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Title: Topological-insulator-based terahertz modulator

Abstract

Three dimensional topological insulators, as a new phase of quantum matters, are characterized by an insulating gap in the bulk and a metallic state on the surface. Particularly, most of the topological insulators have narrow band gaps, and hence have promising applications in the area of terahertz optoelectronics. In this work, we experimentally demonstrate an electronically-tunable terahertz intensity modulator based on Bi1:5Sb0:5Te1:8Se1:2 single crystal, one of the most insulating topological insulators. A relative frequency-independent modulation depth of ~62% over a wide frequency range from 0.3 to 1.4 THz has been achieved at room temperature, by applying a bias current of 100 mA. The modulation in the low current regime can be further enhanced at low temperature. We propose that the extraordinarily large modulation is a consequence of thermally-activated carrier absorption in the semiconducting bulk states. Our work provides a new application of topological insulators for terahertz technology.

Authors:
 [1];  [1];  [2];  [2];  [3];  [4];  [2]; ORCiD logo [1]
  1. Nanyang Technological Univ. (Singapore)
  2. National Univ. of Singapore (Singapore)
  3. RMIT Univ., Melbourne, VIC (Australia)
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1402632
Report Number(s):
LA-UR-17-23589
Journal ID: ISSN 2045-2322
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Wang, X. B., Cheng, L., Wu, Y., Zhu, D. P., Wang, L., Zhu, Jian-Xin, Yang, Hyunsoo, and Chia, Elbert E. M. Topological-insulator-based terahertz modulator. United States: N. p., 2017. Web. doi:10.1038/s41598-017-13701-9.
Wang, X. B., Cheng, L., Wu, Y., Zhu, D. P., Wang, L., Zhu, Jian-Xin, Yang, Hyunsoo, & Chia, Elbert E. M. Topological-insulator-based terahertz modulator. United States. https://doi.org/10.1038/s41598-017-13701-9
Wang, X. B., Cheng, L., Wu, Y., Zhu, D. P., Wang, L., Zhu, Jian-Xin, Yang, Hyunsoo, and Chia, Elbert E. M. Wed . "Topological-insulator-based terahertz modulator". United States. https://doi.org/10.1038/s41598-017-13701-9. https://www.osti.gov/servlets/purl/1402632.
@article{osti_1402632,
title = {Topological-insulator-based terahertz modulator},
author = {Wang, X. B. and Cheng, L. and Wu, Y. and Zhu, D. P. and Wang, L. and Zhu, Jian-Xin and Yang, Hyunsoo and Chia, Elbert E. M.},
abstractNote = {Three dimensional topological insulators, as a new phase of quantum matters, are characterized by an insulating gap in the bulk and a metallic state on the surface. Particularly, most of the topological insulators have narrow band gaps, and hence have promising applications in the area of terahertz optoelectronics. In this work, we experimentally demonstrate an electronically-tunable terahertz intensity modulator based on Bi1:5Sb0:5Te1:8Se1:2 single crystal, one of the most insulating topological insulators. A relative frequency-independent modulation depth of ~62% over a wide frequency range from 0.3 to 1.4 THz has been achieved at room temperature, by applying a bias current of 100 mA. The modulation in the low current regime can be further enhanced at low temperature. We propose that the extraordinarily large modulation is a consequence of thermally-activated carrier absorption in the semiconducting bulk states. Our work provides a new application of topological insulators for terahertz technology.},
doi = {10.1038/s41598-017-13701-9},
journal = {Scientific Reports},
number = 1,
volume = 7,
place = {United States},
year = {Wed Oct 18 00:00:00 EDT 2017},
month = {Wed Oct 18 00:00:00 EDT 2017}
}

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Works referenced in this record:

Topological insulators and thermoelectric materials
text, January 2012


Graphene terahertz modulators by ionic liquid gating
preprint, January 2015


Observation of Dirac Holes and Electrons in a Topological Insulator
journal, June 2011


Room-temperature operation of an electrically driven terahertz modulator
journal, May 2004

  • Kleine-Ostmann, T.; Dawson, P.; Pierz, K.
  • Applied Physics Letters, Vol. 84, Issue 18
  • DOI: 10.1063/1.1723689

