Conformal Nitrogen-Doped TiO2 Photocatalytic Coatings for Sunlight-Activated Membranes
Abstract
Photocatalytic degradation of organic contaminants is enticing for addressing challenging, nontraditional water sources. A novel nitrogen-doping method is utilized to grow conformal titania coatings with visible-light activity on porous membranes. Here, the resulting membranes exhibit effective degradation of model organic species in simulated sunlight while at the same time requiring substantially lower transmembrane pressure than undoped membranes.
- Authors:
-
- Argonne National Lab. (ANL), Lemont, IL (United States)
- Univ. of Chicago, Chicago, IL (United States)
- Argonne National Lab. (ANL), Lemont, IL (United States); California State Univ. - Long Beach, Long Beach, CA (United States)
- Argonne National Lab. (ANL), Lemont, IL (United States); Univ. of Chicago, Chicago, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1393940
- Alternate Identifier(s):
- OSTI ID: 1401747
- Grant/Contract Number:
- AC02-06CH11357; DE‐AC02‐06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Sustainable Systems
- Additional Journal Information:
- Journal Volume: 1; Journal Issue: 1-2; Journal ID: ISSN 2366-7486
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 59 BASIC BIOLOGICAL SCIENCES; membranes; atomic layer deposition; photocatalysis; water treatment
Citation Formats
Lee, Anna, Libera, Joseph A., Waldman, Ruben Z., Ahmed, Aftab, Avila, Jason R., Elam, Jeffrey W., and Darling, Seth B. Conformal Nitrogen-Doped TiO2 Photocatalytic Coatings for Sunlight-Activated Membranes. United States: N. p., 2017.
Web. doi:10.1002/adsu.201600041.
Lee, Anna, Libera, Joseph A., Waldman, Ruben Z., Ahmed, Aftab, Avila, Jason R., Elam, Jeffrey W., & Darling, Seth B. Conformal Nitrogen-Doped TiO2 Photocatalytic Coatings for Sunlight-Activated Membranes. United States. https://doi.org/10.1002/adsu.201600041
Lee, Anna, Libera, Joseph A., Waldman, Ruben Z., Ahmed, Aftab, Avila, Jason R., Elam, Jeffrey W., and Darling, Seth B. Tue .
"Conformal Nitrogen-Doped TiO2 Photocatalytic Coatings for Sunlight-Activated Membranes". United States. https://doi.org/10.1002/adsu.201600041. https://www.osti.gov/servlets/purl/1393940.
@article{osti_1393940,
title = {Conformal Nitrogen-Doped TiO2 Photocatalytic Coatings for Sunlight-Activated Membranes},
author = {Lee, Anna and Libera, Joseph A. and Waldman, Ruben Z. and Ahmed, Aftab and Avila, Jason R. and Elam, Jeffrey W. and Darling, Seth B.},
abstractNote = {Photocatalytic degradation of organic contaminants is enticing for addressing challenging, nontraditional water sources. A novel nitrogen-doping method is utilized to grow conformal titania coatings with visible-light activity on porous membranes. Here, the resulting membranes exhibit effective degradation of model organic species in simulated sunlight while at the same time requiring substantially lower transmembrane pressure than undoped membranes.},
doi = {10.1002/adsu.201600041},
journal = {Advanced Sustainable Systems},
number = 1-2,
volume = 1,
place = {United States},
year = {2017},
month = {1}
}
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Works referenced in this record:
Precise and Ultrafast Molecular Sieving Through Graphene Oxide Membranes
journal, February 2014
- Joshi, R. K.; Carbone, P.; Wang, F. C.
- Science, Vol. 343, Issue 6172
Modification of ceramic membranes for pore structure tailoring: The atomic layer deposition route
journal, April 2012
- Li, Fengbin; Yang, Yang; Fan, Yiqun
- Journal of Membrane Science, Vol. 397-398
Synthesis of visible-light responsive C, N and Ce co-doped TiO2 mesoporous membranes via weak alkaline sol–gel process
journal, January 2012
- Cao, Xue Ping; Li, Dan; Jing, Wen Heng
- Journal of Materials Chemistry, Vol. 22, Issue 30
Nitrogen-Doped Titanium Dioxide as Visible-Light-Sensitive Photocatalyst: Designs, Developments, and Prospects
journal, May 2014
- Asahi, Ryoji; Morikawa, Takeshi; Irie, Hiroshi
- Chemical Reviews, Vol. 114, Issue 19
Heterogeneous photocatalytic degradation of organic contaminants over titanium dioxide: A review of fundamentals, progress and problems
journal, March 2008
- Gaya, Umar Ibrahim; Abdullah, Abdul Halim
- Journal of Photochemistry and Photobiology C: Photochemistry Reviews, Vol. 9, Issue 1
Deconvoluting the visible absorption spectrum of methyl orange using inverse Raman transform techniques
journal, October 1987
- Rava, Richard P.
- The Journal of Chemical Physics, Vol. 87, Issue 7
Visible Light Activity of Nitrogen-Doped TiO[sub 2] Thin Films Grown by Atomic Layer Deposition
journal, January 2008
- Cheng, Hsyi-En; Lee, Wen-Jen; Hsu, Ching-Ming
- Electrochemical and Solid-State Letters, Vol. 11, Issue 10
On the hydrophilicity of nitrogen-doped TiO2 thin films
journal, September 2007
- Mardare, D.; Luca, D.; Teodorescu, C. -M.
- Surface Science, Vol. 601, Issue 18
Hydrophilization of porous polypropylene membranes by atomic layer deposition of TiO2 for simultaneously improved permeability and selectivity
journal, December 2013
- Xu, Qiang; Yang, Jun; Dai, Jiawei
- Journal of Membrane Science, Vol. 448
Visible-Light Photocatalysis in Nitrogen-Doped Titanium Oxides
journal, July 2001
- Asahi, R.
- Science, Vol. 293, Issue 5528
A review on the visible light active titanium dioxide photocatalysts for environmental applications
journal, August 2012
- Pelaez, Miguel; Nolan, Nicholas T.; Pillai, Suresh C.
- Applied Catalysis B: Environmental, Vol. 125
Atomic Layer Epitaxy Growth of TiN Thin Films
journal, January 1995
- Ritala, Mikko
- Journal of The Electrochemical Society, Vol. 142, Issue 8
Why is anatase a better photocatalyst than rutile? - Model studies on epitaxial TiO2 films
journal, February 2014
- Luttrell, Tim; Halpegamage, Sandamali; Tao, Junguang
- Scientific Reports, Vol. 4, Issue 1
Control of optical properties of TiN_xO_y films and application for high performance solar selective absorbing coatings
journal, January 2014
- Chen, Feiliang; Wang, Shao-Wei; Yu, Liming
- Optical Materials Express, Vol. 4, Issue 9
The role of nitrogen doping on the development of visible light-induced photocatalytic activity in thin TiO2 films grown on glass by chemical vapour deposition
journal, April 2006
- Yates, H. M.; Nolan, M. G.; Sheel, D. W.
- Journal of Photochemistry and Photobiology A: Chemistry, Vol. 179, Issue 1-2
Photocatalytic Water Treatment by Titanium Dioxide: Recent Updates
journal, December 2012
- Lazar, Manoj; Varghese, Shaji; Nair, Santhosh
- Catalysts, Vol. 2, Issue 4
Understanding TiO 2 Photocatalysis: Mechanisms and Materials
journal, May 2014
- Schneider, Jenny; Matsuoka, Masaya; Takeuchi, Masato
- Chemical Reviews, Vol. 114, Issue 19
Visible light active TiO2 photocatalytic filtration membranes with improved permeability and low energy consumption
journal, April 2014
- Moustakas, N. G.; Katsaros, F. K.; Kontos, A. G.
- Catalysis Today, Vol. 224
Effect of nitrogen doping concentration on the properties of TiO2 films grown by atomic layer deposition
journal, April 2011
- Cheng, Hsyi-En; Chen, Yu-Ru; Wu, Wen-Tuan
- Materials Science and Engineering: B, Vol. 176, Issue 7
Nitrogen-Concentration Dependence on Photocatalytic Activity of TiO 2 - x N x Powders
journal, June 2003
- Irie, Hiroshi; Watanabe, Yuka; Hashimoto, Kazuhito
- The Journal of Physical Chemistry B, Vol. 107, Issue 23
Graphene-based membranes
journal, January 2015
- Liu, Gongping; Jin, Wanqin; Xu, Nanping
- Chemical Society Reviews, Vol. 44, Issue 15
Viscous flow reactor with quartz crystal microbalance for thin film growth by atomic layer deposition
journal, August 2002
- Elam, J. W.; Groner, M. D.; George, S. M.
- Review of Scientific Instruments, Vol. 73, Issue 8, p. 2981-2987
Atomic layer deposition of TiO2−xNx thin films for photocatalytic applications
journal, January 2006
- Pore, Viljami; Heikkilä, Mikko; Ritala, Mikko
- Journal of Photochemistry and Photobiology A: Chemistry, Vol. 177, Issue 1
PVDF membranes with simultaneously enhanced permeability and selectivity by breaking the tradeoff effect via atomic layer deposition of TiO2
journal, September 2013
- Wang, Qianqian; Wang, Xiaoting; Wang, Zhaohui
- Journal of Membrane Science, Vol. 442
Critical influence of surface nitrogen species on the activity of N-doped TiO2 thin-films during photodegradation of stearic acid under UV light irradiation
journal, November 2014
- Quesada-Cabrera, Raul; Sotelo-Vazquez, Carlos; Darr, Jawwad A.
- Applied Catalysis B: Environmental, Vol. 160-161
Photocatalytic Activity of Bulk Anatase and Rutile Single Crystals Using Infrared Absorption Spectroscopy
journal, March 2011
- Xu, Mingchun; Gao, Youkun; Moreno, Elias Martinez
- Physical Review Letters, Vol. 106, Issue 13
Carbon nanotube membranes with ultrahigh specific adsorption capacity for water desalination and purification
journal, August 2013
- Yang, Hui Ying; Han, Zhao Jun; Yu, Siu Fung
- Nature Communications, Vol. 4, Issue 1
Membrane materials for water purification: design, development, and application
journal, January 2016
- Lee, Anna; Elam, Jeffrey W.; Darling, Seth B.
- Environmental Science: Water Research & Technology, Vol. 2, Issue 1
Works referencing / citing this record:
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journal, June 2019
- Rosman, Nurafiqah; Wan Salleh, Wan Norharyati; Aziz, Farhana
- Catalysts, Vol. 9, Issue 7
Facile synthesis of thin black TiO2 − x nanosheets with enhanced lithium-storage capacity and visible light photocatalytic hydrogen production
journal, January 2019
- Sun, Lin; Xie, Jie; Li, Qi
- Journal of Solid State Electrochemistry, Vol. 23, Issue 3
One step synthesis of N-doped carbon/amorphous iron oxide composite for enhanced photodegradation activity
journal, August 2019
- Cao, Zhiqin; Zuo, Chengyang
- Materials Research Express, Vol. 6, Issue 10
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text, January 2019
- Rodwihok, Chatchai; Wongratanaphisan, Duangmanee; Ngo, Yen Linh Thi
- Zenodo
TiOxNy Modified TiO2 Powders Prepared by Plasma Enhanced Atomic Layer Deposition for Highly Visible Light Photocatalysis
journal, August 2018
- Cao, Yan-Qiang; Zhao, Xi-Rui; Chen, Jun
- Scientific Reports, Vol. 8, Issue 1
Visible Light Sensitive SnO2/ZnCo2O4 Material for the Photocatalytic Removal of Organic Pollutants in Water
journal, June 2019
- Benhebal, Hadj; Wolfs, Cédric; Kadi, Samir
- Inorganics, Vol. 7, Issue 6
Overview of Photocatalytic Membrane Reactors in Organic Synthesis, Energy Storage and Environmental Applications
journal, March 2019
- Molinari, Raffaele; Lavorato, Cristina; Argurio, Pietro
- Catalysts, Vol. 9, Issue 3
Janus Membranes via Diffusion-Controlled Atomic Layer Deposition
journal, June 2018
- Waldman, Ruben Z.; Yang, Hao-Cheng; Mandia, David J.
- Advanced Materials Interfaces, Vol. 5, Issue 15
Dopamine: Just the Right Medicine for Membranes
journal, January 2018
- Yang, Hao-Cheng; Waldman, Ruben Z.; Wu, Ming-Bang
- Advanced Functional Materials, Vol. 28, Issue 8
Advanced Design and Synthesis of Composite Photocatalysts for the Remediation of Wastewater: A Review
journal, January 2019
- Ge, Jianlong; Zhang, Yifan; Heo, Young-Jung
- Catalysts, Vol. 9, Issue 2
Atomic layer deposition for membrane interface engineering
journal, January 2018
- Yang, Hao-Cheng; Waldman, Ruben Z.; Chen, Zhaowei
- Nanoscale, Vol. 10, Issue 44
Perspective: Interfacial materials at the interface of energy and water
journal, July 2018
- Darling, Seth B.
- Journal of Applied Physics, Vol. 124, Issue 3
Effect of GO additive in ZnO/rGO nanocomposites with enhanced photosensitivity and photocatalytic activity
text, January 2019
- Rodwihok, Chatchai; Wongratanaphisan, Duangmanee; Ngo, Yen Linh Thi
- Zenodo