Hydrothermal synthesis of silicon oxide clad uranium oxide nanowires
Abstract
Here, a facile method to synthesize silicon oxide clad uranium oxide nanowires is presented. U3Si2, used as a precursor, was oxidized to produce uranium oxide nanocrystallites and amorphous silicon oxide under hydrothermal conditions at 300°C and a pressure of 7.8 × 106 Pa. The growth of uranium oxide nanowires was assisted by silicon oxide via assembling the uranium oxide nanocrystallites in an amorphous silicon oxide matrix. The microstructure and composition of silicon oxide clad uranium oxide nanowires were characterized by XRD, SEM, TEM, and EDS. The uranium oxide in the nanowires was determined as UO2.34 with a fluoride cubic structure.
- Authors:
-
- Idaho National Lab. (INL), Idaho Falls, ID (United States)
- Publication Date:
- Research Org.:
- Idaho National Laboratory (INL), Idaho Falls, ID (United States)
- Sponsoring Org.:
- USDOE Office of Nuclear Energy (NE); Westinghouse Electric Company LLC, Cranberry Township, PA (United States)
- OSTI Identifier:
- 1402684
- Alternate Identifier(s):
- OSTI ID: 1408185
- Report Number(s):
- INL/JOU-17-43006
Journal ID: ISSN 0002-7820
- Grant/Contract Number:
- AC07-05ID14517; FOA‐0000712; FOA-0000712; AC07-051D14517
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Ceramic Society
- Additional Journal Information:
- Journal Volume: 101; Journal Issue: 3; Journal ID: ISSN 0002-7820
- Publisher:
- American Ceramic Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY; hydrothermal; nanomaterials; nanowires; oxides; uranium/uranium compounds
Citation Formats
He, Lingfeng, Harp, Jason M., Wagner, Adrian R., Hoggan, Rita E., and Tolman, Kevin R.. Hydrothermal synthesis of silicon oxide clad uranium oxide nanowires. United States: N. p., 2017.
Web. doi:10.1111/jace.15295.
He, Lingfeng, Harp, Jason M., Wagner, Adrian R., Hoggan, Rita E., & Tolman, Kevin R.. Hydrothermal synthesis of silicon oxide clad uranium oxide nanowires. United States. https://doi.org/10.1111/jace.15295
He, Lingfeng, Harp, Jason M., Wagner, Adrian R., Hoggan, Rita E., and Tolman, Kevin R.. Wed .
"Hydrothermal synthesis of silicon oxide clad uranium oxide nanowires". United States. https://doi.org/10.1111/jace.15295. https://www.osti.gov/servlets/purl/1402684.
@article{osti_1402684,
title = {Hydrothermal synthesis of silicon oxide clad uranium oxide nanowires},
author = {He, Lingfeng and Harp, Jason M. and Wagner, Adrian R. and Hoggan, Rita E. and Tolman, Kevin R.},
abstractNote = {Here, a facile method to synthesize silicon oxide clad uranium oxide nanowires is presented. U3Si2, used as a precursor, was oxidized to produce uranium oxide nanocrystallites and amorphous silicon oxide under hydrothermal conditions at 300°C and a pressure of 7.8 × 106 Pa. The growth of uranium oxide nanowires was assisted by silicon oxide via assembling the uranium oxide nanocrystallites in an amorphous silicon oxide matrix. The microstructure and composition of silicon oxide clad uranium oxide nanowires were characterized by XRD, SEM, TEM, and EDS. The uranium oxide in the nanowires was determined as UO2.34 with a fluoride cubic structure.},
doi = {10.1111/jace.15295},
journal = {Journal of the American Ceramic Society},
number = 3,
volume = 101,
place = {United States},
year = {2017},
month = {11}
}
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