DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Perovskite Photovoltaics: The Path to a Printable Terawatt-Scale Technology

Abstract

Abundant, low-cost, reliable, and clean energy is critical not just to maintain but also to improve the living conditions across the globe. Because of the world's unrelenting population and GDP growth that is only slightly offset by reductions in energy intensity per $ of GDP, it has been estimated that by 2050 the world will consume an average of 30 Terawatts (TW) of total (i.e., not just electricity) energy, of which, assuming no current generation capacity retires, at least between 10-15 TW will be completely new capacity. Addressing this 'Terawatt challenge', a term originally coined by Richard Smalley in 2004, in a nonpolluting and sustainable way is integral to addressing socioeconomic needs in both industrial and rapidly developing countries worldwide. In conjunction with ongoing electrification of the energy system, the vastness of the available solar resource will provide a solution to the world's energy needs if we can develop sufficiently low-cost, high-performance, and massively scalable photovoltaic (PV) technology.

Authors:
 [1];  [1];  [1];  [1]; ORCiD logo [2]; ORCiD logo [1]
  1. National Renewable Energy Lab. (NREL), Golden, CO (United States)
  2. Univ. of Toledo, OH (United States)
Publication Date:
Research Org.:
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office
OSTI Identifier:
1405283
Report Number(s):
NREL/JA-5900-70242
Journal ID: ISSN 2380-8195
Grant/Contract Number:  
AC36-08GO28308
Resource Type:
Accepted Manuscript
Journal Name:
ACS Energy Letters
Additional Journal Information:
Journal Volume: 2; Journal Issue: 11; Journal ID: ISSN 2380-8195
Publisher:
American Chemical Society (ACS)
Country of Publication:
United States
Language:
English
Subject:
14 SOLAR ENERGY; 36 MATERIALS SCIENCE; HALIDE PEROVSKITE SOLAR CELLS; TERAWATT SCALE; SCALABLE TECHNOLOGY

Citation Formats

Berry, Joseph J., van de Lagemaat, Jao, Al-Jassim, Mowafak M., Kurtz, Sarah, Yan, Yanfa, and Zhu, Kai. Perovskite Photovoltaics: The Path to a Printable Terawatt-Scale Technology. United States: N. p., 2017. Web. doi:10.1021/acsenergylett.7b00964.
Berry, Joseph J., van de Lagemaat, Jao, Al-Jassim, Mowafak M., Kurtz, Sarah, Yan, Yanfa, & Zhu, Kai. Perovskite Photovoltaics: The Path to a Printable Terawatt-Scale Technology. United States. https://doi.org/10.1021/acsenergylett.7b00964
Berry, Joseph J., van de Lagemaat, Jao, Al-Jassim, Mowafak M., Kurtz, Sarah, Yan, Yanfa, and Zhu, Kai. Mon . "Perovskite Photovoltaics: The Path to a Printable Terawatt-Scale Technology". United States. https://doi.org/10.1021/acsenergylett.7b00964. https://www.osti.gov/servlets/purl/1405283.
@article{osti_1405283,
title = {Perovskite Photovoltaics: The Path to a Printable Terawatt-Scale Technology},
author = {Berry, Joseph J. and van de Lagemaat, Jao and Al-Jassim, Mowafak M. and Kurtz, Sarah and Yan, Yanfa and Zhu, Kai},
abstractNote = {Abundant, low-cost, reliable, and clean energy is critical not just to maintain but also to improve the living conditions across the globe. Because of the world's unrelenting population and GDP growth that is only slightly offset by reductions in energy intensity per $ of GDP, it has been estimated that by 2050 the world will consume an average of 30 Terawatts (TW) of total (i.e., not just electricity) energy, of which, assuming no current generation capacity retires, at least between 10-15 TW will be completely new capacity. Addressing this 'Terawatt challenge', a term originally coined by Richard Smalley in 2004, in a nonpolluting and sustainable way is integral to addressing socioeconomic needs in both industrial and rapidly developing countries worldwide. In conjunction with ongoing electrification of the energy system, the vastness of the available solar resource will provide a solution to the world's energy needs if we can develop sufficiently low-cost, high-performance, and massively scalable photovoltaic (PV) technology.},
doi = {10.1021/acsenergylett.7b00964},
journal = {ACS Energy Letters},
number = 11,
volume = 2,
place = {United States},
year = {Mon Oct 16 00:00:00 EDT 2017},
month = {Mon Oct 16 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 46 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Energy implications of future stabilization of atmospheric CO2 content
journal, October 1998

  • Hoffert, Martin I.; Caldeira, Ken; Jain, Atul K.
  • Nature, Vol. 395, Issue 6705
  • DOI: 10.1038/27638

