High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor
Abstract
A novel polymer donor (PBDTS-Se) is designed to match with a non-fullerene acceptor (SdiPBI-S). The corresponding solar cells show a high efficiency of 8.22%, which result from synergetic improvements of light harvesting, charge carrier transport and collection, and morphology. The results indicate that rational design of novel donor materials is important for non-fullerene organic solar cells.
- Authors:
-
- Beihang Univ., Beijing (China). Heeger Beijing Research and Development Center
- Chinese Academy of Sciences (CAS), Beijing (China). Inst. of Chemistry
- Heeger Beijing Research and Development Center, School of Chemistry and Environment, Beihang University, Beijing 100191 P. R. China
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Science Division
- Univ. of Massachusetts, Amherst, MA (United States). Polymer Science and Engineering Dept.
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1379298
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Science
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 9; Journal ID: ISSN 2198-3844
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY
Citation Formats
Liu, Tao, Meng, Dong, Cai, Yunhao, Sun, Xiaobo, Li, Yan, Huo, Lijun, Liu, Feng, Wang, Zhaohui, Russell, Thomas P., and Sun, Yanming. High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor. United States: N. p., 2016.
Web. doi:10.1002/advs.201600117.
Liu, Tao, Meng, Dong, Cai, Yunhao, Sun, Xiaobo, Li, Yan, Huo, Lijun, Liu, Feng, Wang, Zhaohui, Russell, Thomas P., & Sun, Yanming. High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor. United States. https://doi.org/10.1002/advs.201600117
Liu, Tao, Meng, Dong, Cai, Yunhao, Sun, Xiaobo, Li, Yan, Huo, Lijun, Liu, Feng, Wang, Zhaohui, Russell, Thomas P., and Sun, Yanming. Sat .
"High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor". United States. https://doi.org/10.1002/advs.201600117. https://www.osti.gov/servlets/purl/1379298.
@article{osti_1379298,
title = {High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor},
author = {Liu, Tao and Meng, Dong and Cai, Yunhao and Sun, Xiaobo and Li, Yan and Huo, Lijun and Liu, Feng and Wang, Zhaohui and Russell, Thomas P. and Sun, Yanming},
abstractNote = {A novel polymer donor (PBDTS-Se) is designed to match with a non-fullerene acceptor (SdiPBI-S). The corresponding solar cells show a high efficiency of 8.22%, which result from synergetic improvements of light harvesting, charge carrier transport and collection, and morphology. The results indicate that rational design of novel donor materials is important for non-fullerene organic solar cells.},
doi = {10.1002/advs.201600117},
journal = {Advanced Science},
number = 9,
volume = 3,
place = {United States},
year = {Sat Apr 23 00:00:00 EDT 2016},
month = {Sat Apr 23 00:00:00 EDT 2016}
}
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Works referenced in this record:
Perylene diimides based materials for organic solar cells
journal, July 2013
- Kozma, Erika; Catellani, Marinella
- Dyes and Pigments, Vol. 98, Issue 1
Quantitative Determination of Organic Semiconductor Microstructure from the Molecular to Device Scale
journal, June 2012
- Rivnay, Jonathan; Mannsfeld, Stefan C. B.; Miller, Chad E.
- Chemical Reviews, Vol. 112, Issue 10
Contorted Polycyclic Aromatics
journal, December 2014
- Ball, Melissa; Zhong, Yu; Wu, Ying
- Accounts of Chemical Research, Vol. 48, Issue 2
Rylene and Related Diimides for Organic Electronics
journal, December 2010
- Zhan, Xiaowei; Facchetti, Antonio; Barlow, Stephen
- Advanced Materials, Vol. 23, Issue 2, p. 268-284
Heteroarenes as high performance organic semiconductors
journal, January 2013
- Jiang, Wei; Li, Yan; Wang, Zhaohui
- Chemical Society Reviews, Vol. 42, Issue 14
High-efficiency non-fullerene organic solar cells enabled by a difluorobenzothiadiazole-based donor polymer combined with a properly matched small molecule acceptor
journal, January 2015
- Zhao, Jingbo; Li, Yunke; Lin, Haoran
- Energy & Environmental Science, Vol. 8, Issue 2
Device Physics of PolymerFullerene Bulk Heterojunction Solar Cells
journal, June 2007
- Blom, P. W. M.; Mihailetchi, V. D.; Koster, L. J. A.
