Unfolding the physics of URu2Si2 through silicon to phosphorus substitution

Gallagher, A.; Chen, K. -W.; Moir, C. M.; Cary, S. K.; Kametani, F.; Kikugawa, N.; Graf, D.; Albrecht-Schmitt, T. E.; Riggs, S. C.; Shekhter, A.; Baumbach, R. E.

doi:10.1038/ncomms10712

Title: Unfolding the physics of URu₂Si₂ through silicon to phosphorus substitution

Abstract

The heavy fermion intermetallic compound URu₂Si₂ exhibits a hidden-order phase below the temperature of 17.5 K, which supports both anomalous metallic behavior and unconventional superconductivity. While these individual phenomena have been investigated in detail, it remains unclear how they are related to each other and to what extent uranium f-electron valence fluctuations influence each one. Here we use ligand site substituted URu₂Si_2-xP_x to establish their evolution under electronic tuning. We find that while hidden order is monotonically suppressed and destroyed for x ≤ 0.035, the superconducting strength evolves non-monotonically with a maximum near x ≈ 0.01 and that superconductivity is destroyed near x ≈ 0.028. This behavior reveals that hidden order depends strongly on tuning outside of the U f-electron shells. Furthermore, it also suggests that while hidden order provides an environment for superconductivity and anomalous metallic behavior, it’s fluctuations may not be solely responsible for their progression.

Authors:

Gallagher, A. ^[1]; Chen, K. -W. ^[1]; Moir, C. M. ^[1]; Cary, S. K. ^[1]; Kametani, F. ^[1]; Kikugawa, N. ^[2]; Graf, D. ^[1]; Albrecht-Schmitt, T. E. ^[1]; Riggs, S. C. ^[1];

^[1]; Baumbach, R. E. ^[1]

Florida State Univ., Tallahassee, FL (United States)
Florida State Univ., Tallahassee, FL (United States); National Institute for Materials Science 3-13 Sakura, Tsukuba (Japan)

Publication Date:: Fri Feb 19 00:00:00 EST 2016

Research Org.:: Florida State Univ., Tallahassee, FL (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1395565

Grant/Contract Number:: FG02-13ER16414; SC0010677

Resource Type:: Accepted Manuscript

Journal Name:: Nature Communications

Additional Journal Information:: Journal Volume: 7; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Gallagher, A., Chen, K. -W., Moir, C. M., Cary, S. K., Kametani, F., Kikugawa, N., Graf, D., Albrecht-Schmitt, T. E., Riggs, S. C., Shekhter, A., and Baumbach, R. E. Unfolding the physics of URu2Si2 through silicon to phosphorus substitution.  United States: N. p., 2016. 
Web.  doi:10.1038/ncomms10712.

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                    Gallagher, A., Chen, K. -W., Moir, C. M., Cary, S. K., Kametani, F., Kikugawa, N., Graf, D., Albrecht-Schmitt, T. E., Riggs, S. C., Shekhter, A., & Baumbach, R. E. Unfolding the physics of URu2Si2 through silicon to phosphorus substitution.  United States.  https://doi.org/10.1038/ncomms10712

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                    Gallagher, A., Chen, K. -W., Moir, C. M., Cary, S. K., Kametani, F., Kikugawa, N., Graf, D., Albrecht-Schmitt, T. E., Riggs, S. C., Shekhter, A., and Baumbach, R. E. Fri .  
"Unfolding the physics of URu2Si2 through silicon to phosphorus substitution".  United States.  https://doi.org/10.1038/ncomms10712.  https://www.osti.gov/servlets/purl/1395565.

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@article{osti_1395565,

  title        = {Unfolding the physics of URu2Si2 through silicon to phosphorus substitution},

  author       = {Gallagher, A. and Chen, K. -W. and Moir, C. M. and Cary, S. K. and Kametani, F. and Kikugawa, N. and Graf, D. and Albrecht-Schmitt, T. E. and Riggs, S. C. and Shekhter, A. and Baumbach, R. E.},

  abstractNote = {The heavy fermion intermetallic compound URu2Si2 exhibits a hidden-order phase below the temperature of 17.5 K, which supports both anomalous metallic behavior and unconventional superconductivity. While these individual phenomena have been investigated in detail, it remains unclear how they are related to each other and to what extent uranium f-electron valence fluctuations influence each one. Here we use ligand site substituted URu2Si2-xPx to establish their evolution under electronic tuning. We find that while hidden order is monotonically suppressed and destroyed for x ≤ 0.035, the superconducting strength evolves non-monotonically with a maximum near x ≈ 0.01 and that superconductivity is destroyed near x ≈ 0.028. This behavior reveals that hidden order depends strongly on tuning outside of the U f-electron shells. Furthermore, it also suggests that while hidden order provides an environment for superconductivity and anomalous metallic behavior, it’s fluctuations may not be solely responsible for their progression.},

  doi          = {10.1038/ncomms10712},

  journal      = {Nature Communications},

  number       = ,

  volume       = 7,

  place        = {United States},

  year         = {Fri Feb 19 00:00:00 EST 2016},

  month        = {Fri Feb 19 00:00:00 EST 2016}

}

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Title: Unfolding the physics of URu2Si2 through silicon to phosphorus substitution

