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Title: Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells

Abstract

Here, we have investigated semi-transparent perovskite solar cells and infrared enhanced silicon heterojunction cells for high-efficiency tandem devices. A semi-transparent metal electrode with good electrical conductivity and optical transparency has been fabricated by thermal evaporation of 7 nm of Au onto a 1-nm-thick Cu seed layer. For this electrode to reach its full potential, MAPbI3 thin films were formed by a modified one-step spin-coating method, resulting in a smooth layer that allowed the subsequent metal thin film to remain continuous. The fabricated semi-transparent perovskite solar cells demonstrated 16.5% efficiency under one-sun illumination, and were coupled with infrared-enhanced silicon heterojunction cells tuned specifically for perovskite/Si tandem devices. A double-layer antireflection coating at the front side and MgF2 reflector at rear side of the silicon heterojunction cells reduced parasitic absorption of near-infrared light, leading to 6.5% efficiency after filtering with a perovskite device and 23.0% summed efficiency for the perovskite/Si tandem device.

Authors:
 [1];  [1];  [2];  [1];  [1];  [1];  [1];  [2];  [1];  [2];  [1]
  1. Univ. of Nebraska-Lincoln, Lincoln, NE (United States)
  2. Arizona State Univ., Tempe, AZ (United States)
Publication Date:
Research Org.:
Univ. of Nebraska, Lincoln, NE (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office
OSTI Identifier:
1342622
Alternate Identifier(s):
OSTI ID: 1400993
Grant/Contract Number:  
EE0006709; EE0006335; DE‐EE0006709
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Energy Materials
Additional Journal Information:
Journal Volume: 6; Journal Issue: 19; Journal ID: ISSN 1614-6832
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 25 ENERGY STORAGE; semi-transparent; metal electrode; perovskite solar cell; silicon solar cell; tandem

Citation Formats

Chen, Bo, Bai, Yang, Yu, Zhengshan, Li, Tao, Zheng, Xiaopeng, Dong, Qingfeng, Shen, Liang, Boccard, Mathieu, Gruverman, Alexei, Holman, Zachary, and Huang, Jinsong. Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells. United States: N. p., 2016. Web. doi:10.1002/aenm.201601128.
Chen, Bo, Bai, Yang, Yu, Zhengshan, Li, Tao, Zheng, Xiaopeng, Dong, Qingfeng, Shen, Liang, Boccard, Mathieu, Gruverman, Alexei, Holman, Zachary, & Huang, Jinsong. Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells. United States. https://doi.org/10.1002/aenm.201601128
Chen, Bo, Bai, Yang, Yu, Zhengshan, Li, Tao, Zheng, Xiaopeng, Dong, Qingfeng, Shen, Liang, Boccard, Mathieu, Gruverman, Alexei, Holman, Zachary, and Huang, Jinsong. Tue . "Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells". United States. https://doi.org/10.1002/aenm.201601128. https://www.osti.gov/servlets/purl/1342622.
@article{osti_1342622,
title = {Efficient semitransparent perovskite solar cells for 23.0%-efficiency perovskite/silicon four-terminal tandem cells},
author = {Chen, Bo and Bai, Yang and Yu, Zhengshan and Li, Tao and Zheng, Xiaopeng and Dong, Qingfeng and Shen, Liang and Boccard, Mathieu and Gruverman, Alexei and Holman, Zachary and Huang, Jinsong},
abstractNote = {Here, we have investigated semi-transparent perovskite solar cells and infrared enhanced silicon heterojunction cells for high-efficiency tandem devices. A semi-transparent metal electrode with good electrical conductivity and optical transparency has been fabricated by thermal evaporation of 7 nm of Au onto a 1-nm-thick Cu seed layer. For this electrode to reach its full potential, MAPbI3 thin films were formed by a modified one-step spin-coating method, resulting in a smooth layer that allowed the subsequent metal thin film to remain continuous. The fabricated semi-transparent perovskite solar cells demonstrated 16.5% efficiency under one-sun illumination, and were coupled with infrared-enhanced silicon heterojunction cells tuned specifically for perovskite/Si tandem devices. A double-layer antireflection coating at the front side and MgF2 reflector at rear side of the silicon heterojunction cells reduced parasitic absorption of near-infrared light, leading to 6.5% efficiency after filtering with a perovskite device and 23.0% summed efficiency for the perovskite/Si tandem device.},
doi = {10.1002/aenm.201601128},
journal = {Advanced Energy Materials},
number = 19,
volume = 6,
place = {United States},
year = {Tue Jul 19 00:00:00 EDT 2016},
month = {Tue Jul 19 00:00:00 EDT 2016}
}