- Advanced Materials, Vol. 19, Issue 12, p. 1551-1566
Efficient Organic Solar Cells with Helical Perylene Diimide Electron Acceptors
journal, October 2014
- Zhong, Yu; Trinh, M. Tuan; Chen, Rongsheng
- Journal of the American Chemical Society, Vol. 136, Issue 43
All-Polymer Solar Cells Based on Absorption-Complementary Polymer Donor and Acceptor with High Power Conversion Efficiency of 8.27%
journal, December 2015
- Gao, Liang; Zhang, Zhi-Guo; Xue, Lingwei
- Advanced Materials, Vol. 28, Issue 9
High-Performance Solution-Processed Non-Fullerene Organic Solar Cells Based on Selenophene-Containing Perylene Bisimide Acceptor
journal, December 2015
- Meng, Dong; Sun, Dan; Zhong, Chengmei
- Journal of the American Chemical Society, Vol. 138, Issue 1
Tailor-Made Rylene Arrays for High Performance n-Channel Semiconductors
journal, September 2014
- Jiang, Wei; Li, Yan; Wang, Zhaohui
- Accounts of Chemical Research, Vol. 47, Issue 10
Perylene Imides for Organic Photovoltaics: Yesterday, Today, and Tomorrow
journal, January 2012
- Li, Chen; Wonneberger, Henrike
- Advanced Materials, Vol. 24, Issue 5
Soft x-ray scattering facility at the Advanced Light Source with real-time data processing and analysis
journal, April 2012
- Gann, E.; Young, A. T.; Collins, B. A.
- Review of Scientific Instruments, Vol. 83, Issue 4
Synthesis and Absorption Spectra of n-Type Conjugated Polymers Based on Perylene Diimide
journal, September 2008
- Huo, Lijun; Zhou, Yi; Li, Yongfang
- Macromolecular Rapid Communications, Vol. 29, Issue 17
Alkylthio-Substituted Polythiophene: Absorption and Photovoltaic Properties
journal, June 2009
- Huo, Lijun; Zhou, Yi; Li, Yongfang
- Macromolecular Rapid Communications, Vol. 30, Issue 11
Non-Fullerene-Acceptor-Based Bulk-Heterojunction Organic Solar Cells with Efficiency over 7%
journal, August 2015
- Sun, Dan; Meng, Dong; Cai, Yunhao
- Journal of the American Chemical Society, Vol. 137, Issue 34
Improvement of open-circuit voltage and photovoltaic properties of 2D-conjugated polymers by alkylthio substitution
journal, January 2014
- Cui, Chaohua; Wong, Wai-Yeung; Li, Yongfang
- Energy Environ. Sci., Vol. 7, Issue 7
Endohedral fullerenes for organic photovoltaic devices
journal, February 2009
- Ross, Russel B.; Cardona, Claudia M.; Guldi, Dirk M.
- Nature Materials, Vol. 8, Issue 3
Electrical characteristics and efficiency of single-layer organic light-emitting diodes
journal, November 1998
- Malliaras, G. G.; Salem, J. R.; Brock, P. J.
- Physical Review B, Vol. 58, Issue 20
Electron Trapping in Dye/Polymer Blend Photovoltaic Cells
journal, September 2000
- Dittmer, J. J.; Marseglia, E. A.; Friend, R. H.
