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Title: Dye-sensitized electron transfer from TiO 2 to oxidized triphenylamines that follows first-order kinetics

Abstract

Two sensitizers, [Ru(bpy) 2 (dcb)] 2+ ( RuC ) and [Ru(bpy) 2 (dpb)] 2+ ( RuP ), were anchored to mesoporous TiO 2 thin films and utilized to sensitize the reaction of TiO 2 electrons with oxidized triphenylamines to visible light in CH 3 CN electrolytes.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
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  1. Department of Chemistry, University of North Carolina at Chapel Hill, Chapel Hill, USA
Publication Date:
Research Org.:
University of North Carolina, Chapel Hill, NC (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1411100
Alternate Identifier(s):
OSTI ID: 1505569
Grant/Contract Number:  
SC0013461
Resource Type:
Published Article
Journal Name:
Chemical Science
Additional Journal Information:
Journal Name: Chemical Science Journal Volume: 9 Journal Issue: 4; Journal ID: ISSN 2041-6520
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats

DiMarco, Brian N., Troian-Gautier, Ludovic, Sampaio, Renato N., and Meyer, Gerald J. Dye-sensitized electron transfer from TiO 2 to oxidized triphenylamines that follows first-order kinetics. United Kingdom: N. p., 2018. Web. doi:10.1039/C7SC03839A.
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DiMarco, Brian N., Troian-Gautier, Ludovic, Sampaio, Renato N., & Meyer, Gerald J. Dye-sensitized electron transfer from TiO 2 to oxidized triphenylamines that follows first-order kinetics. United Kingdom. https://doi.org/10.1039/C7SC03839A
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DiMarco, Brian N., Troian-Gautier, Ludovic, Sampaio, Renato N., and Meyer, Gerald J. Mon . "Dye-sensitized electron transfer from TiO 2 to oxidized triphenylamines that follows first-order kinetics". United Kingdom. https://doi.org/10.1039/C7SC03839A.
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@article{osti_1411100,
title = {Dye-sensitized electron transfer from TiO 2 to oxidized triphenylamines that follows first-order kinetics},
author = {DiMarco, Brian N. and Troian-Gautier, Ludovic and Sampaio, Renato N. and Meyer, Gerald J.},
abstractNote = {Two sensitizers, [Ru(bpy) 2 (dcb)] 2+ ( RuC ) and [Ru(bpy) 2 (dpb)] 2+ ( RuP ), were anchored to mesoporous TiO 2 thin films and utilized to sensitize the reaction of TiO 2 electrons with oxidized triphenylamines to visible light in CH 3 CN electrolytes.},
doi = {10.1039/C7SC03839A},
journal = {Chemical Science},
number = 4,
volume = 9,
place = {United Kingdom},
year = {Mon Jan 01 00:00:00 EST 2018},
month = {Mon Jan 01 00:00:00 EST 2018}
}
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https://doi.org/10.1039/C7SC03839A
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Cited by: 29 works
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Figures / Tables:

Scheme 1 Scheme 1: Mechanism for the photoinitiation of the desired reaction. Visible light absorption by the ruthenium sensitizer induced rapid excited-state electron injection to the acceptor state of TiO2, kinj > 108 s–1. The oxidized sensitizer is then regenerated by triphenylamine (TPA) with a rate constant kreg. This sequence provides themore » reactants for the desired charge recombination reaction of the injected electron with the oxidized triphenylamine redox mediator (krec) that was quantified over a 0.5 eV change in driving force.« less
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