Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide
Abstract
Abstract Hybrid perovskites are on a trajectory toward realizing the most efficient single‐junction, solution‐processed photovoltaic devices. However, a critical issue is the limited understanding of the correlation between the degree of crystallinity and the emergent perovskite/hole (or electron) transport layer on device performance and photostability. Here, the controlled growth of hybrid perovskites on nickel oxide (NiO) is shown, resulting in the formation of thin films with enhanced crystallinity with characteristic peak width and splitting reminiscent of the tetragonal phase in single crystals. Photophysical and interface sensitive measurements reveal a reduced trap density at the perovskite/NiO interface in comparison with perovskites grown on poly(3,4‐ethylene dioxy thiophene) polystyrene sulfonate. Photovoltaic cells exhibit a high open circuit voltage (1.12 V), indicating a near‐ideal energy band alignment. Moreover, photostability of photovoltaic devices up to 10‐Suns is observed, which is a direct result of the superior crystallinity of perovskite thin films on NiO. These results elucidate the critical role of the quality of the perovskite/hole transport layer interface in rendering high‐performance and photostable optoelectronic devices.
- Authors:
-
[1];
[2];
[1];
[1];
[1];
[1];
[1]
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Rice Univ., Houston, TX (United States)
- Northwestern Univ., Evanston, IL (United States)
- Univ. de Rennes, Rennes (France)
- INSA de Rennes, Rennes (France)
- Rice Univ., Houston, TX (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1415423
- Alternate Identifier(s):
- OSTI ID: 1412593
- Report Number(s):
- LA-UR-17-28579
Journal ID: ISSN 0935-9648; TRN: US1800816
- Grant/Contract Number:
- AC52-06NA25396; 08SPCE973
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 5; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 14 SOLAR ENERGY; crystallinity; LiNiO; perovskite solar cells; photostability
Citation Formats
Nie, Wanyi, Tsai, Hsinhan, Blancon, Jean -Christophe, Liu, Fangze, Stoumpos, Costas C., Traore, Boubacar, Kepenekian, Mikael, Durand, Olivier, Katan, Claudine, Tretiak, Sergei, Crochet, Jared, Ajayan, Pulickel M., Kanatzidis, Mercouri, Even, Jacky, and Mohite, Aditya D. Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide. United States: N. p., 2017.
Web. doi:10.1002/adma.201703879.
Nie, Wanyi, Tsai, Hsinhan, Blancon, Jean -Christophe, Liu, Fangze, Stoumpos, Costas C., Traore, Boubacar, Kepenekian, Mikael, Durand, Olivier, Katan, Claudine, Tretiak, Sergei, Crochet, Jared, Ajayan, Pulickel M., Kanatzidis, Mercouri, Even, Jacky, & Mohite, Aditya D. Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide. United States. https://doi.org/10.1002/adma.201703879
Nie, Wanyi, Tsai, Hsinhan, Blancon, Jean -Christophe, Liu, Fangze, Stoumpos, Costas C., Traore, Boubacar, Kepenekian, Mikael, Durand, Olivier, Katan, Claudine, Tretiak, Sergei, Crochet, Jared, Ajayan, Pulickel M., Kanatzidis, Mercouri, Even, Jacky, and Mohite, Aditya D. Mon .
"Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide". United States. https://doi.org/10.1002/adma.201703879. https://www.osti.gov/servlets/purl/1415423.