- Advanced Materials, Vol. 12, Issue 17
The Next Breakthrough for Organic Photovoltaics?
journal, December 2014
- Jackson, Nicholas E.; Savoie, Brett M.; Marks, Tobin J.
- The Journal of Physical Chemistry Letters, Vol. 6, Issue 1
Imide- and Amide-Functionalized Polymer Semiconductors
journal, September 2014
- Guo, Xugang; Facchetti, Antonio; Marks, Tobin J.
- Chemical Reviews, Vol. 114, Issue 18
An Electron Acceptor Challenging Fullerenes for Efficient Polymer Solar Cells
journal, January 2015
- Lin, Yuze; Wang, Jiayu; Zhang, Zhi-Guo
- Advanced Materials, Vol. 27, Issue 7
Organic non-fullerene acceptors for organic photovoltaics
journal, January 2011
- Sonar, Prashant; Fong Lim, Jacelyn Pui; Chan, Khai Leok
- Energy & Environmental Science, Vol. 4, Issue 5, p. 1558-1574
Polymer solar cells
journal, February 2012
- Li, Gang; Zhu, Rui; Yang, Yang
- Nature Photonics, Vol. 6, Issue 3
Material and Energy Intensity of Fullerene Production
journal, March 2011
- Anctil, Annick; Babbitt, Callie W.; Raffaelle, Ryne P.
- Environmental Science & Technology, Vol. 45, Issue 6
Perylene bisimide dyes as versatile building blocks for functional supramolecular architectures
journal, January 2004
- Würthner, Frank
- Chem. Commun., Issue 14
High-Performance Non-Fullerene Polymer Solar Cells Based on a Pair of Donor-Acceptor Materials with Complementary Absorption Properties
journal, October 2015
- Lin, Haoran; Chen, Shangshang; Li, Zhengke
- Advanced Materials, Vol. 27, Issue 45
Fine-Tuning the 3D Structure of Nonfullerene Electron Acceptors Toward High-Performance Polymer Solar Cells
journal, April 2015
- Li, Haiyan; Hwang, Ye-Jin; Courtright, Brett A. E.
- Advanced Materials, Vol. 27, Issue 21
Nonfullerene Polymer Solar Cells with 8.5% Efficiency Enabled by a New Highly Twisted Electron Acceptor Dimer
journal, October 2015
- Hwang, Ye-Jin; Li, Haiyan; Courtright, Brett A. E.
- Advanced Materials, Vol. 28, Issue 1
The Active Layer Morphology of Organic Solar Cells Probed with Grazing Incidence Scattering Techniques
journal, February 2014
- Müller-Buschbaum, Peter
- Advanced Materials, Vol. 26, Issue 46
Effect of Temperature and Illumination on the Electrical Characteristics of Polymer–Fullerene Bulk-Heterojunction Solar Cells
journal, January 2004
- Riedel, I.; Parisi, J.; Dyakonov, V.
- Advanced Functional Materials, Vol. 14, Issue 1
Electron Trapping in Higher Adduct Fullerene-Based Solar Cells
journal, September 2009
- Lenes, Martijn; Shelton, Steve W.; Sieval, Alex B.
- Advanced Functional Materials, Vol. 19, Issue 18
Thieno, Furo, and Selenopheno[3,4- c ]pyrrole-4,6-dione Copolymers: Air-Processed Polymer Solar Cells with Power Conversion Efficiency up to 7.1%
journal, September 2015
- Najari, Ahmed; Beaupré, Serge; Allard, Nicolas
- Advanced Energy Materials, Vol. 5, Issue 23
Molecular helices as electron acceptors in high-performance bulk heterojunction solar cells
journal, September 2015
- Zhong, Yu; Trinh, M. Tuan; Chen, Rongsheng
- Nature Communications, Vol. 6, Issue 1
From lab to fab: how must the polymer solar cell materials design change? – an industrial perspective
journal, January 2014
- Po, Riccardo; Bernardi, Andrea; Calabrese, Anna
- Energy & Environmental Science, Vol. 7, Issue 3
All-Polymer Solar Cells with 3.3% Efficiency Based on Naphthalene Diimide-Selenophene Copolymer Acceptor
journal, September 2013
- Earmme, Taeshik; Hwang, Ye-Jin; Murari, Nishit M.