Graphene Terahertz Modulators by Ionic Liquid Gating
journal, February 2015

  • Wu, Yang; La-o-vorakiat, Chan; Qiu, Xuepeng
  • Advanced Materials, Vol. 27, Issue 11
  • DOI: 10.1002/adma.201405251

Switchable Scattering Meta-Surfaces for Broadband Terahertz Modulation
journal, July 2014

  • Unlu, M.; Hashemi, M. R.; Berry, C. W.
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep05708

Active terahertz metamaterial devices
journal, November 2006

  • Chen, Hou-Tong; Padilla, Willie J.; Zide, Joshua M. O.
  • Nature, Vol. 444, Issue 7119, p. 597-600
  • DOI: 10.1038/nature05343

Direct intensity modulation and wireless data transmission characteristics of terahertz-oscillating resonant tunnelling diodes
journal, January 2012

  • Ishigaki, K.; Shiraishi, M.; Suzuki, S.
  • Electronics Letters, Vol. 48, Issue 10
  • DOI: 10.1049/el.2012.0849

Phonon features in terahertz photoconductivity spectra due to data analysis artifact: A case study on organometallic halide perovskites
journal, March 2017

  • La-o-vorakiat, Chan; Cheng, Liang; Salim, Teddy
  • Applied Physics Letters, Vol. 110, Issue 12
  • DOI: 10.1063/1.4978688

An electrically tunable terahertz metamaterial modulator with two independent channels
journal, March 2016

  • Bai, Yang; Chen, Kejian; Bu, Ting
  • Journal of Applied Physics, Vol. 119, Issue 12
  • DOI: 10.1063/1.4944711

Phonon features in terahertz photoconductivity spectra due to data analysis artifact: A case study on organometallic halide perovskites
journal, March 2017

  • La-o-vorakiat, Chan; Cheng, Liang; Salim, Teddy
  • Applied Physics Letters, Vol. 110, Issue 12
  • DOI: 10.1063/1.4978688

Graphene Terahertz Modulators by Ionic Liquid Gating
journal, February 2015

  • Wu, Yang; La-o-vorakiat, Chan; Qiu, Xuepeng
  • Advanced Materials, Vol. 27, Issue 11
  • DOI: 10.1002/adma.201405251

Room-temperature operation of an electrically driven terahertz modulator
journal, May 2004

  • Kleine-Ostmann, T.; Dawson, P.; Pierz, K.
  • Applied Physics Letters, Vol. 84, Issue 18
  • DOI: 10.1063/1.1723689

Evaluation of image quality in terahertz pulsed imaging using test objects
journal, October 2002


Strong nonlinear terahertz response induced by Dirac surface states in Bi2Se3 topological insulator
journal, April 2016

  • Giorgianni, Flavio; Chiadroni, Enrica; Rovere, Andrea
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms11421

Experimental Realization of a Three-Dimensional Topological Insulator, Bi2Te3
journal, June 2009


Double-Layer Graphene Optical Modulator
journal, February 2012

  • Liu, Ming; Yin, Xiaobo; Zhang, Xiang
  • Nano Letters, Vol. 12, Issue 3
  • DOI: 10.1021/nl204202k

A tunable topological insulator in the spin helical Dirac transport regime
text, January 2009


Active Terahertz Nanoantennas Based on VO 2 Phase Transition
journal, June 2010

  • Seo, Minah; Kyoung, Jisoo; Park, Hyeongryeol
  • Nano Letters, Vol. 10, Issue 6
  • DOI: 10.1021/nl1002153

Spintronics and Pseudospintronics in Graphene and Topological Insulators
text, January 2013


Memory Metamaterials
journal, August 2009


A graphene-based broadband optical modulator
journal, May 2011

  • Liu, Ming; Yin, Xiaobo; Ulin-Avila, Erick
  • Nature, Vol. 474, Issue 7349
  • DOI: 10.1038/nature10067

Cutting-edge terahertz technology
journal, February 2007


Broadband graphene terahertz modulators enabled by intraband transitions
journal, January 2012

  • Sensale-Rodriguez, Berardi; Yan, Rusen; Kelly, Michelle M.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1787

