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Title: Excitation energies, radiative and autoionization rates, dielectronic satellite lines, and dielectronic recombination rates for excited states of Rb-like W from Kr-like W [Relativistic atomic data for Rb-like tungsten]

Energy levels, radiative transition probabilities, and autoionization rates for [Ni]$$4{s}^{2}4{p}^{6}{nl}$$, [Ni]$$4{s}^{2}4{p}^{5}4l^{\prime} {nl}$$ ($$l^{\prime} =d,f,n$$ = 4–7), [Ni]$$4s4{p}^{6}4l^{\prime} {nl}$$, ($$l^{\prime} =d,f,n$$ = 4–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\prime} {nl}$$ (n = 5–7), and [Ni]$$4s4{p}^{6}6l^{\prime} {nl}$$ (n = 6–7) states in Rb-like tungsten (W37+) are calculated using the relativistic many-body perturbation theory method (RMBPT code) and the Hartree–Fock-relativistic method (COWAN code). Autoionizing levels above the [Ni]$$4{s}^{2}4{p}^{6}$$ threshold are considered. It is found that configuration mixing among [Ni]$$4{s}^{2}4{p}^{5}4l^{\prime} {nl}$$ and [Ni]$$4s4{p}^{6}4l^{\prime} {nl}$$ plays an important role for all atomic characteristics. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and dielectronic recombination (DR) rate coefficients are determined for the [Ni]$$4{s}^{2}4{p}^{6}{nl}$$ (n = 4–7) singly excited states, as well as the [Ni]$$4{s}^{2}4{p}^{5}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{5}4{fnl}$$, [Ni]$$4s4{p}^{6}4{dnl}$$, [Ni]$$4{s}^{2}4{p}^{6}4{fnl}$$, (n = 4–6), and [Ni]$$4{s}^{2}4{p}^{5}5l^{\prime} 5l$$ doubly excited nonautoionizing states in Rb-like W37+ ion. Contributions from the [Ni]$$4s24{p}^{6}4{fnl}$$ (n = 6–7), [Ni]$$4{s}^{2}4{p}^{5}5l^{\prime} {nl}$$ (n = 5–6), and [Ni]$$4{s}^{2}4{p}^{5}6l^{\prime} {nl}$$ (n = 6–7) doubly excited autoionizing states are evaluated numerically. The high-n state (with n up to 500) contributions are very important for high temperatures. These contributions are determined by using a scaling procedure. Synthetic dielectronic satellite spectra from Rb-like W are simulated in a broad spectral range from 8 to 70 Å. Here, these calculations provide highly accurate values for a number of W 37+ properties useful for a variety of applications including for fusion applications.
Authors:
 [1] ;  [1] ;  [2]
  1. Univ. of Nevada, Reno, NV (United States)
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Report Number(s):
LLNL-JRNL-680589
Journal ID: ISSN 0953-4075; TRN: US1703121
Grant/Contract Number:
AC52-07NA27344; AC52-07NA27344 NNSA DOE grant DE
Type:
Accepted Manuscript
Journal Name:
Journal of Physics. B, Atomic, Molecular and Optical Physics
Additional Journal Information:
Journal Volume: 49; Journal Issue: 22; Journal ID: ISSN 0953-4075
Publisher:
IOP Publishing
Research Org:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION; 74 ATOMIC AND MOLECULAR PHYSICS; atomic theory; dielectronic recombination; dielectronic satellite spectra; perturbation theory
OSTI Identifier:
1404833
Alternate Identifier(s):
OSTI ID: 1330735

Safronova, U. I., Safronova, A. S., and Beiersdorfer, P.. Excitation energies, radiative and autoionization rates, dielectronic satellite lines, and dielectronic recombination rates for excited states of Rb-like W from Kr-like W [Relativistic atomic data for Rb-like tungsten]. United States: N. p., Web. doi:10.1088/0953-4075/49/22/225002.
Safronova, U. I., Safronova, A. S., & Beiersdorfer, P.. Excitation energies, radiative and autoionization rates, dielectronic satellite lines, and dielectronic recombination rates for excited states of Rb-like W from Kr-like W [Relativistic atomic data for Rb-like tungsten]. United States. doi:10.1088/0953-4075/49/22/225002.
Safronova, U. I., Safronova, A. S., and Beiersdorfer, P.. 2016. "Excitation energies, radiative and autoionization rates, dielectronic satellite lines, and dielectronic recombination rates for excited states of Rb-like W from Kr-like W [Relativistic atomic data for Rb-like tungsten]". United States. doi:10.1088/0953-4075/49/22/225002. https://www.osti.gov/servlets/purl/1404833.
@article{osti_1404833,
title = {Excitation energies, radiative and autoionization rates, dielectronic satellite lines, and dielectronic recombination rates for excited states of Rb-like W from Kr-like W [Relativistic atomic data for Rb-like tungsten]},
author = {Safronova, U. I. and Safronova, A. S. and Beiersdorfer, P.},
abstractNote = {Energy levels, radiative transition probabilities, and autoionization rates for [Ni]$4{s}^{2}4{p}^{6}{nl}$, [Ni]$4{s}^{2}4{p}^{5}4l^{\prime} {nl}$ ($l^{\prime} =d,f,n$ = 4–7), [Ni]$4s4{p}^{6}4l^{\prime} {nl}$, ($l^{\prime} =d,f,n$ = 4–7), [Ni]$4{s}^{2}4{p}^{5}5l^{\prime} {nl}$ (n = 5–7), and [Ni]$4s4{p}^{6}6l^{\prime} {nl}$ (n = 6–7) states in Rb-like tungsten (W37+) are calculated using the relativistic many-body perturbation theory method (RMBPT code) and the Hartree–Fock-relativistic method (COWAN code). Autoionizing levels above the [Ni]$4{s}^{2}4{p}^{6}$ threshold are considered. It is found that configuration mixing among [Ni]$4{s}^{2}4{p}^{5}4l^{\prime} {nl}$ and [Ni]$4s4{p}^{6}4l^{\prime} {nl}$ plays an important role for all atomic characteristics. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and dielectronic recombination (DR) rate coefficients are determined for the [Ni]$4{s}^{2}4{p}^{6}{nl}$ (n = 4–7) singly excited states, as well as the [Ni]$4{s}^{2}4{p}^{5}4{dnl}$, [Ni]$4{s}^{2}4{p}^{5}4{fnl}$, [Ni]$4s4{p}^{6}4{dnl}$, [Ni]$4{s}^{2}4{p}^{6}4{fnl}$, (n = 4–6), and [Ni]$4{s}^{2}4{p}^{5}5l^{\prime} 5l$ doubly excited nonautoionizing states in Rb-like W37+ ion. Contributions from the [Ni]$4s24{p}^{6}4{fnl}$ (n = 6–7), [Ni]$4{s}^{2}4{p}^{5}5l^{\prime} {nl}$ (n = 5–6), and [Ni]$4{s}^{2}4{p}^{5}6l^{\prime} {nl}$ (n = 6–7) doubly excited autoionizing states are evaluated numerically. The high-n state (with n up to 500) contributions are very important for high temperatures. These contributions are determined by using a scaling procedure. Synthetic dielectronic satellite spectra from Rb-like W are simulated in a broad spectral range from 8 to 70 Å. Here, these calculations provide highly accurate values for a number of W37+ properties useful for a variety of applications including for fusion applications.},
doi = {10.1088/0953-4075/49/22/225002},
journal = {Journal of Physics. B, Atomic, Molecular and Optical Physics},
number = 22,
volume = 49,
place = {United States},
year = {2016},
month = {11}
}