A high-resolution and observationally constrained OMI NO2 satellite retrieval
Abstract
Here, this work presents a new high-resolution NO2 dataset derived from the NASA Ozone Monitoring Instrument (OMI) NO2 version 3.0 retrieval that can be used to estimate surface-level concentrations. The standard NASA product uses NO2 vertical profile shape factors from a 1.25° × 1° (~110 km × 110 km) resolution Global Model Initiative (GMI) model simulation to calculate air mass factors, a critical value used to determine observed tropospheric NO2 vertical columns. To better estimate vertical profile shape factors, we use a high-resolution (1.33 km × 1.33 km) Community Multi-scale Air Quality (CMAQ) model simulation constrained by in situ aircraft observations to recalculate tropospheric air mass factors and tropospheric NO2 vertical columns during summertime in the eastern US. In this new product, OMI NO2 tropospheric columns increase by up to 160% in city centers and decrease by 20–50 % in the rural areas outside of urban areas when compared to the operational NASA product. Our new product shows much better agreement with the Pandora NO2 and Airborne Compact Atmospheric Mapper (ACAM) NO2 spectrometer measurements acquired during the DISCOVER-AQ Maryland field campaign. Furthermore, the correlation between our satellite product and EPA NO2 monitors in urban areas has improved dramatically: r2 = 0.60 in the new productmore »
- Authors:
-
[4];
- Argonne National Lab. (ANL), Argonne, IL (United States); Univ. of Chicago, Chicago, IL (United States)
- Univ. Space Research Assoc., Columbia, MD (United States); NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States)
- NOAA Air Resources Lab., College Park, MD (United States); Univ. of Maryland, College Park, MD (United States)
- NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States); Johns Hopkins Univ. Applied Physics Lab., Laurel, MD (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USEPA
- OSTI Identifier:
- 1411029
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online); Journal Volume: 17; Journal Issue: 18; Journal ID: ISSN 1680-7324
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, and Streets, David G. A high-resolution and observationally constrained OMI NO2 satellite retrieval. United States: N. p., 2017.
Web. doi:10.5194/acp-17-11403-2017.
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, & Streets, David G. A high-resolution and observationally constrained OMI NO2 satellite retrieval. United States. https://doi.org/10.5194/acp-17-11403-2017
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, and Streets, David G. Tue .
"A high-resolution and observationally constrained OMI NO2 satellite retrieval". United States. https://doi.org/10.5194/acp-17-11403-2017. https://www.osti.gov/servlets/purl/1411029.
@article{osti_1411029,
title = {A high-resolution and observationally constrained OMI NO2 satellite retrieval},
author = {Goldberg, Daniel L. and Lamsal, Lok N. and Loughner, Christopher P. and Swartz, William H. and Lu, Zifeng and Streets, David G.},
abstractNote = {Here, this work presents a new high-resolution NO2 dataset derived from the NASA Ozone Monitoring Instrument (OMI) NO2 version 3.0 retrieval that can be used to estimate surface-level concentrations. The standard NASA product uses NO2 vertical profile shape factors from a 1.25° × 1° (~110 km × 110 km) resolution Global Model Initiative (GMI) model simulation to calculate air mass factors, a critical value used to determine observed tropospheric NO2 vertical columns. To better estimate vertical profile shape factors, we use a high-resolution (1.33 km × 1.33 km) Community Multi-scale Air Quality (CMAQ) model simulation constrained by in situ aircraft observations to recalculate tropospheric air mass factors and tropospheric NO2 vertical columns during summertime in the eastern US. In this new product, OMI NO2 tropospheric columns increase by up to 160% in city centers and decrease by 20–50 % in the rural areas outside of urban areas when compared to the operational NASA product. Our new product shows much better agreement with the Pandora NO2 and Airborne Compact Atmospheric Mapper (ACAM) NO2 spectrometer measurements acquired during the DISCOVER-AQ Maryland field campaign. Furthermore, the correlation between our satellite product and EPA NO2 monitors in urban areas has improved dramatically: r2 = 0.60 in the new product vs. r2 = 0.39 in the operational product, signifying that this new product is a better indicator of surface concentrations than the operational product. Our work emphasizes the need to use both high-resolution and high-fidelity models in order to recalculate satellite data in areas with large spatial heterogeneities in NOx emissions. Although the current work is focused on the eastern US, the methodology developed in this work can be applied to other world regions to produce high-quality region-specific NO2 satellite retrievals.},
doi = {10.5194/acp-17-11403-2017},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 18,
volume = 17,
place = {United States},
year = {Tue Sep 26 00:00:00 EDT 2017},
month = {Tue Sep 26 00:00:00 EDT 2017}
}
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journal, January 2020
- Choi, Sungyeon; Lamsal, Lok N.; Follette-Cook, Melanie
- Atmospheric Measurement Techniques, Vol. 13, Issue 5
Disentangling the Drivers of the Summertime Ozone‐Temperature Relationship Over the United States
journal, October 2019
- Kerr, Gaige Hunter; Waugh, Darryn W.; Strode, Sarah A.
- Journal of Geophysical Research: Atmospheres, Vol. 124, Issue 19
Retrieval of total column and surface NO2 from Pandora zenith-sky measurements
journal, January 2019
- Zhao, Xiaoyi; Griffin, Debora; Fioletov, Vitali
- Atmospheric Chemistry and Physics, Vol. 19, Issue 16
Mapping and Statistical Analysis of NO2 Concentration for Local Government Air Quality Regulation
journal, July 2019
- Ryu, Jieun; Park, Chan; Jeon, Seong Woo
- Sustainability, Vol. 11, Issue 14
NO 2 and HCHO measurements in Korea from 2012 to 2016 from Pandora spectrometer instruments compared with OMI retrievals and with aircraft measurements during the KORUS-AQ campaign
journal, January 2018
- Herman, Jay; Spinei, Elena; Fried, Alan
- Atmospheric Measurement Techniques, Vol. 11, Issue 8