Future Global Energy Prosperity: The Terawatt Challenge
journal, June 2005


24.7% Record Efficiency HIT Solar Cell on Thin Silicon Wafer
journal, January 2014


Silicon heterojunction solar cell with interdigitated back contacts for a photoconversion efficiency over 26%
journal, March 2017


A technoeconomic analysis of perovskite solar module manufacturing with low-cost materials and techniques
journal, January 2017

  • Song, Zhaoning; McElvany, Chad L.; Phillips, Adam B.
  • Energy & Environmental Science, Vol. 10, Issue 6
  • DOI: 10.1039/C7EE00757D

Solar cell efficiency tables (version 50)
journal, June 2017

  • Green, Martin A.; Hishikawa, Yoshihiro; Warta, Wilhelm
  • Progress in Photovoltaics: Research and Applications, Vol. 25, Issue 7
  • DOI: 10.1002/pip.2909

A large area (70 cm 2 ) monolithic perovskite solar module with a high efficiency and stability
journal, January 2016

  • Priyadarshi, Anish; Haur, Lew Jia; Murray, Paul
  • Energy & Environmental Science, Vol. 9, Issue 12
  • DOI: 10.1039/C6EE02693A

A solvent- and vacuum-free route to large-area perovskite films for efficient solar modules
journal, September 2017


Incorporation of rubidium cations into perovskite solar cells improves photovoltaic performance
journal, September 2016


High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells
journal, July 2016

  • Tsai, Hsinhan; Nie, Wanyi; Blancon, Jean-Christophe
  • Nature, Vol. 536, Issue 7616
  • DOI: 10.1038/nature18306

Efficient and stable solution-processed planar perovskite solar cells via contact passivation
journal, February 2017


Colloidally prepared La-doped BaSnO 3 electrodes for efficient, photostable perovskite solar cells
journal, March 2017


Perovskite ink with wide processing window for scalable high-efficiency solar cells
journal, March 2017


Perovskite Solar Cells—Towards Commercialization
journal, July 2017


Graphene Interface Engineering for Perovskite Solar Modules: 12.6% Power Conversion Efficiency over 50 cm 2 Active Area
journal, December 2016


Plasmonic-Induced Photon Recycling in Metal Halide Perovskite Solar Cells
journal, July 2015

  • Saliba, Michael; Zhang, Wei; Burlakov, Victor M.
  • Advanced Functional Materials, Vol. 25, Issue 31
  • DOI: 10.1002/adfm.201500669

Photon recycling in lead iodide perovskite solar cells
journal, March 2016


Quantification of re-absorption and re-emission processes to determine photon recycling efficiency in perovskite single crystals
journal, February 2017

  • Fang, Yanjun; Wei, Haotong; Dong, Qingfeng
  • Nature Communications, Vol. 8, Issue 1
  • DOI: 10.1038/ncomms14417

Detailed Balance Limit of Efficiency of p‐n Junction Solar Cells
journal, March 1961

  • Shockley, William; Queisser, Hans J.
  • Journal of Applied Physics, Vol. 32, Issue 3, p. 510-519
  • DOI: 10.1063/1.1736034

Detailed balance limit of the efficiency of tandem solar cells
journal, May 1980


Supercharging Silicon Solar Cell Performance by Means of Multijunction Concept
journal, May 2015

  • Almansouri, Ibraheem; Ho-Baillie, Anita; Bremner, Stephen P.
  • IEEE Journal of Photovoltaics, Vol. 5, Issue 3
  • DOI: 10.1109/JPHOTOV.2015.2395140

Selecting tandem partners for silicon solar cells
journal, September 2016


35.8% space and 38.8% terrestrial 5J direct bonded cells
conference, June 2014

  • Chiu, P. T.; Law, D. C.; Woo, R. L.
  • 2014 IEEE 40th Photovoltaic Specialists Conference (PVSC), 2014 IEEE 40th Photovoltaic Specialist Conference (PVSC)
  • DOI: 10.1109/PVSC.2014.6924957

Raising the one-sun conversion efficiency of III–V/Si solar cells to 32.8% for two junctions and 35.9% for three junctions
journal, August 2017


Flexible Thin-Film Tandem Solar Cells With >30% Efficiency
journal, March 2014


Rubidium Multication Perovskite with Optimized Bandgap for Perovskite-Silicon Tandem with over 26% Efficiency
journal, April 2017

  • Duong, The; Wu, YiLiang; Shen, Heping
  • Advanced Energy Materials, Vol. 7, Issue 14
  • DOI: 10.1002/aenm.201700228

