A high-resolution and observationally constrained OMI NO 2 satellite retrieval
Abstract
Here, this work presents a new high-resolution NO 2 dataset derived from the NASA Ozone Monitoring Instrument (OMI) NO 2 version 3.0 retrieval that can be used to estimate surface-level concentrations. The standard NASA product uses NO 2 vertical profile shape factors from a 1.25° × 1° (~110 km × 110 km) resolution Global Model Initiative (GMI) model simulation to calculate air mass factors, a critical value used to determine observed tropospheric NO 2 vertical columns. To better estimate vertical profile shape factors, we use a high-resolution (1.33 km × 1.33 km) Community Multi-scale Air Quality (CMAQ) model simulation constrained by in situ aircraft observations to recalculate tropospheric air mass factors and tropospheric NO 2 vertical columns during summertime in the eastern US. In this new product, OMI NO 2 tropospheric columns increase by up to 160% in city centers and decrease by 20–50 % in the rural areas outside of urban areas when compared to the operational NASA product. Our new product shows much better agreement with the Pandora NO 2 and Airborne Compact Atmospheric Mapper (ACAM) NO 2 spectrometer measurements acquired during the DISCOVER-AQ Maryland field campaign. Furthermore, the correlation between our satellite product and EPA NO 2 monitors in urban areas hasmore »
- Authors:
- Argonne National Lab. (ANL), Argonne, IL (United States); Univ. of Chicago, Chicago, IL (United States)
- Univ. Space Research Assoc., Columbia, MD (United States); NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States)
- NOAA Air Resources Lab., College Park, MD (United States); Univ. of Maryland, College Park, MD (United States)
- NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States); Johns Hopkins Univ. Applied Physics Lab., Laurel, MD (United States)
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USEPA
- OSTI Identifier:
- 1411029
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online); Journal Volume: 17; Journal Issue: 18; Journal ID: ISSN 1680-7324
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, and Streets, David G. A high-resolution and observationally constrained OMI NO2 satellite retrieval. United States: N. p., 2017.
Web. doi:10.5194/acp-17-11403-2017.
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, & Streets, David G. A high-resolution and observationally constrained OMI NO2 satellite retrieval. United States. doi:10.5194/acp-17-11403-2017.
Goldberg, Daniel L., Lamsal, Lok N., Loughner, Christopher P., Swartz, William H., Lu, Zifeng, and Streets, David G. Tue .
"A high-resolution and observationally constrained OMI NO2 satellite retrieval". United States. doi:10.5194/acp-17-11403-2017. https://www.osti.gov/servlets/purl/1411029.
@article{osti_1411029,
title = {A high-resolution and observationally constrained OMI NO2 satellite retrieval},
author = {Goldberg, Daniel L. and Lamsal, Lok N. and Loughner, Christopher P. and Swartz, William H. and Lu, Zifeng and Streets, David G.},
abstractNote = {Here, this work presents a new high-resolution NO2 dataset derived from the NASA Ozone Monitoring Instrument (OMI) NO2 version 3.0 retrieval that can be used to estimate surface-level concentrations. The standard NASA product uses NO2 vertical profile shape factors from a 1.25° × 1° (~110 km × 110 km) resolution Global Model Initiative (GMI) model simulation to calculate air mass factors, a critical value used to determine observed tropospheric NO2 vertical columns. To better estimate vertical profile shape factors, we use a high-resolution (1.33 km × 1.33 km) Community Multi-scale Air Quality (CMAQ) model simulation constrained by in situ aircraft observations to recalculate tropospheric air mass factors and tropospheric NO2 vertical columns during summertime in the eastern US. In this new product, OMI NO2 tropospheric columns increase by up to 160% in city centers and decrease by 20–50 % in the rural areas outside of urban areas when compared to the operational NASA product. Our new product shows much better agreement with the Pandora NO2 and Airborne Compact Atmospheric Mapper (ACAM) NO2 spectrometer measurements acquired during the DISCOVER-AQ Maryland field campaign. Furthermore, the correlation between our satellite product and EPA NO2 monitors in urban areas has improved dramatically: r2 = 0.60 in the new product vs. r2 = 0.39 in the operational product, signifying that this new product is a better indicator of surface concentrations than the operational product. Our work emphasizes the need to use both high-resolution and high-fidelity models in order to recalculate satellite data in areas with large spatial heterogeneities in NOx emissions. Although the current work is focused on the eastern US, the methodology developed in this work can be applied to other world regions to produce high-quality region-specific NO2 satellite retrievals.},
doi = {10.5194/acp-17-11403-2017},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 18,
volume = 17,
place = {United States},
year = {2017},
month = {9}
}
Web of Science
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TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for global observations of the atmospheric composition for climate, air quality and ozone layer applications
journal, May 2012
- Veefkind, J. P.; Aben, I.; McMullan, K.
- Remote Sensing of Environment, Vol. 120
Validation of OMI tropospheric NO2 observations during INTEX-B and application to constrain NOxNOx emissions over the eastern United States and Mexico
journal, June 2008
- Boersma, K. F.; Jacob, D. J.; Bucsela, E. J.