Abstract

Citation Formats

Chemical pressure tuning of URu 2 Si 2 via isoelectronic substitution of Ru with Fe journal, February 2015

Hastatic order in the heavy-fermion compound URu2Si2 journal, January 2013

Hybridization-driven orthorhombic lattice instability in URu 2 Si 2 journal, November 2013

Non-Fermi-Liquid Behavior within the Ferromagnetic Phase in U R u 2 − x R e x S i 2 journal, February 2005

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

From quantum matter to high-temperature superconductivity in copper oxides journal, February 2015

Superconducting phases of f -electron compounds journal, November 2009

Fermi-liquid instabilities at magnetic quantum phase transitions journal, August 2007

Nature of the 5 f states in actinide metals journal, February 2009

Spectroscopic Determination of the Atomic f -Electron Symmetry Underlying Hidden Order in URu 2 Si 2 journal, June 2015

Quasiparticle Mass Enhancement Close to the Quantum Critical Point in BaFe 2 ( As 1 − x P x ) 2 journal, June 2013

Effect of pressure on competing electronic correlations in the heavy-electron system URu 2 Si 2 journal, January 1987

The evolution of the ordered states of single-crystal URu 2 Si 2 under pressure journal, February 2008

The State of d Electrons in Transition Metals journal, May 1960

High purity specimens of URu 2 Si 2 produced by a molten metal flux technique journal, April 2014

Effect of transition-metal substitutions on competing electronic transitions in the heavy-electron compound URu 2 Si 2 journal, February 1990

Superconducting and Magnetic Transitions in the Heavy-Fermion System U Ru 2 Si 2 journal, December 1985

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of URu 2 Si 2 journal, November 2010

Evidence for broken time-reversal symmetry in the superconducting phase of URu 2 Si 2 journal, April 2015

Enhancement of the hidden order/large moment antiferromagnetic transition temperature in the URu 2− x Os x Si 2 system journal, April 2014

Ferromagnetic instability in the heavy-electron compound URu 2 Si 2 doped with Re or Tc journal, February 1989

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Zur magnetischen Widerstandsänderung reiner Metalle journal, January 1938

The suppression of hidden order and the onset of ferromagnetism in URu 2 Si 2 via Re substitution journal, March 2010

Chirality density wave of the "hidden order" phase in URu2Si2 journal, February 2015

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 journal, January 2011

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu 2 − x Fe x Si 2 system journal, December 2011

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements journal, March 2015

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 journal, June 2014

Specific heat and susceptibility of U(Ru1−xRhx)2Si2 journal, December 1988

Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu 2 Si 2 journal, December 1999

A new heavy-fermion superconductor CeIrIn 5 : A relative of the cuprates? journal, February 2001

The doping dependence of T* – what is the real high-Tc phase diagram? journal, January 2001

3 Recent advances in the electron theory of metals journal, January 1952

The Kondo Problem to Heavy Fermions book, January 1993

Zur magnetischen Widerstandsänderung reiner Metalle journal, January 1938

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2 journal, June 1986

From quantum matter to high-temperature superconductivity in copper oxides journal, February 2015

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 journal, June 2014

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements journal, March 2015

The State of d Electrons in Transition Metals journal, May 1960

The suppression of hidden order and the onset of ferromagnetism in URu 2 Si 2 via Re substitution journal, March 2010

Superconducting Pairs with Extreme Uniaxial Anisotropy in URu 2 Si 2 journal, February 2012

Colloquium: Hidden Order, Superconductivity, and Magnetism -- The Unsolved Case of URu2Si2 text, January 2011

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 text, January 2011

Highly Sensitive Detection of Ionizing Radiations by a Photoluminescent Uranyl Organic Framework journal, May 2017

Rapid suppression of the energy gap and the possibility of a gapless hidden order state in URu 2− x Re x Si 2 journal, April 2019

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu 2 Si 2 journal, January 2020

NMR investigation of antiferromagnetism and coherence in URu 2 Si 2 − x P x journal, January 2017

Pressure-induced rotational symmetry breaking in URu 2 Si 2 journal, December 2018

Instability of the f -electron state in URu 2 Si 2 − x P x probed using high magnetic fields journal, June 2019

Single Crystal Growth of URu2Si2 by the Modified Bridgman Technique journal, October 2016

Pressure-induced rotational symmetry breaking in URu2Si2 text, January 2018

Highly Sensitive Detection of Ionizing Radiations by a Photoluminescent Uranyl Organic Framework journal, May 2017