- Journal of the American Chemical Society, Vol. 135, Issue 40, p. 14960-14963
Rylene and Related Diimides for Organic Electronics
journal, December 2010
- Zhan, Xiaowei; Facchetti, Antonio; Barlow, Stephen
- Advanced Materials, Vol. 23, Issue 2, p. 268-284
Perylene Imides for Organic Photovoltaics: Yesterday, Today, and Tomorrow
journal, January 2012
- Li, Chen; Wonneberger, Henrike
- Advanced Materials, Vol. 24, Issue 5
The Active Layer Morphology of Organic Solar Cells Probed with Grazing Incidence Scattering Techniques
journal, February 2014
- Müller-Buschbaum, Peter
- Advanced Materials, Vol. 26, Issue 46
An Electron Acceptor Challenging Fullerenes for Efficient Polymer Solar Cells
journal, January 2015
- Lin, Yuze; Wang, Jiayu; Zhang, Zhi-Guo
- Advanced Materials, Vol. 27, Issue 7
Fine-Tuning the 3D Structure of Nonfullerene Electron Acceptors Toward High-Performance Polymer Solar Cells
journal, April 2015
- Li, Haiyan; Hwang, Ye-Jin; Courtright, Brett A. E.
- Advanced Materials, Vol. 27, Issue 21
High-Performance Non-Fullerene Polymer Solar Cells Based on a Pair of Donor-Acceptor Materials with Complementary Absorption Properties
journal, October 2015
- Lin, Haoran; Chen, Shangshang; Li, Zhengke
- Advanced Materials, Vol. 27, Issue 45
Nonfullerene Polymer Solar Cells with 8.5% Efficiency Enabled by a New Highly Twisted Electron Acceptor Dimer
journal, October 2015
- Hwang, Ye-Jin; Li, Haiyan; Courtright, Brett A. E.
- Advanced Materials, Vol. 28, Issue 1
Tailor-Made Rylene Arrays for High Performance n-Channel Semiconductors
journal, September 2014
- Jiang, Wei; Li, Yan; Wang, Zhaohui
- Accounts of Chemical Research, Vol. 47, Issue 10
Contorted Polycyclic Aromatics
journal, December 2014
- Ball, Melissa; Zhong, Yu; Wu, Ying
- Accounts of Chemical Research, Vol. 48, Issue 2
Quantitative Determination of Organic Semiconductor Microstructure from the Molecular to Device Scale
journal, June 2012
- Rivnay, Jonathan; Mannsfeld, Stefan C. B.; Miller, Chad E.
- Chemical Reviews, Vol. 112, Issue 10
Imide- and Amide-Functionalized Polymer Semiconductors
journal, September 2014
- Guo, Xugang; Facchetti, Antonio; Marks, Tobin J.
- Chemical Reviews, Vol. 114, Issue 18
Material and Energy Intensity of Fullerene Production
journal, March 2011
- Anctil, Annick; Babbitt, Callie W.; Raffaelle, Ryne P.
- Environmental Science & Technology, Vol. 45, Issue 6
All-Polymer Solar Cells with 3.3% Efficiency Based on Naphthalene Diimide-Selenophene Copolymer Acceptor
journal, September 2013
- Earmme, Taeshik; Hwang, Ye-Jin; Murari, Nishit M.
