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Title: Spectroscopic fast neutron transmission imaging in a treaty verification setting

Abstract

Measurements of the geometric configuration of objects and their material composition are needed for nuclear treaty verification purposes. We experimentally demonstrate a simple method based on monoenergetic fast neutron transmission to realize crude imaging of the geometric configuration of special nuclear material, confirm its fissionable content, and obtain information on its approximate fissile mass. In the experiment, we used monoenergetic neutrons from D(d, n)3He and T(d, n)4He reactions and a linear array of liquid scintillation detectors to perform spectroscopic neutron imaging of up to 13.7 kg of highly enriched uranium in a spherical geometry. We also show an example of detection of material diversion and confirm the presence of fissionable material based on the measurement of high-energy prompt fission neutrons, including estimating the quantity of material from the comparison of measured and predicted fission neutron emission rate. The combination of crude imaging and fissionable material detection and quantification in a simple approach may be attractive in certain treaty verification scenarios.

Authors:
 [1];  [1];  [1]
  1. Univ. of Michigan, Ann Arbor, MI (United States)
Publication Date:
Research Org.:
Univ. of Michigan, Ann Arbor, MI (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1499138
Alternate Identifier(s):
OSTI ID: 1415665
Grant/Contract Number:  
NA0002534
Resource Type:
Accepted Manuscript
Journal Name:
AIP Advances
Additional Journal Information:
Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Citation Formats

Ogren, K., Nattress, J., and Jovanovic, I. Spectroscopic fast neutron transmission imaging in a treaty verification setting. United States: N. p., 2018. Web. doi:10.1063/1.5004698.
Ogren, K., Nattress, J., & Jovanovic, I. Spectroscopic fast neutron transmission imaging in a treaty verification setting. United States. https://doi.org/10.1063/1.5004698
Ogren, K., Nattress, J., and Jovanovic, I. Thu . "Spectroscopic fast neutron transmission imaging in a treaty verification setting". United States. https://doi.org/10.1063/1.5004698. https://www.osti.gov/servlets/purl/1499138.
@article{osti_1499138,
title = {Spectroscopic fast neutron transmission imaging in a treaty verification setting},
author = {Ogren, K. and Nattress, J. and Jovanovic, I.},
abstractNote = {Measurements of the geometric configuration of objects and their material composition are needed for nuclear treaty verification purposes. We experimentally demonstrate a simple method based on monoenergetic fast neutron transmission to realize crude imaging of the geometric configuration of special nuclear material, confirm its fissionable content, and obtain information on its approximate fissile mass. In the experiment, we used monoenergetic neutrons from D(d, n)3He and T(d, n)4He reactions and a linear array of liquid scintillation detectors to perform spectroscopic neutron imaging of up to 13.7 kg of highly enriched uranium in a spherical geometry. We also show an example of detection of material diversion and confirm the presence of fissionable material based on the measurement of high-energy prompt fission neutrons, including estimating the quantity of material from the comparison of measured and predicted fission neutron emission rate. The combination of crude imaging and fissionable material detection and quantification in a simple approach may be attractive in certain treaty verification scenarios.},
doi = {10.1063/1.5004698},
journal = {AIP Advances},
number = 1,
volume = 8,
place = {United States},
year = {Thu Jan 04 00:00:00 EST 2018},
month = {Thu Jan 04 00:00:00 EST 2018}
}

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Works referenced in this record:

Rattling nucleons: New developments in active interrogation of special nuclear material
journal, January 2012

  • Runkle, Robert C.; Chichester, David L.; Thompson, Scott J.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 663, Issue 1
  • DOI: 10.1016/j.nima.2011.09.052

Compendium of Material Composition Data for Radiation Transport Modeling
report, March 2011

  • McConn, Ronald J.; Gesh, Christopher J.; Pagh, Richard T.
  • DOI: 10.2172/1023125

Direct reconstruction of the effective atomic number of materials by the method of multi-energy radiography
journal, February 2004

  • Naydenov, Sergey V.; Ryzhikov, Vladimir D.; Smith, Craig F.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 215, Issue 3-4
  • DOI: 10.1016/j.nimb.2003.09.020

Fissile mass estimation by pulsed neutron source interrogation
journal, June 2015

  • Israelashvili, I.; Dubi, C.; Ettedgui, H.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 785
  • DOI: 10.1016/j.nima.2015.02.048

Portable fast-neutron radiography with the nuclear materials identification system for fissile material transfers
journal, August 2007

  • Hausladen, P. A.; Bingham, P. R.; Neal, J. S.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 261, Issue 1-2, p. 387-390
  • DOI: 10.1016/j.nimb.2007.04.206

A zero-knowledge protocol for nuclear warhead verification
journal, June 2014

  • Glaser, Alexander; Barak, Boaz; Goldston, Robert J.
  • Nature, Vol. 510, Issue 7506
  • DOI: 10.1038/nature13457

Recent Fast Neutron Imaging Measurements with the Fieldable Nuclear Materials Identification System1
journal, January 2015


Linear models to perform treaty verification tasks for enhanced information security
journal, February 2017

  • MacGahan, Christopher J.; Kupinski, Matthew A.; Brubaker, Erik M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 844
  • DOI: 10.1016/j.nima.2016.11.010

Development and experimental validation of a monte carlo modeling of the neutron emission from a d-t generator
journal, January 2017

  • Remetti, Romolo; Lepore, Luigi; Cherubini, Nadia
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 842
  • DOI: 10.1016/j.nima.2016.10.031

Spectroscopic neutron radiography for a cargo scanning system
journal, June 2016

  • Rahon, Jill; Danagoulian, Areg; MacDonald, Thomas D.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 820
  • DOI: 10.1016/j.nima.2016.03.025

ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
journal, December 2011


Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging
journal, April 2016

  • Rose, P. B.; Erickson, A. S.; Mayer, M.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep24388

Neutron light output response and resolution functions in EJ-309 liquid scintillation detectors
journal, July 2013

  • Enqvist, Andreas; Lawrence, Christopher C.; Wieger, Brian M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 715
  • DOI: 10.1016/j.nima.2013.03.032

Proposed low-energy absolute calibration of nuclear recoils in a dual-phase noble element TPC using D-D neutron scattering kinematics
journal, April 2017

  • Verbus, J. R.; Rhyne, C. A.; Malling, D. C.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 851
  • DOI: 10.1016/j.nima.2017.01.053

Imaging for dismantlement verification: Information management and analysis algorithms
journal, January 2012

  • Robinson, S. M.; Jarman, K. D.; Pitts, W. K.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 662, Issue 1
  • DOI: 10.1016/j.nima.2011.09.036