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Surface Chlorination of ZnO for Perovskite Solar Cells with Enhanced Efficiency and Stability
journal, May 2019


Interface Molecular Engineering for Laminated Monolithic Perovskite/Silicon Tandem Solar Cells with 80.4% Fill Factor
journal, August 2019

  • Ramírez Quiroz, César Omar; Spyropoulos, George D.; Salvador, Michael
  • Advanced Functional Materials, Vol. 29, Issue 40
  • DOI: 10.1002/adfm.201901476

Solution‐Processed Laminated Perovskite Layers for High‐Performance Solar Cells
journal, September 2019

  • Wang, Yangyang; Li, Tianhao; Li, Zengrong
  • Advanced Functional Materials, Vol. 29, Issue 45
  • DOI: 10.1002/adfm.201903330

Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering
journal, June 2018

  • Rajagopal, Adharsh; Yao, Kai; Jen, Alex K. -Y.
  • Advanced Materials, Vol. 30, Issue 32
  • DOI: 10.1002/adma.201800455

Nonprecious Copper‐Based Transparent Top Electrode via Seed Layer–Assisted Thermal Evaporation for High‐Performance Semitransparent n‐i‐p Perovskite Solar Cells
journal, February 2019

  • Giuliano, Giuliana; Cataldo, Sebastiano; Scopelliti, Michelangelo
  • Advanced Materials Technologies, Vol. 4, Issue 5
  • DOI: 10.1002/admt.201800688

Perovskite—a Perfect Top Cell for Tandem Devices to Break the S–Q Limit
journal, January 2019


Flexible and Semitransparent Organic Solar Cells
journal, November 2017

  • Li, Yaowen; Xu, Guiying; Cui, Chaohua
  • Advanced Energy Materials, Vol. 8, Issue 7
  • DOI: 10.1002/aenm.201701791

Emerging Novel Metal Electrodes for Photovoltaic Applications
journal, January 2018


Recent Advances in Controlled Synthesis of Upconversion Nanoparticles and Semiconductor Heterostructures
journal, April 2019

  • Wang, Wanni; Zhao, Mengli; Zhang, Chenyang
  • The Chemical Record, Vol. 20, Issue 1
  • DOI: 10.1002/tcr.201900006

High-efficiency inverted semi-transparent planar perovskite solar cells in substrate configuration
journal, December 2016


Interface engineering of CsPbI 3 -black phosphorus van der Waals heterostructure
journal, January 2018

  • Liu, Biao; Long, Mengqiu; Cai, Meng-Qiu
  • Applied Physics Letters, Vol. 112, Issue 4
  • DOI: 10.1063/1.5016868

Triple-halide wide–band gap perovskites with suppressed phase segregation for efficient tandems
journal, March 2020


Self-Filtered Narrowband Perovskite Photodetectors with Ultrafast and Tuned Spectral Response
text, January 2017

  • S., Tang,; H., Wei,; Y., Fang,
  • The University of North Carolina at Chapel Hill University Libraries
  • DOI: 10.17615/0cct-yg83

Fully Solution‐Processed Semi‐Transparent Perovskite Solar Cells With Ink‐Jet Printed Silver Nanowires Top Electrode
journal, January 2018


Nanoscale Back Contact Perovskite Solar Cell Design for Improved Tandem Efficiency
journal, August 2017


Electrical analysis of c-Si/CGSe monolithic tandem solar cells by using a cell-selective light absorption scheme
journal, November 2017