiencies and pressure drop were predicted and discussed. In conclusion, the microstructure of the GPF substrate including inhomogeneous porosity and pore size distribution is found to significantly influence local particulate deposition inside the substrate and macroscopic filtration performance and is recommended to be resolved in the filtration model to simulate and evaluate the filtration performance of GPFs.},
doi = {10.1016/J.CEJ.2018.01.006},
journal = {Chemical Engineering Journal},
number = C,
volume = 338,
place = {United States},
year = {Wed Jan 03 00:00:00 EST 2018},
month = {Wed Jan 03 00:00:00 EST 2018}
}
Web of Science
Figures / Tables:
Works referenced in this record:
Science and technology of catalytic diesel particulate filters
journal, November 2001
- van Setten, Barry A. A. L.; Makkee, Michiel; Moulijn, Jacob A.
- Catalysis Reviews, Vol. 43, Issue 4
Black Carbon Emissions in Gasoline Exhaust and a Reduction Alternative with a Gasoline Particulate Filter
journal, May 2014
- Chan, Tak W.; Meloche, Eric; Kubsh, Joseph
- Environmental Science & Technology, Vol. 48, Issue 10
Review of Vehicular Emissions Trends
journal, January 2015
- Johnson, Timothy V.
- SAE International Journal of Engines, Vol. 8, Issue 3
Gasoline Particle Filter Development
journal, February 2017
- Lambert, Christine; Chanko, Timothy; Dobson, Douglas
- Emission Control Science and Technology, Vol. 3, Issue 1
Review of the state-of-the-art of exhaust particulate filter technology in internal combustion engines
journal, May 2015
- Guan, Bin; Zhan, Reggie; Lin, He
- Journal of Environmental Management, Vol. 154
Automotive spark-ignited direct-injection gasoline engines
journal, October 1999
- Zhao, F.; Lai, M. -C; Harrington, D. L.
- Progress in Energy and Combustion Science, Vol. 25, Issue 5
A Quasi-Dimensional NO x Emission Model for Spark Ignition Direct Injection (SIDI) Gasoline Engines
conference, April 2013
- Gong, Jian; Rutland, Christopher
- SAE 2013 World Congress & Exhibition, SAE Technical Paper Series
New Particulate Filter Concept to Reduce Particle Number Emissions
conference, April 2011
- Saito, Chika; Nakatani, Takahiko; Miyairi, Yukio
- SAE 2011 World Congress & Exhibition, SAE Technical Paper Series
Cost effectiveness of particulate filter installation on Direct Injection Gasoline vehicles
journal, October 2013
- Mamakos, Athanasios; Steininger, Nikolaus; Martini, Giorgio
- Atmospheric Environment, Vol. 77
Detailed characterization of particulates emitted by pre-commercial single-cylinder gasoline compression ignition engine
journal, August 2014
- Zelenyuk, Alla; Reitz, Paul; Stewart, Mark
- Combustion and Flame, Vol. 161, Issue 8
Physical and chemical characterization of SIDI engine particulates
journal, November 2013
- Gaddam, Chethan K.; Vander Wal, Randy L.
- Combustion and Flame, Vol. 160, Issue 11
Filtration Characteristics of Fuel Neutral Particulates Using a Heterogeneous Multiscale Filtration Model
journal, November 2015
- Gong, Jian; Rutland, Christopher J.
- Journal of Engineering for Gas Turbines and Power, Vol. 137, Issue 11
Light scattering technique for estimating soot mass loading in diesel particulate filters
journal, May 2009
- Kamimoto, T.; Murayama, Y.; Minagawa, T.
- International Journal of Engine Research, Vol. 10, Issue 5
Experimental Study on the Influence of DPF Micropore Structure and Particle Property on Its Filtration Process
journal, January 2016
- Meng, Zhongwei; Fang, Jia; Pu, Yunfei
- Journal of Combustion, Vol. 2016
Impact of filtration velocities and particulate matter characteristics on diesel particulate filter wall loading
journal, June 2009
- Yapaulo, R. A.; Wirojsakunchai, E.; Orita, T.