- Journal of the American Chemical Society, Vol. 135, Issue 40, p. 14960-14963
Non-Fullerene-Acceptor-Based Bulk-Heterojunction Organic Solar Cells with Efficiency over 7%
journal, August 2015
- Sun, Dan; Meng, Dong; Cai, Yunhao
- Journal of the American Chemical Society, Vol. 137, Issue 34
High-Performance Solution-Processed Non-Fullerene Organic Solar Cells Based on Selenophene-Containing Perylene Bisimide Acceptor
journal, December 2015
- Meng, Dong; Sun, Dan; Zhong, Chengmei
- Journal of the American Chemical Society, Vol. 138, Issue 1
Molecular helices as electron acceptors in high-performance bulk heterojunction solar cells
journal, September 2015
- Zhong, Yu; Trinh, M. Tuan; Chen, Rongsheng
- Nature Communications, Vol. 6, Issue 1
Endohedral fullerenes for organic photovoltaic devices
journal, February 2009
- Ross, Russel B.; Cardona, Claudia M.; Guldi, Dirk M.
- Nature Materials, Vol. 8, Issue 3
Soft x-ray scattering facility at the Advanced Light Source with real-time data processing and analysis
journal, April 2012
- Gann, E.; Young, A. T.; Collins, B. A.
- Review of Scientific Instruments, Vol. 83, Issue 4
Works referencing / citing this record:
Achieving a High Fill Factor and Stability in Perylene Diimide–Based Polymer Solar Cells Using the Molecular Lock Effect between 4,4′‐Bipyridine and a Tri(8‐hydroxyquinoline)aluminum(III) Core
journal, May 2019
- Zhang, Guangjun; Xu, Xiaopeng; Lee, Young Woong
- Advanced Functional Materials, Vol. 29, Issue 29
Design of Diketopyrrolopyrrole (DPP)-Based Small Molecules for Organic-Solar-Cell Applications
journal, November 2016
- Tang, Ailing; Zhan, Chuanlang; Yao, Jiannian
- Advanced Materials, Vol. 29, Issue 2
Ternary Organic Solar Cells Based on Two Compatible Nonfullerene Acceptors with Power Conversion Efficiency >10%
journal, September 2016
- Liu, Tao; Guo, Yuan; Yi, Yuanping
- Advanced Materials, Vol. 28, Issue 45
Nonfullerene Tandem Organic Solar Cells with High Open-Circuit Voltage of 1.97 V
journal, September 2016
- Liu, Wenqing; Li, Shuixing; Huang, Jiang
- Advanced Materials, Vol. 28, Issue 44
Alkyl Side-Chain Engineering in Wide-Bandgap Copolymers Leading to Power Conversion Efficiencies over 10%
journal, December 2016
- Liu, Tao; Pan, Xuexue; Meng, Xiangyi
- Advanced Materials, Vol. 29, Issue 6
Recent Advances in Wide-Bandgap Photovoltaic Polymers
journal, March 2017
- Cai, Yunhao; Huo, Lijun; Sun, Yanming
- Advanced Materials, Vol. 29, Issue 22
Isomerization of Perylene Diimide Based Acceptors Enabling High‐Performance Nonfullerene Organic Solar Cells with Excellent Fill Factor
journal, January 2019
- Luo, Zhenghui; Liu, Tao; Chen, Zhanxiang
- Advanced Science, Vol. 6, Issue 6
Donor Derivative Incorporation: An Effective Strategy toward High Performance All‐Small‐Molecule Ternary Organic Solar Cells
journal, August 2019
- Tang, Hua; Xu, Tongle; Yan, Cenqi
- Advanced Science, Vol. 6, Issue 21
Effect of Benzene Rings’ Incorporation on Photovoltaic Performance of Indacenodithiophene-cored Molecular Acceptors
journal, February 2018
- Fan, Haijun; Wu, Hao; Wang, Pengfei
- Chinese Journal of Chemistry, Vol. 36, Issue 4
A Novel Thiophene-Fused Ending Group Enabling an Excellent Small Molecule Acceptor for High-Performance Fullerene-Free Polymer Solar Cells with 11.8% Efficiency
