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Title: High temperature ferromagnetism in π-conjugated two-dimensional metal–organic frameworks

Simulations demonstrate the critical roles of π-conjugation and large magnetic anisotropy in realizing high-temperature ferromagnetic 2D metal–organic framework, which is also half-metallic.
Authors:
 [1] ;  [1] ;  [1] ;  [1] ; ORCiD logo [1] ; ORCiD logo [1]
  1. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Publication Date:
Grant/Contract Number:
SC0001088
Type:
Accepted Manuscript
Journal Name:
Chemical Science
Additional Journal Information:
Journal Volume: 8; Journal Issue: 4; Related Information: CE partners with Massachusetts Institute of Technology (lead); Brookhaven National Laboratory; Harvard University; Journal ID: ISSN 2041-6520
Publisher:
Royal Society of Chemistry
Research Org:
Energy Frontier Research Centers (EFRC) (United States). Center for Excitonics (CE)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; solar (photovoltaic), solid state lighting, photosynthesis (natural and artificial), charge transport, optics, synthesis (novel materials), synthesis (self-assembly), synthesis (scalable processing)
OSTI Identifier:
1388515