Thermal conductivity of Kapton tape
journal, January 1999


A tunable topological insulator in the spin helical Dirac transport regime
journal, July 2009


THz Wave Modulators: A Brief Review on Different Modulation Techniques
journal, November 2012

  • Rahm, Marco; Li, Jiu-Sheng; Padilla, Willie J.
  • Journal of Infrared, Millimeter, and Terahertz Waves, Vol. 34, Issue 1
  • DOI: 10.1007/s10762-012-9946-2

Superconductivity-Induced Transparency in Terahertz Metamaterials
journal, June 2014

  • Limaj, Odeta; Giorgianni, Flavio; Di Gaspare, Alessandra
  • ACS Photonics, Vol. 1, Issue 7
  • DOI: 10.1021/ph500104k

Electrical control of terahertz nano antennas on VO_2 thin film
journal, January 2011

  • Jeong, Young-Gyun; Bernien, Hannes; Kyoung, Ji-Soo
  • Optics Express, Vol. 19, Issue 22
  • DOI: 10.1364/oe.19.021211

Strong nonlinear terahertz response induced by Dirac surface states in Bi2Se3 Topological Insulator
text, January 2018


Temperature dependent characterization of terahertz vibrations of explosives and related threat materials
journal, January 2010

  • Melinger, Joseph S.; Harsha, S. Sree; Laman, N.
  • Optics Express, Vol. 18, Issue 26
  • DOI: 10.1364/oe.18.027238

Topological insulators in Bi2Se3, Bi2Te3 and Sb2Te3 with a single Dirac cone on the surface
journal, May 2009

  • Zhang, Haijun; Liu, Chao-Xing; Qi, Xiao-Liang
  • Nature Physics, Vol. 5, Issue 6, p. 438-442
  • DOI: 10.1038/nphys1270

The birth of topological insulators
journal, March 2010


Materials for terahertz science and technology
journal, September 2002

  • Ferguson, Bradley; Zhang, Xi-Cheng
  • Nature Materials, Vol. 1, Issue 1
  • DOI: 10.1038/nmat708

The birth of topological insulators
journal, March 2010


Materials for terahertz science and technology
journal, September 2002

  • Ferguson, Bradley; Zhang, Xi-Cheng
  • Nature Materials, Vol. 1, Issue 1
  • DOI: 10.1038/nmat708

Mid-infrared photonics in silicon and germanium
journal, August 2010


A sudden collapse in the transport lifetime across the topological phase transition in (Bi1−xInx)2Se3
journal, June 2013

  • Wu, Liang; Brahlek, M.; Valdés Aguilar, R.
  • Nature Physics, Vol. 9, Issue 7
  • DOI: 10.1038/nphys2647

Mid-infrared photonics in silicon and germanium
journal, August 2010


Colloquium: Topological insulators
journal, November 2010


Observation of Time-Reversal-Protected Single-Dirac-Cone Topological-Insulator States in Bi 2 Te 3 and Sb 2 Te 3
journal, September 2009


Observation of a large-gap topological-insulator class with a single Dirac cone on the surface
journal, May 2009

  • Xia, Y.; Qian, D.; Hsieh, D.
  • Nature Physics, Vol. 5, Issue 6, p. 398-402
  • DOI: 10.1038/nphys1274

THz Wave Modulators: A Brief Review on Different Modulation Techniques
journal, November 2012

  • Rahm, Marco; Li, Jiu-Sheng; Padilla, Willie J.
  • Journal of Infrared, Millimeter, and Terahertz Waves, Vol. 34, Issue 1
  • DOI: 10.1007/s10762-012-9946-2

Active Terahertz Nanoantennas Based on VO 2 Phase Transition
journal, June 2010

  • Seo, Minah; Kyoung, Jisoo; Park, Hyeongryeol
  • Nano Letters, Vol. 10, Issue 6
  • DOI: 10.1021/nl1002153

Observation of Dirac Holes and Electrons in a Topological Insulator
text, January 2011


Topological insulators in Bi2Se3, Bi2Te3 and Sb2Te3 with a single Dirac cone on the surface
journal, May 2009