Title: Unfolding the physics of URu₂Si₂ through silicon to phosphorus substitution

Chemical pressure tuning of ${URu}_{2} {Si}_{2}$ via isoelectronic substitution of Ru with Fe
journal, February 2015

Hastatic order in the heavy-fermion compound URu2Si2
journal, January 2013

Hybridization-driven orthorhombic lattice instability in URu $_{2}$ Si $_{2}$
journal, November 2013

Non-Fermi-Liquid Behavior within the Ferromagnetic Phase in ${U R u}_{2 - x} {R e}_{x} {S i}_{2}$
journal, February 2005

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

Superconducting phases of $f$ -electron compounds
journal, November 2009

Fermi-liquid instabilities at magnetic quantum phase transitions
journal, August 2007

Nature of the $5 f$ states in actinide metals
journal, February 2009

Spectroscopic Determination of the Atomic $f$ -Electron Symmetry Underlying Hidden Order in ${URu}_{2} {Si}_{2}$
journal, June 2015

Quasiparticle Mass Enhancement Close to the Quantum Critical Point in ${BaFe}_{2} ({As}_{1 - x} P_{x})_{2}$
journal, June 2013

Effect of pressure on competing electronic correlations in the heavy-electron system ${URu}_{2}$ ${Si}_{2}$
journal, January 1987

The evolution of the ordered states of single-crystal URu ₂ Si ₂ under pressure
journal, February 2008

The State of d Electrons in Transition Metals
journal, May 1960

High purity specimens of URu ₂ Si ₂ produced by a molten metal flux technique
journal, April 2014

Effect of transition-metal substitutions on competing electronic transitions in the heavy-electron compound ${URu}_{2}$ ${Si}_{2}$
journal, February 1990

Superconducting and Magnetic Transitions in the Heavy-Fermion System U ${Ru}_{2}$ ${Si}_{2}$
journal, December 1985

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of ${URu}_{2} {Si}_{2}$
journal, November 2010

Evidence for broken time-reversal symmetry in the superconducting phase of ${URu}_{2} {Si}_{2}$
journal, April 2015

Enhancement of the hidden order/large moment antiferromagnetic transition temperature in the URu _{2− x} Os _x Si ₂ system
journal, April 2014

Ferromagnetic instability in the heavy-electron compound ${URu}_{2}$ ${Si}_{2}$ doped with Re or Tc
journal, February 1989

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Zur magnetischen Widerstandsänderung reiner Metalle
journal, January 1938

The suppression of hidden order and the onset of ferromagnetism in URu ₂ Si ₂ via Re substitution
journal, March 2010

Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu $_{2 - x}$ Fe $_{x}$ Si $_{2}$ system
journal, December 2011

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements
journal, March 2015

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

Specific heat and susceptibility of U(Ru1−xRhx)2Si2
journal, December 1988

Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound ${URu}_{2} {Si}_{2}$
journal, December 1999

A new heavy-fermion superconductor CeIrIn ₅ : A relative of the cuprates?
journal, February 2001

The doping dependence of T* – what is the real high-Tc phase diagram?
journal, January 2001

3 Recent advances in the electron theory of metals
journal, January 1952

The Kondo Problem to Heavy Fermions
book, January 1993

Zur magnetischen Widerstandsänderung reiner Metalle
journal, January 1938

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2
journal, June 1986

From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements
journal, March 2015

The State of d Electrons in Transition Metals
journal, May 1960

The suppression of hidden order and the onset of ferromagnetism in URu ₂ Si ₂ via Re substitution
journal, March 2010

Superconducting Pairs with Extreme Uniaxial Anisotropy in ${URu}_{2} {Si}_{2}$
journal, February 2012

Colloquium: Hidden Order, Superconductivity, and Magnetism -- The Unsolved Case of URu2Si2
text, January 2011

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
text, January 2011

Highly Sensitive Detection of Ionizing Radiations by a Photoluminescent Uranyl Organic Framework
journal, May 2017

Rapid suppression of the energy gap and the possibility of a gapless hidden order state in URu _{2− x} Re _x Si ₂
journal, April 2019

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020

NMR investigation of antiferromagnetism and coherence in ${URu}_{2} {Si}_{2 - x} P_{x}$
journal, January 2017

Pressure-induced rotational symmetry breaking in ${URu}_{2} {Si}_{2}$
journal, December 2018

Instability of the f -electron state in URu 2 Si 2 − x P x probed using high magnetic fields
journal, June 2019

Single Crystal Growth of URu2Si2 by the Modified Bridgman Technique
journal, October 2016

Pressure-induced rotational symmetry breaking in URu2Si2
text, January 2018

Highly Sensitive Detection of Ionizing Radiations by a Photoluminescent Uranyl Organic Framework
journal, May 2017