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Title: Standardization of accelerator irradiation procedures for simulation of neutron induced damage in reactor structural materials

Abstract

Self-ion irradiation is widely used as a method to simulate neutron damage in reactor structural materials. Accelerator-based simulation of void swelling, however, introduces a number of neutron-atypical features which require careful data extraction and, in some cases, introduction of innovative irradiation techniques to alleviate these issues. In this paper, we briefly summarize three such atypical features: defect imbalance effects, pulsed beam effects, and carbon contamination. The latter issue has just been recently recognized as being relevant to simulation of void swelling and is discussed here in greater detail. It is shown that carbon ions are entrained in the ion beam by Coulomb force drag and accelerated toward the target surface. Beam-contaminant interactions are modeled using molecular dynamics simulation. Finally, by applying a multiple beam deflection technique, carbon and other contaminants can be effectively filtered out, as demonstrated in an irradiation of HT-9 alloy by 3.5 MeV Fe ions.

Authors:
ORCiD logo [1];  [1];  [2];  [1];  [1];  [3];  [4]
  1. Texas A & M Univ., College Station, TX (United States). Dept. of Nuclear Engineering
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  3. Texas A & M Univ., College Station, TX (United States). Dept. of Nuclear Engineering; Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
  4. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Publication Date:
Research Org.:
Texas A & M Univ., College Station, TX (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Org.:
USDOE Office of Nuclear Energy (NE)
OSTI Identifier:
1415407
Alternate Identifier(s):
OSTI ID: 1550186
Report Number(s):
LA-UR-17-25080
Journal ID: ISSN 0168-583X; TRN: US1800805
Grant/Contract Number:  
AC52-06NA25396; NE0008297
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms
Additional Journal Information:
Journal Volume: 409; Journal ID: ISSN 0168-583X
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; ion irradiation; beam contamination; carbon

Citation Formats

Shao, Lin, Gigax, Jonathan, Chen, Di, Kim, Hyosim, Garner, Frank A., Wang, Jing, and Toloczko, Mychailo B. Standardization of accelerator irradiation procedures for simulation of neutron induced damage in reactor structural materials. United States: N. p., 2017. Web. doi:10.1016/j.nimb.2017.05.026.
Shao, Lin, Gigax, Jonathan, Chen, Di, Kim, Hyosim, Garner, Frank A., Wang, Jing, & Toloczko, Mychailo B. Standardization of accelerator irradiation procedures for simulation of neutron induced damage in reactor structural materials. United States. https://doi.org/10.1016/j.nimb.2017.05.026
Shao, Lin, Gigax, Jonathan, Chen, Di, Kim, Hyosim, Garner, Frank A., Wang, Jing, and Toloczko, Mychailo B. Mon . "Standardization of accelerator irradiation procedures for simulation of neutron induced damage in reactor structural materials". United States. https://doi.org/10.1016/j.nimb.2017.05.026. https://www.osti.gov/servlets/purl/1415407.
@article{osti_1415407,
title = {Standardization of accelerator irradiation procedures for simulation of neutron induced damage in reactor structural materials},
author = {Shao, Lin and Gigax, Jonathan and Chen, Di and Kim, Hyosim and Garner, Frank A. and Wang, Jing and Toloczko, Mychailo B.},
abstractNote = {Self-ion irradiation is widely used as a method to simulate neutron damage in reactor structural materials. Accelerator-based simulation of void swelling, however, introduces a number of neutron-atypical features which require careful data extraction and, in some cases, introduction of innovative irradiation techniques to alleviate these issues. In this paper, we briefly summarize three such atypical features: defect imbalance effects, pulsed beam effects, and carbon contamination. The latter issue has just been recently recognized as being relevant to simulation of void swelling and is discussed here in greater detail. It is shown that carbon ions are entrained in the ion beam by Coulomb force drag and accelerated toward the target surface. Beam-contaminant interactions are modeled using molecular dynamics simulation. Finally, by applying a multiple beam deflection technique, carbon and other contaminants can be effectively filtered out, as demonstrated in an irradiation of HT-9 alloy by 3.5 MeV Fe ions.},
doi = {10.1016/j.nimb.2017.05.026},
journal = {Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms},
number = ,
volume = 409,
place = {United States},
year = {Mon Jun 12 00:00:00 EDT 2017},
month = {Mon Jun 12 00:00:00 EDT 2017}
}

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Cited by: 27 works
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Works referenced in this record:

Effect of defect imbalance on void swelling distributions produced in pure iron irradiated with 3.5 MeV self-ions
journal, October 2014


Retardation of boron diffusion in silicon by defect engineering
journal, April 2001

  • Shao, Lin; Lu, Xinming; Wang, Xuemei
  • Applied Physics Letters, Vol. 78, Issue 16
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The influence of ion beam rastering on the swelling of self-ion irradiated pure iron at 450 °C
journal, October 2015


Effect of irradiation mode on the microstructure of self-ion irradiated ferritic-martensitic alloys
journal, October 2015


Compositional and temperature dependence of void swelling in model Fe–Cr base alloys irradiated in the EBR-II fast reactor
journal, December 2000


Beam-contamination-induced compositional alteration and its neutron-atypical consequences in ion simulation of neutron-induced void swelling
journal, May 2017


Fast Parallel Algorithms for Short-Range Molecular Dynamics
journal, March 1995


Modeling injected interstitial effects on void swelling in self-ion irradiation experiments
journal, April 2016


Void swelling and microstructure evolution at very high damage level in self-ion irradiated ferritic-martensitic steels
journal, November 2016


Works referencing / citing this record:

Magnetic Properties of Proton Irradiated Mn3Si2Te6 van der Waals Single Crystals
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Carbon Contamination During Ion Irradiation - Accurate Detection and Characterization of its Effect on Microstructure of Ferritic/Martensitic Steels
journal, November 2017


Effect of Helium on Dispersoid Evolution under Self-Ion Irradiation in A Dual-Phase 12Cr Oxide-Dispersion-Strengthened Alloy
journal, October 2019

  • Kim, Hyosim; Wang, Tianyao; Gigax, Jonathan G.
  • Materials, Vol. 12, Issue 20
  • DOI: 10.3390/ma12203343

The Effect of Internal Free Surfaces on Void Swelling of Irradiated Pure Iron Containing Subsurface Trenches
journal, May 2019


Magnetic Properties of Proton Irradiated Fe2.7GeTe2 Bulk Crystals
journal, January 2019


Effect of Helium on Dispersoid Evolution under Self-Ion Irradiation in A Dual-Phase 12Cr Oxide-Dispersion-Strengthened Alloy
journal, October 2019

  • Kim, Hyosim; Wang, Tianyao; Gigax, Jonathan G.
  • Materials, Vol. 12, Issue 20
  • DOI: 10.3390/ma12203343