journal, May 2017
- Xie, Dongjun; Liu, Tao; Gao, Wei
- Solar RRL, Vol. 1, Issue 6
Chlorination Strategy‐Induced Abnormal Nanomorphology Tuning in High‐Efficiency Organic Solar Cells: A Study of Phenyl‐Substituted Benzodithiophene‐Based Nonfullerene Acceptors
journal, July 2019
- Yan, Cenqi; Yang, Tao; Gao, Wei
- Solar RRL, Vol. 3, Issue 11
Chalcogen‐Fused Perylene Diimides‐Based Nonfullerene Acceptors for High‐Performance Organic Solar Cells: Insight into the Effect of O, S, and Se
journal, December 2019
- Li, Gang; Wang, Shuaihua; Li, Dandan
- Solar RRL, Vol. 4, Issue 3
Deciphering the Role of Fluorination: Morphological Manipulation Prompts Charge Separation and Reduces Carrier Recombination in All‐Small‐Molecule Photovoltaics
journal, April 2020
- Tang, Hua; Yan, Cenqi; Karuthedath, Safakath
- Solar RRL, Vol. 4, Issue 4
Benzodithiophenedione-based polymers: recent advances in organic photovoltaics
journal, January 2020
- Zheng, Bing; Huo, Lijun; Li, Yongfang
- NPG Asia Materials, Vol. 12, Issue 1
9-Fluorenone and 9,10-anthraquinone potential fused aromatic building blocks to synthesize electron acceptors for organic solar cells
journal, January 2017
- Do, Thu Trang; Rundel, Kira; Gu, Qinying
- New Journal of Chemistry, Vol. 41, Issue 8
Influence of alkyl chains on photovoltaic properties of 3D rylene propeller electron acceptors
journal, January 2017
- Fu, Huiting; Meng, Dong; Meng, Xiangyi
- Journal of Materials Chemistry A, Vol. 5, Issue 7
A three-dimensional thiophene-annulated perylene bisimide as a fullerene-free acceptor for a high performance polymer solar cell with the highest PCE of 8.28% and a V OC over 1.0 V
journal, January 2018
- Luo, Zhenghui; Liu, Tao; Cheng, Wanli
- Journal of Materials Chemistry C, Vol. 6, Issue 5
Pyran-annulated perylene diimide derivatives as non-fullerene acceptors for high performance organic solar cells
journal, January 2018
- Li, Gang; Zhang, Yu; Liu, Tao
- Journal of Materials Chemistry C, Vol. 6, Issue 41
Non-fullerene acceptor engineering with three-dimensional thiophene/selenophene-annulated perylene diimides for high performance polymer solar cells
journal, January 2018
- Li, Gang; Wang, Shuaihua; Liu, Tao
- Journal of Materials Chemistry C, Vol. 6, Issue 46
A fully fused non-fullerene acceptor containing angular-shaped S , N -heteroacene and perylene diimide for additive-free organic solar cells
journal, January 2019
- Li, Zhaoning; Wang, Jungan; Huang, Hongyan
- New Journal of Chemistry, Vol. 43, Issue 35
Functionalizing tetraphenylpyrazine with perylene diimides (PDIs) as high-performance nonfullerene acceptors
journal, January 2019
- Li, Gang; Yang, Shufan; Liu, Tao
- Journal of Materials Chemistry C, Vol. 7, Issue 46
Comparing non-fullerene acceptors with fullerene in polymer solar cells: a case study with FTAZ and PyCNTAZ
text, January 2017
- F., So,; H., Ade,; L., Yan,
- The University of North Carolina at Chapel Hill University Libraries
A Novel Thiophene-fused Ending Group Enabling an Excellent Small Molecule Acceptor for High-performance Fullerene-free Polymer Solar Cells with 11.8% Efficiency
preprint, January 2017
- Xie, Dongjun; Liu, Tao; Gao, Wei
- arXiv