Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation
Abstract
Magnetoelastoelectric coupling in an engineered biphasic multiferroic nanocomposite enables a novel magnetic field direction-defined propagation control of terahertz (THz) waves. These core–shell nanoparticles are comprised of a ferromagnetic cobalt ferrite core and a ferroelectric barium titanate shell. Furthermore, an assembly of these nanoparticles, when operated in external magnetic fields, exhibits a controllable amplitude modulation when the magnetic field is applied antiparallel to the THz wave propagation direction; yet the same assembly displays an additional phase modulation when the magnetic field is applied along the propagation direction. And while field-induced magnetostriction of the core leads to amplitude modulation, phase modulation is a result of stress-mediated piezoelectricity of the outer ferroelectric shell.
- Authors:
-
- Univ. of Texas, San Antonio, TX (United States). Dept. of Electrical and Computer Engineering
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22); National Science Foundation (NSF); National Institutes of Health (NIH)
- OSTI Identifier:
- 1392884
- Report Number(s):
- LA-UR-17-25491
Journal ID: ISSN 2040-3364 ; 2040-3372 (Electronic)
- Grant/Contract Number:
- AC52-06NA25396; W911NF-12-1-0082; 1002380; G12MD007591
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nanoscale
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 35; Journal ID: ISSN 2040-3364
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Material Science
Citation Formats
Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., and Guo, Ruyan. Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation. United States: N. p., 2017.
Web. doi:10.1039/C7NR03504G.
Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., & Guo, Ruyan. Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation. United States. https://doi.org/10.1039/C7NR03504G
Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., and Guo, Ruyan. Mon .
"Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation". United States. https://doi.org/10.1039/C7NR03504G. https://www.osti.gov/servlets/purl/1392884.
@article{osti_1392884,
title = {Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation},
author = {Dutta, Moumita and Prasankumar, Rohit Prativadi and Natarajan, Kamaraju and Betal, Soutik and Bhalla, Amar S. and Guo, Ruyan},
abstractNote = {Magnetoelastoelectric coupling in an engineered biphasic multiferroic nanocomposite enables a novel magnetic field direction-defined propagation control of terahertz (THz) waves. These core–shell nanoparticles are comprised of a ferromagnetic cobalt ferrite core and a ferroelectric barium titanate shell. Furthermore, an assembly of these nanoparticles, when operated in external magnetic fields, exhibits a controllable amplitude modulation when the magnetic field is applied antiparallel to the THz wave propagation direction; yet the same assembly displays an additional phase modulation when the magnetic field is applied along the propagation direction. And while field-induced magnetostriction of the core leads to amplitude modulation, phase modulation is a result of stress-mediated piezoelectricity of the outer ferroelectric shell.},
doi = {10.1039/C7NR03504G},
journal = {Nanoscale},
number = 35,
volume = 9,
place = {United States},
year = {Mon Aug 07 00:00:00 EDT 2017},
month = {Mon Aug 07 00:00:00 EDT 2017}
}
Web of Science
Works referenced in this record:
Synthesis of barium titanate nanopowder using polymeric precursor method
journal, January 2006
- Vinothini, V.; Singh, Paramanand; Balasubramanian, M.
- Ceramics International, Vol. 32, Issue 2
Plasma wave terahertz electronics
journal, January 2010
- Shur, M.
- Electronics Letters, Vol. 46, Issue 26
Infrared and terahertz studies of polar phonons and magnetodielectric effect in multiferroic ceramics
journal, January 2007
- Kamba, S.; Nuzhnyy, D.; Savinov, M.
- Physical Review B, Vol. 75, Issue 2
Surface potential at a ferroelectric grain due to asymmetric screening of depolarization fields
journal, March 2014
- Genenko, Yuri A.; Hirsch, Ofer; Erhart, Paul
- Journal of Applied Physics, Vol. 115, Issue 10
Probing ultrafast spin dynamics through a magnon resonance in the antiferromagnetic multiferroic
journal, September 2016
- Bowlan, P.; Trugman, S. A.; Bowlan, J.