- International Journal of Engine Research, Vol. 10, Issue 5
Study on Wall Pore Structure for Next Generation Diesel Particulate Filter
conference, April 2008
- Mizuno, Yukio; Miyairi, Yukio; Katsube, Fumio
- SAE World Congress & Exhibition, SAE Technical Paper Series
Effects of Microstructure and Cell Geometry on Performance of Cordierite Diesel Particulate Filters
conference, March 2001
- Merkel, G. A.; Beall, D. M.; Hickman, D. L.
- SAE 2001 World Congress, SAE Technical Paper Series
Lattice-Boltzmann simulation of gas-particle flow in filters
journal, September 1997
- Filippova, O.; Hänel, D.
- Computers & Fluids, Vol. 26, Issue 7
A CFD-model describing filtration, regeneration and deposit rearrangement effects in gas filter systems
journal, January 2008
- Deuschle, Timo; Janoske, Uwe; Piesche, Manfred
- Chemical Engineering Journal, Vol. 135, Issue 1-2
PDF-Based Heterogeneous Multiscale Filtration Model
journal, April 2015
- Gong, Jian; Rutland, Christopher J.
- Environmental Science & Technology, Vol. 49, Issue 8
Nanoparticle motion trajectories and deposition in an inlet channel of wall-flow diesel particulate filter
journal, April 2009
- Liu, Yunqing; Gong, Jinke; Fu, Jun
- Journal of Aerosol Science, Vol. 40, Issue 4
Single wall diesel particulate filter (DPF) filtration efficiency studies using laboratory generated particles
journal, April 2009
- Yang, Juan; Stewart, Mark; Maupin, Gary
- Chemical Engineering Science, Vol. 64, Issue 8
Modelling of diesel particulate filtration in wall-flow traps
journal, November 2009
- Bensaid, S.; Marchisio, D. L.; Fino, D.
- Chemical Engineering Journal, Vol. 154, Issue 1-3
Modelling of diesel filters for particulates removal
journal, November 2009
- Schejbal, M.; Marek, M.; Kubíček, M.
- Chemical Engineering Journal, Vol. 154, Issue 1-3
Dynamic Heterogeneous Multiscale Filtration Model: Probing Micro- and Macroscopic Filtration Characteristics of Gasoline Particulate Filters
journal, September 2017
- Gong, Jian; Viswanathan, Sandeep; Rothamer, David A.
- Environmental Science & Technology, Vol. 51, Issue 19
Fundamental Studies of Diesel Particulate Filters: Transient Loading, Regeneration and Aging
conference, March 2000
- Konstandopoulos, Athanasios G.; Kostoglou, Margaritis; Skaperdas, Evangelos
- SAE 2000 World Congress, SAE Technical Paper Series
Effect of Particle Size Distribution on the Deep-Bed Capture Efficiency of an Exhaust Particulate Filter
journal, October 2015
- Viswanathan, Sandeep; Rothamer, David; Sakai, Stephen
- Journal of Engineering for Gas Turbines and Power, Vol. 137, Issue 10
Detailed characterization of particulate matter emitted by lean-burn gasoline direct injection engine
journal, November 2016
- Zelenyuk, Alla; Wilson, Jacqueline; Imre, Dan
- International Journal of Engine Research, Vol. 18, Issue 5-6
The effective density and fractal dimension of soot particles from premixed flames and motor vehicle exhaust
journal, October 2004
- Maricq, M. Matti; Xu, Ning
- Journal of Aerosol Science, Vol. 35, Issue 10
Study the DPF Regeneration at Transient Operating Conditions Using Integrated System-Level Model
conference, April 2010
- Gong, Jian; Rutland, Christopher J.
- SAE 2010 World Congress & Exhibition, SAE Technical Paper Series
A Model Development for Evaluating Soot-NO x Interactions in a Blended 2-Way Diesel Particulate Filter/Selective Catalytic Reduction
journal, November 2012
- Park, Soo-Youl; Narayanaswamy, Kushal; Schmieg, Steven J.
