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Title: Deterministic Placement of Quantum-Size Controlled Quantum Dots for Seamless Top-Down Integration

We demonstrate a new route toward the integration and deterministic placement of quantum dots (QDs) within prepatterned nanostructures. Using standard electron-beam lithography (EBL) and inductively coupled plasma reactive-ion etching (ICP-RIE), we fabricate arrays of nanowires on a III-nitride platform. Next, we integrate QDs of controlled size within the prepatterned nanowires using a bandgap-selective, wet-etching technique: quantum-size-controlled photoelectrochemical (QSC-PEC) etching. Low-temperature microphotoluminescence (μ-PL) measurements of individual nanowires reveal sharp spectral signatures, indicative of QD formation. Further, internal quantum efficiency (IQE) measurements reveal a near order of magnitude improvement in emitter efficiency following QSC-PEC etching. Finally, second-order cross-correlation (g(2)(0)) measurements of individual QDs directly confirm nonclassical, antibunching behavior. Lastly, our results illustrate an exciting approach toward the top-down integration of nonclassical light sources within nanophotonic platforms.
Authors:
 [1] ;  [2] ;  [1] ; ORCiD logo [3]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Univ. of Southern California, Los Angeles, CA (United States). Ming Hsieh Dept. of Electrical Engineering
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Univ. of New Mexico, Albuquerque, NM (United States). Dept. of Electrical and Computer Engineering
Publication Date:
Report Number(s):
SAND-2017-10106J
Journal ID: ISSN 2330-4022; 657140
Grant/Contract Number:
AC04-94AL85000; NA0003525
Type:
Accepted Manuscript
Journal Name:
ACS Photonics
Additional Journal Information:
Journal Volume: 4; Journal Issue: 9; Journal ID: ISSN 2330-4022
Publisher:
American Chemical Society (ACS)
Research Org:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org:
USDOE National Nuclear Security Administration (NNSA)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; antibunched; InGaN; nanophotonics; photoelectrochemical etching; photoluminescence; quantum dots
OSTI Identifier:
1398784

Fischer, Arthur J., Anderson, P. Duke, Koleske, Daniel D., and Subramania, Ganapathi. Deterministic Placement of Quantum-Size Controlled Quantum Dots for Seamless Top-Down Integration. United States: N. p., Web. doi:10.1021/acsphotonics.7b00774.
Fischer, Arthur J., Anderson, P. Duke, Koleske, Daniel D., & Subramania, Ganapathi. Deterministic Placement of Quantum-Size Controlled Quantum Dots for Seamless Top-Down Integration. United States. doi:10.1021/acsphotonics.7b00774.
Fischer, Arthur J., Anderson, P. Duke, Koleske, Daniel D., and Subramania, Ganapathi. 2017. "Deterministic Placement of Quantum-Size Controlled Quantum Dots for Seamless Top-Down Integration". United States. doi:10.1021/acsphotonics.7b00774. https://www.osti.gov/servlets/purl/1398784.
@article{osti_1398784,
title = {Deterministic Placement of Quantum-Size Controlled Quantum Dots for Seamless Top-Down Integration},
author = {Fischer, Arthur J. and Anderson, P. Duke and Koleske, Daniel D. and Subramania, Ganapathi},
abstractNote = {We demonstrate a new route toward the integration and deterministic placement of quantum dots (QDs) within prepatterned nanostructures. Using standard electron-beam lithography (EBL) and inductively coupled plasma reactive-ion etching (ICP-RIE), we fabricate arrays of nanowires on a III-nitride platform. Next, we integrate QDs of controlled size within the prepatterned nanowires using a bandgap-selective, wet-etching technique: quantum-size-controlled photoelectrochemical (QSC-PEC) etching. Low-temperature microphotoluminescence (μ-PL) measurements of individual nanowires reveal sharp spectral signatures, indicative of QD formation. Further, internal quantum efficiency (IQE) measurements reveal a near order of magnitude improvement in emitter efficiency following QSC-PEC etching. Finally, second-order cross-correlation (g(2)(0)) measurements of individual QDs directly confirm nonclassical, antibunching behavior. Lastly, our results illustrate an exciting approach toward the top-down integration of nonclassical light sources within nanophotonic platforms.},
doi = {10.1021/acsphotonics.7b00774},
journal = {ACS Photonics},
number = 9,
volume = 4,
place = {United States},
year = {2017},
month = {8}
}