Title: Network design for quantifying urban CO₂ emissions: assessing trade-offs between precision and network density

Abstract

The majority of anthropogenic CO₂ emissions are attributable to urban areas. While the emissions from urban electricity generation often occur in locations remote from consumption, many of the other emissions occur within the city limits. Evaluating the effectiveness of strategies for controlling these emissions depends on our ability to observe urban CO₂ emissions and attribute them to specific activities. Cost-effective strategies for doing so have yet to be described. Here we characterize the ability of a prototype measurement network, modeled after the Berkeley Atmospheric CO₂ Observation Network (BEACO₂N) in California's Bay Area, in combination with an inverse model based on the coupled Weather Research and Forecasting/Stochastic Time-Inverted Lagrangian Transport (WRF-STILT) to improve our understanding of urban emissions. The pseudo-measurement network includes 34 sites at roughly 2 km spacing covering an area of roughly 400 km². The model uses an hourly 1  ×  1 km² emission inventory and 1  ×  1 km² meteorological calculations. We perform an ensemble of Bayesian atmospheric inversions to sample the combined effects of uncertainties of the pseudo-measurements and the model. We vary the estimates of the combined uncertainty of the pseudo-observations and model over a range of 20 to 0.005 ppm and vary the number of sites from 1 to 34. We use these inversions tomore » develop statistical models that estimate the efficacy of the combined model–observing system in reducing uncertainty in CO₂ emissions. We examine uncertainty in estimated CO₂ fluxes on the urban scale, as well as for sources embedded within the city such as a line source (e.g., a highway) or a point source (e.g., emissions from the stacks of small industrial facilities). Using our inversion framework, we find that a dense network with moderate precision is the preferred setup for estimating area, line, and point sources from a combined uncertainty and cost perspective. The dense network considered here (modeled after the BEACO₂N network with an assumed mismatch error of 1 ppm at an hourly temporal resolution) could estimate weekly CO₂ emissions from an urban region with less than 5 % error, given our characterization of the combined observation and model uncertainty.« less

Authors:

Turner, Alexander J.; Shusterman, Alexis A.; McDonald, Brian C.; Teige, Virginia; Harley, Robert A.; Cohen, Ronald C.

• Search DOE PAGES for author "Cohen, Ronald C."
• Search DOE PAGES for ORCID "0000-0001-6617-7691"

Publication Date:

Tue Nov 01 00:00:00 EDT 2016

Research Org.:

Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Org.:

USDOE Office of Science (SC), Advanced Scientific Computing Research (ASCR); National Science Foundation (NSF); Bay Area Air Quality Management District (BAAQMD) (United States)

OSTI Identifier:

1330588

Alternate Identifier(s):

OSTI ID: 1411643

Grant/Contract Number:  

AC02-05CH11231; 1035050; 2013.145

Resource Type:

Published Article

Journal Name:

Atmospheric Chemistry and Physics (Online)

Additional Journal Information:

Journal Name: Atmospheric Chemistry and Physics (Online) Journal Volume: 16 Journal Issue: 21; Journal ID: ISSN 1680-7324

Publisher:

Copernicus Publications, EGU

Country of Publication:

Germany

Language:

English

Subject:

54 ENVIRONMENTAL SCIENCES