@article{osti_1415423,
title = {Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide},
author = {Nie, Wanyi and Tsai, Hsinhan and Blancon, Jean -Christophe and Liu, Fangze and Stoumpos, Costas C. and Traore, Boubacar and Kepenekian, Mikael and Durand, Olivier and Katan, Claudine and Tretiak, Sergei and Crochet, Jared and Ajayan, Pulickel M. and Kanatzidis, Mercouri and Even, Jacky and Mohite, Aditya D.},
abstractNote = {Abstract Hybrid perovskites are on a trajectory toward realizing the most efficient single‐junction, solution‐processed photovoltaic devices. However, a critical issue is the limited understanding of the correlation between the degree of crystallinity and the emergent perovskite/hole (or electron) transport layer on device performance and photostability. Here, the controlled growth of hybrid perovskites on nickel oxide (NiO) is shown, resulting in the formation of thin films with enhanced crystallinity with characteristic peak width and splitting reminiscent of the tetragonal phase in single crystals. Photophysical and interface sensitive measurements reveal a reduced trap density at the perovskite/NiO interface in comparison with perovskites grown on poly(3,4‐ethylene dioxy thiophene) polystyrene sulfonate. Photovoltaic cells exhibit a high open circuit voltage (1.12 V), indicating a near‐ideal energy band alignment. Moreover, photostability of photovoltaic devices up to 10‐Suns is observed, which is a direct result of the superior crystallinity of perovskite thin films on NiO. These results elucidate the critical role of the quality of the perovskite/hole transport layer interface in rendering high‐performance and photostable optoelectronic devices.},
doi = {10.1002/adma.201703879},
journal = {Advanced Materials},
number = 5,
volume = 30,
place = {United States},
year = {Mon Dec 11 00:00:00 EST 2017},
month = {Mon Dec 11 00:00:00 EST 2017}
}
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- Liu, Chao Ping; Egbo, Kingsley O.; Ho, Chun Yuen
- Physical Review Applied, Vol. 11, Issue 1
Light-induced lattice expansion leads to high-efficiency perovskite solar cells
journal, April 2018
- Tsai, Hsinhan; Asadpour, Reza; Blancon, Jean-Christophe
- Science, Vol. 360, Issue 6384
Synthesis and Characterization of Graphene Oxide/Chitosan Composite Aerogels with High Mechanical Performance
journal, May 2019
- Gong, Yang; Yu, Yingchun; Kang, Huixuan
- Polymers, Vol. 11, Issue 5
Highly Efficient and Stable Planar Perovskite Solar Cells with Modulated Diffusion Passivation Toward High Power Conversion Efficiency and Ultrahigh Fill Factor
journal, November 2019
- Zhou, Long; Lin, Zhenhua; Ning, Zhijun
- Solar RRL, Vol. 3, Issue 11
A Cu 3 PS 4 nanoparticle hole selective layer for efficient inverted perovskite solar cells
journal, January 2019
- Yin, Xinxing; McClary, Scott A.; Song, Zhaoning
- Journal of Materials Chemistry A, Vol. 7, Issue 9
Control of Interface Defects for Efficient and Stable Quasi-2D Perovskite Light-Emitting Diodes Using Nickel Oxide Hole Injection Layer.
journalarticle, January 2018
- Lee, Seungjin; Kim, Da Bin; Hamilton, Iain
- Wiley
Stability and Dark Hysteresis Correlate in NiO-Based Perovskite Solar Cells
text, January 2019
- Di Girolamo, D.; Matteocci, F.; Kosasih, Felix
- Apollo - University of Cambridge Repository
Deepening the Valance Band Edges of NiO x Contacts by Alkaline Earth Metal Doping for Efficient Perovskite Photovoltaics with High Open‐Circuit Voltage
journal, May 2019
- Ge, Bing; Qiao, Hong Wei; Lin, Ze Qing
- Solar RRL, Vol. 3, Issue 8
Elucidating the Impact of Thin Film Texture on Charge Transport and Collection in Perovskite Solar Cells
journal, March 2018
- Jiang, Chuanpeng; Xie, Yuling; Lunt, Richard R.
- ACS Omega, Vol. 3, Issue 3
Design principles for electronic charge transport in solution-processed vertically stacked 2D perovskite quantum wells
journal, May 2018
- Tsai, Hsinhan; Asadpour, Reza; Blancon, Jean-Christophe
- Nature Communications, Vol. 9, Issue 1
The Impact of Hybrid Compositional Film/Structure on Organic–Inorganic Perovskite Solar Cells
journal, May 2018
- Wu, Yinghui; Chen, Wei; Chen, Guo
- Nanomaterials, Vol. 8, Issue 6
Synthesis and Characterization of Graphene Oxide/Chitosan Composite Aerogels with High Mechanical Performance
journal, May 2019
- Gong, Yang; Yu, Yingchun; Kang, Huixuan
- Polymers, Vol. 11, Issue 5