Investigation of the commensurate magnetic structure in the heavy-fermion compound using magnetic resonant x-ray diffraction
Abstract
In this paper, we investigated the magnetic structure of the heavy-fermion compound CePt2In7 below TN = 5.34 (2) K using magnetic resonant x-ray diffraction at ambient pressure. The magnetic order is characterized by a commensurate propagation vector k1/2 = (1/2, 1/2, 1/2) with spins lying in the basal plane. Our measurements did not reveal the presence of an incommensurate order propagating along the high-symmetry directions in reciprocal space but cannot exclude other incommensurate modulations or weak scattering intensities. The observed commensurate order can be described equivalently by either a single-k structure or by a multi-k structure. Furthermore we explain how a commensurate-only ordering may explain the broad distribution of internal fields observed in nuclear quadrupolar resonance experiments [Sakai et al., Phys. Rev. B 83, 140408 (2011)] that was previously attributed to an incommensurate order. We also report powder x-ray diffraction showing that the crystallographic structure of CePt2In7 changes monotonically with pressure up to P = 7.3 GPa at room temperature. The determined bulk modulus B0 = 81.1 (3) GPa is similar to those of the Ce-115 family. Broad diffraction peaks confirm the presence of pronounced strain in polycrystalline samples of CePt2In7. Lastly, we discuss how strain effects can lead tomore »
- Authors:
-
[5];
- Laboratory for Scientific Developments and Novel Materials, Paul Scherrer Institut (Switzerland)
- European Synchrotron Radiation Facility (France); University of Liverpool (United Kingdom)
- Laboratory for Synchrotron Radiation, Paul Scherrer Institut (Switzerland)
- Advanced Science Research Center, Japan Atomic Energy Agency (Japan)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut (Switzerland)
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE
- OSTI Identifier:
- 1414109
- Alternate Identifier(s):
- OSTI ID: 1374772
- Report Number(s):
- LA-UR-17-22945
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1800637
- Grant/Contract Number:
- AC52-06NA25396
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 96; Journal Issue: 6; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Antiferromagnetism; Heavy-fermion systems; Unconventional superconductors; X-ray powder diffraction; X-ray resonant magnetic scattering
Citation Formats
Gauthier, Nicolas, Wermeille, Didier, Casati, Nicola, Sakai, Hironori, Baumbach, Ryan E., Bauer, Eric D., and White, Jonathan S. Investigation of the commensurate magnetic structure in the heavy-fermion compound CePt2In7 using magnetic resonant x-ray diffraction. United States: N. p., 2017.
Web. doi:10.1103/PhysRevB.96.064414.
Gauthier, Nicolas, Wermeille, Didier, Casati, Nicola, Sakai, Hironori, Baumbach, Ryan E., Bauer, Eric D., & White, Jonathan S. Investigation of the commensurate magnetic structure in the heavy-fermion compound CePt2In7 using magnetic resonant x-ray diffraction. United States. https://doi.org/10.1103/PhysRevB.96.064414
Gauthier, Nicolas, Wermeille, Didier, Casati, Nicola, Sakai, Hironori, Baumbach, Ryan E., Bauer, Eric D., and White, Jonathan S. Thu .
"Investigation of the commensurate magnetic structure in the heavy-fermion compound CePt2In7 using magnetic resonant x-ray diffraction". United States. https://doi.org/10.1103/PhysRevB.96.064414. https://www.osti.gov/servlets/purl/1414109.
@article{osti_1414109,
title = {Investigation of the commensurate magnetic structure in the heavy-fermion compound CePt2In7 using magnetic resonant x-ray diffraction},
author = {Gauthier, Nicolas and Wermeille, Didier and Casati, Nicola and Sakai, Hironori and Baumbach, Ryan E. and Bauer, Eric D. and White, Jonathan S.},
abstractNote = {In this paper, we investigated the magnetic structure of the heavy-fermion compound CePt2In7 below TN = 5.34 (2) K using magnetic resonant x-ray diffraction at ambient pressure. The magnetic order is characterized by a commensurate propagation vector k1/2 = (1/2, 1/2, 1/2) with spins lying in the basal plane. Our measurements did not reveal the presence of an incommensurate order propagating along the high-symmetry directions in reciprocal space but cannot exclude other incommensurate modulations or weak scattering intensities. The observed commensurate order can be described equivalently by either a single-k structure or by a multi-k structure. Furthermore we explain how a commensurate-only ordering may explain the broad distribution of internal fields observed in nuclear quadrupolar resonance experiments [Sakai et al., Phys. Rev. B 83, 140408 (2011)] that was previously attributed to an incommensurate order. We also report powder x-ray diffraction showing that the crystallographic structure of CePt2In7 changes monotonically with pressure up to P = 7.3 GPa at room temperature. The determined bulk modulus B0 = 81.1 (3) GPa is similar to those of the Ce-115 family. Broad diffraction peaks confirm the presence of pronounced strain in polycrystalline samples of CePt2In7. Lastly, we discuss how strain effects can lead to different electronic and magnetic properties between polycrystalline and single crystal samples.},
doi = {10.1103/PhysRevB.96.064414},
journal = {Physical Review B},
number = 6,
volume = 96,
place = {United States},
year = {Thu Aug 10 00:00:00 EDT 2017},
month = {Thu Aug 10 00:00:00 EDT 2017}
}
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Works referencing / citing this record:
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