23.6%-efficient monolithic perovskite/silicon tandem solar cells with improved stability
journal, February 2017

  • Bush, Kevin A.; Palmstrom, Axel F.; Yu, Zhengshan J.
  • Nature Energy, Vol. 2, Issue 4
  • DOI: 10.1038/nenergy.2017.9

High-efficiency inverted semi-transparent planar perovskite solar cells in substrate configuration
journal, December 2016


Low-bandgap mixed tin–lead iodide perovskite absorbers with long carrier lifetimes for all-perovskite tandem solar cells
journal, March 2017


Highly Efficient Perovskite-Perovskite Tandem Solar Cells Reaching 80% of the Theoretical Limit in Photovoltage
journal, July 2017

  • Rajagopal, Adharsh; Yang, Zhibin; Jo, Sae Byeok
  • Advanced Materials, Vol. 29, Issue 34
  • DOI: 10.1002/adma.201702140

LCA of renewable energy for electricity generation systems—A review
journal, June 2009


Selective dissolution of halide perovskites as a step towards recycling solar cells
journal, May 2016

  • Kim, Byeong Jo; Kim, Dong Hoe; Kwon, Seung Lee
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms11735

Recycling Perovskite Solar Cells To Avoid Lead Waste
journal, May 2016

  • Binek, Andreas; Petrus, Michiel L.; Huber, Niklas
  • ACS Applied Materials & Interfaces, Vol. 8, Issue 20
  • DOI: 10.1021/acsami.6b03767

Proof-of-concept for facile perovskite solar cell recycling
journal, January 2016

  • Kadro, Jeannette M.; Pellet, Norman; Giordano, Fabrizio
  • Energy & Environmental Science, Vol. 9, Issue 10
  • DOI: 10.1039/C6EE02013E

Towards stable and commercially available perovskite solar cells
journal, October 2016


Nonhazardous Solvent Systems for Processing Perovskite Photovoltaics
journal, May 2016

  • Gardner, Kira L.; Tait, Jeffrey G.; Merckx, Tamara
  • Advanced Energy Materials, Vol. 6, Issue 14
  • DOI: 10.1002/aenm.201600386

A low viscosity, low boiling point, clean solvent system for the rapid crystallisation of highly specular perovskite films
journal, January 2017

  • Noel, Nakita K.; Habisreutinger, Severin N.; Wenger, Bernard
  • Energy & Environmental Science, Vol. 10, Issue 1
  • DOI: 10.1039/C6EE02373H

Works referencing / citing this record:

Graphene-engineered automated sprayed mesoscopic structure for perovskite device scaling-up
journal, September 2018


Scalable fabrication of perovskite solar cells
journal, March 2018


Negligible‐Pb‐Waste and Upscalable Perovskite Deposition Technology for High‐Operational‐Stability Perovskite Solar Modules
journal, February 2019

  • Jiang, Yan; Remeika, Mikas; Hu, Zhanhao
  • Advanced Energy Materials, Vol. 9, Issue 13
  • DOI: 10.1002/aenm.201803047

Reducing Saturation-Current Density to Realize High-Efficiency Low-Bandgap Mixed Tin-Lead Halide Perovskite Solar Cells
journal, November 2018

  • Li, Chongwen; Song, Zhaoning; Zhao, Dewei
  • Advanced Energy Materials, Vol. 9, Issue 3
  • DOI: 10.1002/aenm.201803135

Rapid Aqueous Spray Fabrication of Robust NiO x : A Simple and Scalable Platform for Efficient Perovskite Solar Cells
journal, March 2019

  • Scheideler, William J.; Rolston, Nicholas; Zhao, Oliver
  • Advanced Energy Materials, Vol. 9, Issue 19
  • DOI: 10.1002/aenm.201803600

Research progress on organic–inorganic halide perovskite materials and solar cells
journal, February 2018


Layered Germanium Hybrid Perovskite Bromides: Insights from Experiments and First‐Principles Calculations
journal, April 2019

  • Chang, Xueqing; Marongiu, Daniela; Sarritzu, Valerio
  • Advanced Functional Materials, Vol. 29, Issue 31
  • DOI: 10.1002/adfm.201903528

Carrier lifetimes of >1 μs in Sn-Pb perovskites enable efficient all-perovskite tandem solar cells
journal, April 2019


Ag/In lead‐free double perovskites
journal, February 2020

  • Liu, Fang; Marongiu, Daniela; Pau, Riccardo
  • EcoMat, Vol. 2, Issue 1
  • DOI: 10.1002/eom2.12017

The Role of Graphene and Other 2D Materials in Solar Photovoltaics
journal, September 2018