- Industrial & Engineering Chemistry Research, Vol. 51, Issue 48
Integrated Engine, Emissions, and Exhaust Aftertreatment System Level Models to Simulate DPF Regeneration
conference, October 2007
- Rutland, Christopher J.; England, Stephen B.; Foster, David E.
- Powertrain & Fluid Systems Conference and Exhibition, SAE Technical Paper Series
Pulsed Regeneration for DPF Aftertreatment Devices
conference, September 2011
- Gong, Jian; Rutland, Christopher J.
- 10th International Conference on Engines & Vehicles, SAE Technical Paper Series
Mathematical model of the thermal regeneration of a wall-flow monolith diesel particulate filter
journal, January 1984
- Bissett, Edward J.
- Chemical Engineering Science, Vol. 39, Issue 7-8
A One-Dimensional Computational Model for Studying the Filtration and Regeneration Characteristics of a Catalyzed Wall-Flow Diesel Particulate Filter
conference, March 2003
- Huynh, Cuong T.; Johnson, John H.; Yang, Song L.
- SAE 2003 World Congress & Exhibition, SAE Technical Paper Series
Simulating the Concentration Equations and the Gas-Wall Interface for One-Dimensional Based Diesel Particulate Filter Models
journal, November 2009
- Depcik, Christopher
- Journal of Engineering for Gas Turbines and Power, Vol. 132, Issue 3
Optimizing the Advanced Ceramic Material for Diesel Particulate Filter Applications
conference, April 2007
- Dillon, Heather; Stewart, Mark; Maupin, Gary
- SAE World Congress & Exhibition, SAE Technical Paper Series
Filtration and regeneration modeling for particulate filters with inhomogeneous wall structure
journal, July 2012
- Bollerhoff, Thomas; Markomanolakis, Ioannis; Koltsakis, Grigorios
- Catalysis Today, Vol. 188, Issue 1
Measurement and prediction of filtration efficiency evolution of soot loaded diesel particulate filters
journal, August 2010
- Tandon, Pushkar; Heibel, Achim; Whitmore, Jeanni
- Chemical Engineering Science, Vol. 65, Issue 16
Microscopic Visualization of PM Trapping and Regeneration in Micro-Structural Pores of a DPF Wall
journal, April 2009
- Karin, Preechar; Cui, Liyan; Rubio, Pedro
- SAE International Journal of Fuels and Lubricants, Vol. 2, Issue 1
Numerical simulation of soot filtration and combustion within diesel particulate filters
journal, January 2010
- Bensaid, Samir; Marchisio, Daniele L.; Fino, Debora
- Chemical Engineering Science, Vol. 65, Issue 1
Multi-Dimensional Modeling of the Soot Deposition Mechanism in Diesel Particulate Filters
journal, April 2008
- Piscaglia, F.; Onorati, A.; Rutland, C. J.
- SAE International Journal of Fuels and Lubricants, Vol. 1, Issue 1
Filtration modelling in wall-flow particulate filters of low soot penetration thickness
journal, October 2016
- Serrano, José Ramón; Climent, Héctor; Piqueras, Pedro
- Energy, Vol. 112
Filtration Efficiency and Pressure Drop of Miniature Diesel Particulate Filters
journal, April 2013
- Swanson, J.; Watts, W.; Kittelson, D.
- Aerosol Science and Technology, Vol. 47, Issue 4
Works referencing / citing this record:
Development of a Kalman filter estimator for simulation and control of particulate matter distribution of a diesel catalyzed particulate filter
journal, July 2018
- Singalandapuram Mahadevan, Boopathi; Johnson, John H.; Shahbakhti, Mahdi
- International Journal of Engine Research
3D pore analysis of gasoline particulate filters using X-ray tomography: impact of coating and ash loading
journal, January 2019
- Seong, Heeje; Choi, Seungmok; Matusik, Katarzyna E.
- Journal of Materials Science, Vol. 54, Issue 8
Development of GPF Using Micro-CT Measurement and Numerical Analytical Technique
journal, January 2019
- Nakayama, Hiroki; Banno, Yasuyuki; Mochizuki, Hiroshi
- Topics in Catalysis, Vol. 62, Issue 1-4
Figures / Tables found in this record: