New Insights into Perfluorinated Sulfonic-Acid Ionomers
Abstract
In this comprehensive review, recent progress and developments on perfluorinated sulfonic-acid (PFSA) membranes have been summarized on many key topics. Although quite well investigated for decades, PFSA ionomers’ complex behavior, along with their key role in many emerging technologies, have presented significant scientific challenges but also helped create a unique cross-disciplinary research field to overcome such challenges. Research and progress on PFSAs, especially when considered with their applications, are at the forefront of bridging electrochemistry and polymer (physics), which have also opened up development of state-of-the-art in situ characterization techniques as well as multiphysics computation models. Topics reviewed stem from correlating the various physical (e.g., mechanical) and transport properties with morphology and structure across time and length scales. In addition, topics of recent interest such as structure/transport correlations and modeling, composite PFSA membranes, degradation phenomena, and PFSA thin films are presented. Throughout, the impact of PFSA chemistry and side-chain is also discussed to present a broader perspective.
- Authors:
-
[1];
- Energy Conversion Group, Energy Technologies Area, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, MS70-108B, Berkeley, California 94720, United States
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Fuel Cell Technologies Office; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office
- OSTI Identifier:
- 1341223
- Alternate Identifier(s):
- OSTI ID: 1393613
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Published Article
- Journal Name:
- Chemical Reviews
- Additional Journal Information:
- Journal Name: Chemical Reviews Journal Volume: 117 Journal Issue: 3; Journal ID: ISSN 0009-2665
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Kusoglu, Ahmet, and Weber, Adam Z. New Insights into Perfluorinated Sulfonic-Acid Ionomers. United States: N. p., 2017.
Web. doi:10.1021/acs.chemrev.6b00159.
Kusoglu, Ahmet, & Weber, Adam Z. New Insights into Perfluorinated Sulfonic-Acid Ionomers. United States. https://doi.org/10.1021/acs.chemrev.6b00159
Kusoglu, Ahmet, and Weber, Adam Z. Mon .
"New Insights into Perfluorinated Sulfonic-Acid Ionomers". United States. https://doi.org/10.1021/acs.chemrev.6b00159.
@article{osti_1341223,
title = {New Insights into Perfluorinated Sulfonic-Acid Ionomers},
author = {Kusoglu, Ahmet and Weber, Adam Z.},
abstractNote = {In this comprehensive review, recent progress and developments on perfluorinated sulfonic-acid (PFSA) membranes have been summarized on many key topics. Although quite well investigated for decades, PFSA ionomers’ complex behavior, along with their key role in many emerging technologies, have presented significant scientific challenges but also helped create a unique cross-disciplinary research field to overcome such challenges. Research and progress on PFSAs, especially when considered with their applications, are at the forefront of bridging electrochemistry and polymer (physics), which have also opened up development of state-of-the-art in situ characterization techniques as well as multiphysics computation models. Topics reviewed stem from correlating the various physical (e.g., mechanical) and transport properties with morphology and structure across time and length scales. In addition, topics of recent interest such as structure/transport correlations and modeling, composite PFSA membranes, degradation phenomena, and PFSA thin films are presented. Throughout, the impact of PFSA chemistry and side-chain is also discussed to present a broader perspective.},
doi = {10.1021/acs.chemrev.6b00159},
journal = {Chemical Reviews},
number = 3,
volume = 117,
place = {United States},
year = {Mon Jan 23 00:00:00 EST 2017},
month = {Mon Jan 23 00:00:00 EST 2017}
}
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