Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice

Wan, Chunlei; Tian, Ruoming; Kondou, Mami; Yang, Ronggui; Zong, Pengan; Koumoto, Kunihito

doi:10.1038/s41467-017-01149-4

Title: Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice

Journal Article · 18 October 2017 · Nature Communications

DOI: https://doi.org/10.1038/s41467-017-01149-4 · OSTI ID:1406989

Wan, Chunlei ^[1]; Tian, Ruoming ^[2]; Kondou, Mami ^[3]; Yang, Ronggui ^[4]; Zong, Pengan ^[1]; Koumoto, Kunihito ^[2]

Tsinghua Univ., Beijing (China)
Toyota Physical and Chemical Research Institute, Nagakute (Japan)
Nagoya Univ., Nagoya (Japan)
Univ. of Colorado, Boulder, CO (United States); National Renewable Energy Lab. (NREL), Golden, CO (United States)

Hybrid inorganic–organic superlattice with an electron-transmitting but phonon-blocking structure has emerged as a promising flexible thin film thermoelectric material. However, the substantial challenge in optimizing carrier concentration without disrupting the superlattice structure prevents further improvement of the thermoelectric performance. Here we demonstrate a strategy for carrier optimization in a hybrid inorganic–organic superlattice of TiS₂[tetrabutylammonium] x [hexylammonium] y, where the organic layers are composed of a random mixture of tetrabutylammonium and hexylammonium molecules. By vacuum heating the hybrid materials at an intermediate temperature, the hexylammonium molecules with a lower boiling point are selectively de-intercalated, which reduces the electron density due to the requirement of electroneutrality. The tetrabutylammonium molecules with a higher boiling point remain to support and stabilize the superlattice structure. Furthermore, the carrier concentration can thus be effectively reduced, resulting in a remarkably high power factor of 904 µW m^–1 K^–2 at 300 K for flexible thermoelectrics, approaching the values achieved in conventional inorganic semiconductors.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1406989

Report Number(s):: NREL/JA-5500-70434

Journal Information:: Nature Communications, Vol. 8, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 131 works

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Thermoelectrics: Carbon nanotubes get high Crispin, Xavier Nature Energy, Vol. 1, Issue 4 https://doi.org/10.1038/nenergy.2016.37	journal	April 2016
Copper ion liquid-like thermoelectrics Liu, Huili; Shi, Xun; Xu, Fangfang Nature Materials, Vol. 11, Issue 5, p. 422-425 https://doi.org/10.1038/nmat3273	journal	March 2012
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Flexible n-type thermoelectric materials by organic intercalation of layered transition metal dichalcogenide TiS2 Wan, Chunlei; Gu, Xiaokun; Dang, Feng Nature Materials, Vol. 14, Issue 6 https://doi.org/10.1038/nmat4251	journal	April 2015
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