- Atmospheric Environment, Vol. 42, Issue 19
Estimates of lightning NO x production based on OMI NO 2 observations over the Gulf of Mexico : Lightning NO
journal, July 2016
- Pickering, Kenneth E.; Bucsela, Eric; Allen, Dale
- Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 14
Why do models overestimate surface ozone in the Southeast United States?
journal, January 2016
- Travis, Katherine R.; Jacob, Daniel J.; Fisher, Jenny A.
- Atmospheric Chemistry and Physics, Vol. 16, Issue 21
Synergistic use of OMI NO2 tropospheric columns and LOTOS–EUROS to evaluate the NOx emission trends across Europe
journal, June 2014
- Curier, R. L.; Kranenburg, R.; Segers, A. J. S.
- Remote Sensing of Environment, Vol. 149
Tropospheric NO 2 column densities deduced from zenith-sky DOAS measurements in Shanghai, China, and their application to satellite validation
journal, January 2009
- Chen, D.; Zhou, B.; Beirle, S.
- Atmospheric Chemistry and Physics, Vol. 9, Issue 11
Structural uncertainty in air mass factor calculation for NO 2 and HCHO satellite retrievals
journal, January 2017
- Lorente, Alba; Folkert Boersma, K.; Yu, Huan
- Atmospheric Measurement Techniques, Vol. 10, Issue 3
A high spatial resolution retrieval of NO 2 column densities from OMI: method and evaluation
journal, January 2011
- Russell, A. R.; Perring, A. E.; Valin, L. C.
- Atmospheric Chemistry and Physics, Vol. 11, Issue 16
Satellite-Based NO 2 and Model Validation in a National Prediction Model Based on Universal Kriging and Land-Use Regression
journal, March 2016
- Young, Michael T.; Bechle, Matthew J.; Sampson, Paul D.
- Environmental Science & Technology, Vol. 50, Issue 7
OMI NO 2 column densities over North American urban cities: the effect of satellite footprint resolution
journal, January 2016
- Kim, Hyun Cheol; Lee, Pius; Judd, Laura
- Geoscientific Model Development, Vol. 9, Issue 3
Tropospheric NO 2 vertical column densities over Beijing: results of the first three years of ground-based MAX-DOAS measurements (2008–2011) and satellite validation
journal, January 2013
- Ma, J. Z.; Beirle, S.; Jin, J. L.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 3
Aura OMI observations of regional SO 2 and NO 2 pollution changes from 2005 to 2015
journal, January 2016
- Krotkov, Nickolay A.; McLinden, Chris A.; Li, Can
- Atmospheric Chemistry and Physics, Vol. 16, Issue 7
Relationship between column-density and surface mixing ratio: Statistical analysis of O3 and NO2 data from the July 2011 Maryland DISCOVER-AQ mission
journal, August 2014
- Flynn, Clare M.; Pickering, Kenneth E.; Crawford, James H.
- Atmospheric Environment, Vol. 92
Ships going slow in reducing their NOx emissions: changes in 2005–2012 ship exhaust inferred from satellite measurements over Europe
journal, July 2015
- Boersma, K. Folkert; Vinken, Geert C. M.; Tournadre, Jean
- Environmental Research Letters, Vol. 10, Issue 7
Enhanced representation of soil NO emissions in the Community Multiscale Air Quality (CMAQ) model version 5.0.2
journal, January 2016
- Rasool, Quazi Z.; Zhang, Rui; Lash, Benjamin
- Geoscientific Model Development, Vol. 9, Issue 9
Algorithm for NO/sub 2/ vertical column retrieval from the ozone monitoring instrument
journal, May 2006
- Bucsela, E. J.; Celarier, E. A.; Wenig, M. O.
- IEEE Transactions on Geoscience and Remote Sensing, Vol. 44, Issue 5
Global inventory of nitrogen oxide emissions constrained by space-based observations of NO 2 columns
journal, January 2003
- Martin, Randall V.
- Journal of Geophysical Research, Vol. 108, Issue D17
Variability of O3 and NO2 profile shapes during DISCOVER-AQ: Implications for satellite observations and comparisons to model-simulated profiles
journal, December 2016
- Flynn, Clare Marie; Pickering, Kenneth E.; Crawford, James H.
- Atmospheric Environment, Vol. 147
Interannual variability in soil nitric oxide emissions over the United States as viewed from space
journal, January 2010
- Hudman, R. C.; Russell, A. R.; Valin, L. C.
- Atmospheric Chemistry and Physics, Vol. 10, Issue 20
Evaluation of OMI operational standard NO 2 column retrievals using in situ and surface-based NO 2 observations
journal, January 2014
- Lamsal, L. N.; Krotkov, N. A.; Celarier, E. A.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 21
Tropospheric emissions: Monitoring of pollution (TEMPO)
journal, January 2017
- Zoogman, P.; Liu, X.; Suleiman, R. M.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 186
Long-term changes of tropospheric NO 2 over megacities derived from multiple satellite instruments
journal, January 2013
- Hilboll, A.; Richter, A.; Burrows, J. P.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 8
Impact of Bay-Breeze Circulations on Surface Air Quality and Boundary Layer Export
journal, July 2014
- Loughner, Christopher P.; Tzortziou, Maria; Follette-Cook, Melanie
- Journal of Applied Meteorology and Climatology, Vol. 53, Issue 7
Impacts of control strategies, the Great Recession and weekday variations on NO 2 columns above North American cities
journal, August 2016
- de Foy, Benjamin; Lu, Zifeng; Streets, David G.