- Physical Review B, Vol. 94, Issue 10
Polarizing effect of aligned nanoparticles in terahertz frequency region
journal, January 2013
- Polley, Debanjan; Ganguly, Arnab; Barman, Anjan
- Optics Letters, Vol. 38, Issue 15
Ferroelectromagnets [Segnetomagnetiki]
journal, January 1982
- Smolenskii, G. A.; Chupis, I. E.
- Uspekhi Fizicheskih Nauk, Vol. 137, Issue 7
Terahertz magnetic modulator based on magnetically clustered nanoparticles
journal, October 2014
- Shalaby, Mostafa; Peccianti, Marco; Ozturk, Yavuz
- Applied Physics Letters, Vol. 105, Issue 15
Gigantic terahertz magnetochromism via electromagnons in the hexaferrite magnet Ba Mg Fe O
journal, February 2011
- Kida, N.; Kumakura, S.; Ishiwata, S.
- Physical Review B, Vol. 83, Issue 6
Electromagnons in Multiferroic and
journal, January 2007
- Sushkov, A. B.; Aguilar, R. Valdés; Park, S.
- Physical Review Letters, Vol. 98, Issue 2
Temperature dependence of the structural, magnetic, and magnetostrictive properties of zinc-substituted cobalt ferrite
journal, May 2013
- Nlebedim, I. C.; Vinitha, M.; Praveen, P. J.
- Journal of Applied Physics, Vol. 113, Issue 19
Effect of spin excitations with simultaneous magnetic- and electric-dipole character on the static magnetoelectric properties of multiferroic materials
journal, May 2014
- Szaller, Dávid; Bordács, Sándor; Kocsis, Vilmos
- Physical Review B, Vol. 89, Issue 18
Multiferroic BaTiO3-CoFe2O4 Nanostructures
journal, January 2004
- Zheng, H.
- Science, Vol. 303, Issue 5658
Contrast-enhanced continuous-terahertz-wave imaging based on superparamagnetic iron oxide nanoparticles for biomedical applications
journal, January 2016
- Zhang, Rui; Zhang, Liangliang; Wu, Tong
- Optics Express, Vol. 24, Issue 8
High magnetostriction and coupling coefficient for sintered cobalt ferrite derived from superparamagnetic nanoparticles
journal, August 2012
- Khaja Mohaideen, K.; Joy, P. A.
- Applied Physics Letters, Vol. 101, Issue 7
Terahertz magneto-optical spectroscopy of a two-dimensional hole gas
journal, January 2015
- Kamaraju, N.; Pan, W.; Ekenberg, U.
- Applied Physics Letters, Vol. 106, Issue 3
Why Are There so Few Magnetic Ferroelectrics?
journal, July 2000
- Hill, Nicola A.
- The Journal of Physical Chemistry B, Vol. 104, Issue 29
Spectrally Wide-Band Terahertz Wave Modulator Based on Optically Tuned Graphene
journal, September 2012
- Weis, Peter; Garcia-Pomar, Juan L.; Höh, Michael
- ACS Nano, Vol. 6, Issue 10
Chirality of matter shows up via spin excitations
journal, August 2012
- Bordács, S.; Kézsmárki, I.; Szaller, D.
- Nature Physics, Vol. 8, Issue 10
Magnetoelectric resonance with electromagnons in a perovskite helimagnet
journal, December 2011
- Takahashi, Youtarou; Shimano, Ryo; Kaneko, Yoshio
- Nature Physics, Vol. 8, Issue 2
Origin of Magnetic Anisotropy in Co x Fe 3− x O 4
journal, March 1958
- Slonczewski, J. C.
- Journal of Applied Physics, Vol. 29, Issue 3
Low frequency piezoresonance defined dynamic control of terahertz wave propagation
journal, November 2016
- Dutta, Moumita; Betal, Soutik; Peralta, Xomalin G.
