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Title: Electrochemical performance of MXenes as K-ion battery anodes

In this paper, we report on the electrochemical performance of two-dimensional transition metal carbonitrides as novel promising electrode materials in K-ion batteries. Titanium carbonitride, Ti 3CNT z, was investigated in detail using electrochemical galvanostatic cycling at various current densities. Finally, X-ray diffraction and X-ray photoelectron spectroscopy were used to study the potassiation mechanism and its structural changes.
Authors:
ORCiD logo [1] ;  [2] ;  [2] ;  [2] ;  [2] ;  [1] ; ORCiD logo [2]
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  2. Purdue Univ., West Lafayette, IN (United States)
Publication Date:
Grant/Contract Number:
AC05-00OR22725
Type:
Accepted Manuscript
Journal Name:
ChemComm
Additional Journal Information:
Journal Volume: 53; Journal Issue: 51; Journal ID: ISSN 1359-7345
Publisher:
Royal Society of Chemistry
Research Org:
Purdue Univ., West Lafayette, IN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org:
USDOE; ORNL Laboratory Directed Research and Development (LDRD) Program
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE
OSTI Identifier:
1394414

Naguib, Michael, Adams, Ryan A., Zhao, Yunpu, Zemlyanov, Dmitry, Varma, Arvind, Nanda, Jagjit, and Pol, Vilas G.. Electrochemical performance of MXenes as K-ion battery anodes. United States: N. p., Web. doi:10.1039/C7CC02026K.
Naguib, Michael, Adams, Ryan A., Zhao, Yunpu, Zemlyanov, Dmitry, Varma, Arvind, Nanda, Jagjit, & Pol, Vilas G.. Electrochemical performance of MXenes as K-ion battery anodes. United States. doi:10.1039/C7CC02026K.
Naguib, Michael, Adams, Ryan A., Zhao, Yunpu, Zemlyanov, Dmitry, Varma, Arvind, Nanda, Jagjit, and Pol, Vilas G.. 2017. "Electrochemical performance of MXenes as K-ion battery anodes". United States. doi:10.1039/C7CC02026K. https://www.osti.gov/servlets/purl/1394414.
@article{osti_1394414,
title = {Electrochemical performance of MXenes as K-ion battery anodes},
author = {Naguib, Michael and Adams, Ryan A. and Zhao, Yunpu and Zemlyanov, Dmitry and Varma, Arvind and Nanda, Jagjit and Pol, Vilas G.},
abstractNote = {In this paper, we report on the electrochemical performance of two-dimensional transition metal carbonitrides as novel promising electrode materials in K-ion batteries. Titanium carbonitride, Ti3CNTz, was investigated in detail using electrochemical galvanostatic cycling at various current densities. Finally, X-ray diffraction and X-ray photoelectron spectroscopy were used to study the potassiation mechanism and its structural changes.},
doi = {10.1039/C7CC02026K},
journal = {ChemComm},
number = 51,
volume = 53,
place = {United States},
year = {2017},
month = {5}
}

Works referenced in this record:

Two-Dimensional Nanocrystals Produced by Exfoliation of Ti3AlC2
journal, August 2011
  • Naguib, Michael; Kurtoglu, Murat; Presser, Volker
  • Advanced Materials, Vol. 23, Issue 37, p. 4248-4253
  • DOI: 10.1002/adma.201102306

25th Anniversary Article: MXenes: A New Family of Two-Dimensional Materials
journal, December 2013
  • Naguib, Michael; Mochalin, Vadym N.; Barsoum, Michel W.
  • Advanced Materials, Vol. 26, Issue 7, p. 992-1005
  • DOI: 10.1002/adma.201304138

Adsorption of Gases in Multimolecular Layers
journal, February 1938
  • Brunauer, Stephen; Emmett, P. H.; Teller, Edward
  • Journal of the American Chemical Society, Vol. 60, Issue 2, p. 309-319
  • DOI: 10.1021/ja01269a023

MXene: a promising transition metal carbide anode for lithium-ion batteries
journal, March 2012
  • Naguib, Michael; Come, Jérémy; Dyatkin, Boris
  • Electrochemistry Communications, Vol. 16, Issue 1, p. 61-64
  • DOI: 10.1016/j.elecom.2012.01.002