  • Zhang, Haijun; Liu, Chao-Xing; Qi, Xiao-Liang
  • Nature Physics, Vol. 5, Issue 6, p. 438-442
  • DOI: 10.1038/nphys1270

Spintronics and pseudospintronics in graphene and topological insulators
journal, April 2012

  • Pesin, Dmytro; MacDonald, Allan H.
  • Nature Materials, Vol. 11, Issue 5
  • DOI: 10.1038/nmat3305

Observation of Dirac Holes and Electrons in a Topological Insulator
text, January 2011


Terahertz conductivity of topological surface states in Bi1.5Sb0.5Te1.8Se1.2
journal, December 2013

  • Tang, Chi Sin; Xia, Bin; Zou, Xingquan
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep03513

Broadband graphene terahertz modulators enabled by intraband transitions
journal, January 2012

  • Sensale-Rodriguez, Berardi; Yan, Rusen; Kelly, Michelle M.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1787

Infrared probe of the bulk insulating response in Bi 2 x Sb x Te 3 y Se y topological insulator alloys
journal, April 2015


Memory Metamaterials
text, January 2010


Cutting-edge terahertz technology
journal, February 2007


Topological insulators and thermoelectric materials
journal, November 2012

  • Müchler, Lukas; Casper, Frederick; Yan, Binghai
  • physica status solidi (RRL) - Rapid Research Letters, Vol. 7, Issue 1-2
  • DOI: 10.1002/pssr.201206411

Direct intensity modulation and wireless data transmission characteristics of terahertz-oscillating resonant tunnelling diodes
journal, January 2012

  • Ishigaki, K.; Shiraishi, M.; Suzuki, S.
  • Electronics Letters, Vol. 48, Issue 10
  • DOI: 10.1049/el.2012.0849

An introduction to medical imaging with coherent terahertz frequency radiation
journal, March 2002


Active terahertz metamaterial devices
journal, November 2006

  • Chen, Hou-Tong; Padilla, Willie J.; Zide, Joshua M. O.
  • Nature, Vol. 444, Issue 7119, p. 597-600
  • DOI: 10.1038/nature05343

An introduction to medical imaging with coherent terahertz frequency radiation
journal, March 2002


Filling the THz gap—high power sources and applications
journal, December 2005


Switchable Scattering Meta-Surfaces for Broadband Terahertz Modulation
journal, July 2014

  • Unlu, M.; Hashemi, M. R.; Berry, C. W.
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep05708

An electrically tunable terahertz metamaterial modulator with two independent channels
journal, March 2016

  • Bai, Yang; Chen, Kejian; Bu, Ting
  • Journal of Applied Physics, Vol. 119, Issue 12
  • DOI: 10.1063/1.4944711

Tuning the Resonance in High-Temperature Superconducting Terahertz Metamaterials
journal, December 2010


Topological insulators and superconductors
journal, October 2011


Topological insulators for high-performance terahertz to infrared applications
journal, December 2010


p-type Bi2Se3 for topological insulator and low-temperature thermoelectric applications
journal, May 2009

  • Hor, Y. S.; Richardella, A.; Roushan, P.
  • Physical Review B, Vol. 79, Issue 19, Article No. 195208
  • DOI: 10.1103/PhysRevB.79.195208

Terahertz conductivity of topological surface states in Bi1.5Sb0.5Te1.8Se1.2
journal, December 2013

  • Tang, Chi Sin; Xia, Bin; Zou, Xingquan
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep03513

Works referencing / citing this record:

Dynamic Terahertz Plasmonics Enabled by Phase‐Change Materials
journal, August 2019

  • Jeong, Young‐Gyun; Bahk, Young‐Mi; Kim, Dai‐Sik
  • Advanced Optical Materials, Vol. 8, Issue 3
  • DOI: 10.1002/adom.201900548

Design, Fabrication, and Modulation of THz Bandpass Metamaterials
journal, October 2019

  • Wang, Qinghua; Gao, Bingtao; Raglione, Michaella
  • Laser & Photonics Reviews, Vol. 13, Issue 11
  • DOI: 10.1002/lpor.201900071

Device Applications of Synthetic Topological Insulator Nanostructures
journal, October 2018