- Atmospheric Environment, Vol. 138
Comparison of OMI NO 2 observations and their seasonal and
weekly cycles with ground-based measurements in Helsinki
journal, January 2016
- Ialongo, Iolanda; Herman, Jay; Krotkov, Nick
- Atmospheric Measurement Techniques, Vol. 9, Issue 10
Model study of the cross-tropopause transport of biomass burning pollution
journal, January 2007
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- Atmospheric Chemistry and Physics, Vol. 7, Issue 14
An improved tropospheric NO 2 column retrieval algorithm for the Ozone Monitoring Instrument
journal, January 2011
- Boersma, K. F.; Eskes, H. J.; Dirksen, R. J.
- Atmospheric Measurement Techniques, Vol. 4, Issue 9
Evaluation of nitrogen dioxide chemiluminescence monitors in a polluted urban environment
journal, January 2007
- Dunlea, E. J.; Herndon, S. C.; Nelson, D. D.
- Atmospheric Chemistry and Physics, Vol. 7, Issue 10
Air mass factor formulation for spectroscopic measurements from satellites: Application to formaldehyde retrievals from the Global Ozone Monitoring Experiment
journal, July 2001
- Palmer, Paul I.; Jacob, Daniel J.; Chance, Kelly
- Journal of Geophysical Research: Atmospheres, Vol. 106, Issue D13
National Satellite-Based Land-Use Regression: NO 2 in the United States
journal, May 2011
- Novotny, Eric V.; Bechle, Matthew J.; Millet, Dylan B.
- Environmental Science & Technology, Vol. 45, Issue 10
Estimates of power plant NOx emissions and lifetimes from OMI NO2 satellite retrievals
journal, September 2015
- de Foy, Benjamin; Lu, Zifeng; Streets, David G.
- Atmospheric Environment, Vol. 116
Worldwide biogenic soil NO x emissions inferred from OMI NO 2 observations
journal, January 2014
- Vinken, G. C. M.; Boersma, K. F.; Maasakkers, J. D.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 18
Analysis of aircraft and satellite measurements from the Intercontinental Chemical Transport Experiment (INTEX-B) to quantify long-range transport of East Asian sulfur to Canada
journal, January 2008
- van Donkelaar, A.; Martin, R. V.; Leaitch, W. R.
- Atmospheric Chemistry and Physics, Vol. 8, Issue 11
Near-real time retrieval of tropospheric NO<sub>2</sub> from OMI
journal, January 2007
- Boersma, K. F.; Eskes, H. J.; Veefkind, J. P.
- Atmospheric Chemistry and Physics, Vol. 7, Issue 8
Constraints on ship NO x emissions in Europe using GEOS-Chem and OMI satellite NO 2 observations
journal, January 2014
- Vinken, G. C. M.; Boersma, K. F.; van Donkelaar, A.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 3
Western European Land Use Regression Incorporating Satellite- and Ground-Based Measurements of NO 2 and PM 10
journal, November 2013
- Vienneau, Danielle; de Hoogh, Kees; Bechle, Matthew J.
- Environmental Science & Technology, Vol. 47, Issue 23
Assessment of NO2 satellite observations for en-route aircraft emissions detection
journal, December 2011
- Pujadas, Manuel; Núñez, Lourdes; Lubrani, Peter
- Remote Sensing of Environment, Vol. 115, Issue 12
Satellite NO2 retrievals suggest China has exceeded its NOx reduction goals from the twelfth Five-Year Plan
journal, October 2016
- de Foy, Benjamin; Lu, Zifeng; Streets, David G.
- Scientific Reports, Vol. 6, Issue 1
Higher surface ozone concentrations over the Chesapeake Bay than over the adjacent land: Observations and models from the DISCOVER-AQ and CBODAQ campaigns
journal, February 2014
- Goldberg, Daniel L.; Loughner, Christopher P.; Tzortziou, Maria
- Atmospheric Environment, Vol. 84
Daily Ambient NO 2 Concentration Predictions Using Satellite Ozone Monitoring Instrument NO 2 Data and Land Use Regression
journal, February 2014
- Lee, Hyung Joo; Koutrakis, Petros
- Environmental Science & Technology
Emissions estimation from satellite retrievals: A review of current capability
journal, October 2013
- Streets, David G.; Canty, Timothy; Carmichael, Gregory R.
- Atmospheric Environment, Vol. 77
A comparison study between CMAQ-simulated and OMI-retrieved NO 2 columns over East Asia for evaluation of NO x emission fluxes of INTEX-B, CAPSS, and REAS inventories
journal, January 2015
- Han, K. M.; Lee, S.; Chang, L. S.
- Atmospheric Chemistry and Physics, Vol. 15, Issue 4