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Title: Unconventional spin dynamics in the honeycomb-lattice material α - RuCl 3 : High-field electron spin resonance studies

Abstract

Here, we present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material α-RuCl 3, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered phase, with magnetic field applied in the a b plane. A very rich excitation spectrum was observed in the field-induced quantum paramagnetic phase. We compare the data obtained with the results of recent numerical calculations, strongly suggesting a very unconventional multiparticle character of the spin dynamics in α-RuCl 3. Finally, the frequency-field diagram of the lowest-energy ESR mode is found consistent with the behavior of the field-induced energy gap, revealed by thermodynamic measurements.

Authors:
 [1];  [2];  [2];  [3];  [4];  [5];  [6];  [5];  [4];  [7];  [1]
  1. Helmholtz-Zentrum Berlin (HZB), (Germany). Dresden High Magnetic Field Lab. (HLD-EMFL)
  2. Helmholtz-Zentrum Berlin (HZB), (Germany). Dresden High Magnetic Field Lab. (HLD-EMFL); Technical Univ. of Dresden (Germany). Inst. of Solid State and Material Physics
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division; Univ. of Tennessee, Knoxville, TN (United States). Dept. of Materials Science and Engineering
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum of Materials Science and Engineering
  5. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division
  6. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical Science Division
  7. Taras Shevchenko National Univ., Kyiv (Ukraine). Inst. of High Technologies; National Academy of Sciences and Ministry of Education, Kyiv (Ukraine). Inst. of Magnetism
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1414677
Alternate Identifier(s):
OSTI ID: 1414037
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 96; Journal Issue: 24; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Ponomaryov, A. N., Schulze, E., Wosnitza, J., Lampen-Kelley, P., Banerjee, A., Yan, J. -Q., Bridges, C. A., Mandrus, D. G., Nagler, S. E., Kolezhuk, A. K., and Zvyagin, S. A. Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3 : High-field electron spin resonance studies. United States: N. p., 2017. Web. doi:10.1103/PhysRevB.96.241107.
Ponomaryov, A. N., Schulze, E., Wosnitza, J., Lampen-Kelley, P., Banerjee, A., Yan, J. -Q., Bridges, C. A., Mandrus, D. G., Nagler, S. E., Kolezhuk, A. K., & Zvyagin, S. A. Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3 : High-field electron spin resonance studies. United States. doi:10.1103/PhysRevB.96.241107.
Ponomaryov, A. N., Schulze, E., Wosnitza, J., Lampen-Kelley, P., Banerjee, A., Yan, J. -Q., Bridges, C. A., Mandrus, D. G., Nagler, S. E., Kolezhuk, A. K., and Zvyagin, S. A. Tue . "Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3 : High-field electron spin resonance studies". United States. doi:10.1103/PhysRevB.96.241107. https://www.osti.gov/servlets/purl/1414677.
@article{osti_1414677,
title = {Unconventional spin dynamics in the honeycomb-lattice material α-RuCl3 : High-field electron spin resonance studies},
author = {Ponomaryov, A. N. and Schulze, E. and Wosnitza, J. and Lampen-Kelley, P. and Banerjee, A. and Yan, J. -Q. and Bridges, C. A. and Mandrus, D. G. and Nagler, S. E. and Kolezhuk, A. K. and Zvyagin, S. A.},
abstractNote = {Here, we present high-field electron spin resonance (ESR) studies of the honeycomb-lattice material α-RuCl3, a prime candidate to exhibit Kitaev physics. Two modes of antiferromagnetic resonance were detected in the zigzag ordered phase, with magnetic field applied in the a b plane. A very rich excitation spectrum was observed in the field-induced quantum paramagnetic phase. We compare the data obtained with the results of recent numerical calculations, strongly suggesting a very unconventional multiparticle character of the spin dynamics in α-RuCl3. Finally, the frequency-field diagram of the lowest-energy ESR mode is found consistent with the behavior of the field-induced energy gap, revealed by thermodynamic measurements.},
doi = {10.1103/PhysRevB.96.241107},
journal = {Physical Review B},
number = 24,
volume = 96,
place = {United States},
year = {2017},
month = {12}
}

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Cited by: 17 works
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Figures / Tables:

FIG. 1 FIG. 1: (color online) (a) Schematic view of the α-RuCl3 crystal structure in the trigonal setting (ab view). The Ru3+ ions are shown in cyan, while the Cl ions are shown in red. (b) The reciprocal lattice of the honeycomb lattice (first and second Brillouin zones are shown).

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Works referenced in this record:

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