- Scientific Reports, Vol. 6, Issue 1
Terahertz Faraday rotation in a magnetic liquid: High magneto-optical figure of merit and broadband operation in a ferrofluid
journal, June 2012
- Shalaby, Mostafa; Peccianti, Marco; Ozturk, Yavuz
- Applied Physics Letters, Vol. 100, Issue 24
High-order photonic bandgap reflex klystron using carbon nanotube multi-beam cathode
journal, January 2012
- Jang, Kyu-Ha; Park, Seong Hee; Lee, Kitae
- Electronics Letters, Vol. 48, Issue 12
Recent Progress in Multiferroic Magnetoelectric Composites: from Bulk to Thin Films
journal, February 2011
- Ma, Jing; Hu, Jiamian; Li, Zheng
- Advanced Materials, Vol. 23, Issue 9
Broadband and subwavelength terahertz modulators using tunable plasmonic crystals with semiconductor rods
journal, February 2012
- Vasić, Borislav; Gajić, Radoš
- Journal of Physics D: Applied Physics, Vol. 45, Issue 9
Hysteretic magnetoelectric behavior of CoFe 2 O 4 –BaTiO 3 composites prepared by reductive sintering and reoxidation
journal, January 2016
- Walther, Till; Straube, Ulrich; Köferstein, Roberto
- Journal of Materials Chemistry C, Vol. 4, Issue 21
Directly probing spin dynamics in insulating antiferromagnets using ultrashort terahertz pulses
journal, November 2016
- Bowlan, P.; Trugman, S. A.; Wang, X.
- Physical Review B, Vol. 94, Issue 18
Multiferroics progress and prospects in thin films
journal, January 2007
- Ramesh, R.; Spaldin, Nicola A.
- Nature Materials, Vol. 6, Issue 1, p. 21-29
Possible evidence for electromagnons in multiferroic manganites
journal, January 2006
- Pimenov, A.; Mukhin, A. A.; Ivanov, V. Yu.
- Nature Physics, Vol. 2, Issue 2
Electromagnon excitation in the field-induced noncollinear ferrimagnetic phase of studied by polarized inelastic neutron scattering and terahertz time-domain optical spectroscopy
journal, January 2016
- Nakajima, Taro; Takahashi, Youtarou; Kibayashi, Shunsuke
- Physical Review B, Vol. 93, Issue 3
Magnetically tunable terahertz magnetoplasmons in ferrofluid-filled photonic crystals
journal, October 2013
- Fan, Fei; Chen, Sai; Lin, Wei
- Applied Physics Letters, Vol. 103, Issue 16
Terahertz fields and applications
journal, January 2004
- Dragoman, D.; Dragoman, M.
- Progress in Quantum Electronics, Vol. 28, Issue 1
Nanobolometers for THz Photon Detection
journal, September 2011
- Karasik, Boris S.; Sergeev, Andrei V.; Prober, Daniel E.
- IEEE Transactions on Terahertz Science and Technology, Vol. 1, Issue 1
Terahertz electro-optic properties of PbZr0.52Ti0.48O3 and BaTiO3 ferroelectric thin films
journal, September 2014
- Chen, Lei; Zhang, Yuan; Guo, Quan
- Applied Physics Letters, Vol. 105, Issue 11
Numerical approach for tailoring performance of magnetoelectric PZT/terfenol-D laminated composites
journal, April 2010
- Wang, Jimmy. H.; Priya, Shashank; Guo, Ruyan
- Journal of Applied Physics, Vol. 107, Issue 8
A magnetic non-reciprocal isolator for broadband terahertz operation
journal, March 2013
- Shalaby, Mostafa; Peccianti, Marco; Ozturk, Yavuz
- Nature Communications, Vol. 4, Issue 1
Channel Modeling and Capacity Analysis for Electromagnetic Wireless Nanonetworks in the Terahertz Band
journal, October 2011
- Jornet, Josep Miquel; Akyildiz, Ian F.
- IEEE Transactions on Wireless Communications, Vol. 10, Issue 10
Multiferroic and magnetoelectric materials
journal, August 2006
- Eerenstein, W.; Mathur, N. D.; Scott, J. F.
- Nature, Vol. 442, Issue 7104