DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Realizing in-plane surface diffraction by x-ray multiple-beam diffraction with large incidence angle

Journal Article · · Applied Physics Letters
DOI: https://doi.org/10.1063/1.4901046 · OSTI ID:1392293
 [1];  [2];  [1];  [3];  [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Nanjing Univ. (China)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States)

Based on rigorous dynamical-theory calculations, we demonstrate in this paper the principle of an x-ray multiple-beam diffraction (MBD) scheme that overcomes the long-lasting difficulties of high-resolution in-plane diffraction from crystal surfaces. This scheme only utilizes symmetric reflection geometry with large incident angles but activates the out-of-plane and in-plane diffraction processes simultaneously and separately in the continuous MBD planes. The in-plane diffraction is realized by detoured MBD, where the intermediate diffracted waves propagate parallel to the surface, which corresponds to an absolute Bragg surface diffraction configuration that is extremely sensitive to surface structures. Finally, a series of MBD diffraction and imaging techniques may be developed from this principle to study surface/interface (misfit) strains, lateral nanostructures, and phase transitions of a wide range of (pseudo)cubic crystal structures, including ultrathin epitaxial films and multilayers, quantum dots, strain-engineered semiconductor or (multi)ferroic materials, etc.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States); Brookhaven National Lab. (BNL), Upton, NY (United States); Nanjing Univ. (China)
Sponsoring Organization:
Ministry of Science and Technology (MOST) (China); National Natural Science Foundation of China (NSFC); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
AC02-06CH11357; AC02-98CH10886
OSTI ID:
1392293
Journal Information:
Applied Physics Letters, Journal Name: Applied Physics Letters Journal Issue: 18 Vol. 105; ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (17)

X-Ray Multiple-Wave Diffraction book January 2004
Ultimate upgrade for US synchrotron journal September 2013
A strong ferroelectric ferromagnet created by means of spin–lattice coupling journal August 2010
High-geometrical-resolution imaging of dislocations in SiC using monochromatic synchrotron topography journal December 2007
High resolution grazing-incidence in-plane x-ray diffraction for measuring the strain of a Si thin layer journal November 2010
Fourier coupled-wave diffraction theory of periodic structures and crystals journal June 2013
Dynamical x-ray diffraction of multilayers and superlattices: Recursion matrix extension to grazing angles journal February 1998
Multiple-beam x-ray diffraction near exact backscattering in silicon journal January 2001
Competing Misfit Relaxation Mechanisms in Epitaxial Correlated Oxides journal March 2013
Spin-Orbital Superstructure in Strained Ferrimagnetic Perovskite Cobalt Oxide journal July 2013
Orbital Control of Noncollinear Magnetic Order in Nickel Oxide Heterostructures journal September 2013
Tuning Magnetic Coupling in Sr 2 IrO 4 Thin Films with Epitaxial Strain journal April 2014
Strain Imaging of Nanoscale Semiconductor Heterostructures with X-Ray Bragg Projection Ptychography journal April 2014
Interplay between Anisotropic Strain Relaxation and Uniaxial Interface Magnetic Anisotropy in Epitaxial Fe Films on (001) GaAs journal January 2003
X-Ray Resonance in Crystal Cavities: Realization of Fabry-Perot Resonator for Hard X Rays journal May 2005
Lattice strain distribution resolved by X-ray Bragg-surface diffraction in an Si matrix distorted by embedded FeSi 2 nanoparticles journal November 2013
Continuous X-ray multiple-beam diffraction with primary Bragg angle from 0 to 90° journal September 2014

Cited By (1)

Assessment of phase transition and thermal expansion coefficients by means of secondary multiple reflections of Renninger scans journal October 2019