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Title: Observation of a three-dimensional quasi-long-range electronic supermodulation in YBa 2Cu 3O 7-x/La 0.7Ca 0.3MnO 3 heterostructures

Abstract

Recent developments in high-temperature superconductivity highlight a generic tendency of the cuprates to develop competing electronic (charge) supermodulations. While coupled with the lattice and showing different characteristics in different materials, these supermodulations themselves are generally conceived to be quasi-two-dimensional, residing mainly in individual CuO 2 planes, and poorly correlated along the c axis. Here we observed with resonant elastic X-ray scattering a distinct type of electronic supermodulation in YBa 2Cu 3O 7–x (YBCO) thin films grown epitaxially on La 0.7Ca 0.3MnO 3 (LCMO). This supermodulation has a periodicity nearly commensurate with four lattice constants in-plane, eight out of plane, with long correlation lengths in three dimensions. It sets in far above the superconducting transition temperature and competes with superconductivity below this temperature for electronic states predominantly in the CuO 2 plane. Our finding sheds light on the nature of charge ordering in cuprates as well as a reported long-range proximity effect between superconductivity and ferromagnetism in YBCO/LCMO heterostructures.

Authors:
 [1];  [2];  [1];  [3];  [4];  [1];  [2];  [2];  [1];  [5];  [6];  [2];  [1]
  1. Boston College, Chestnut Hill, MA (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  3. National Chiao Tung Univ., Hsinchu (Taiwan)
  4. Durham Univ., Durham (United Kingdom)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); National Chiao Tung Univ., Hsinchu (Taiwan)
  6. Academia Sinica, Taipei (Taiwan); National Chiao Tung Univ., Hsinchu (Taiwan)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1379124
Grant/Contract Number:  
AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
Journal Volume: 7; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Electronic properties and materials; Superconducting properties and materials

Citation Formats

He, Junfeng, Shafer, Padraic, Mion, Thomas R., Tra, Vu Thanh, He, Qing, Kong, J., Chuang, Y. -D., Yang, W. L., Graf, M. J., Lin, J. -Y., Chu, Y. -H., Arenholz, E., and He, Rui -Hua. Observation of a three-dimensional quasi-long-range electronic supermodulation in YBa2Cu3O7-x/La0.7Ca0.3MnO3 heterostructures. United States: N. p., 2016. Web. doi:10.1038/ncomms10852.
He, Junfeng, Shafer, Padraic, Mion, Thomas R., Tra, Vu Thanh, He, Qing, Kong, J., Chuang, Y. -D., Yang, W. L., Graf, M. J., Lin, J. -Y., Chu, Y. -H., Arenholz, E., & He, Rui -Hua. Observation of a three-dimensional quasi-long-range electronic supermodulation in YBa2Cu3O7-x/La0.7Ca0.3MnO3 heterostructures. United States. doi:10.1038/ncomms10852.
He, Junfeng, Shafer, Padraic, Mion, Thomas R., Tra, Vu Thanh, He, Qing, Kong, J., Chuang, Y. -D., Yang, W. L., Graf, M. J., Lin, J. -Y., Chu, Y. -H., Arenholz, E., and He, Rui -Hua. Tue . "Observation of a three-dimensional quasi-long-range electronic supermodulation in YBa2Cu3O7-x/La0.7Ca0.3MnO3 heterostructures". United States. doi:10.1038/ncomms10852. https://www.osti.gov/servlets/purl/1379124.
@article{osti_1379124,
title = {Observation of a three-dimensional quasi-long-range electronic supermodulation in YBa2Cu3O7-x/La0.7Ca0.3MnO3 heterostructures},
author = {He, Junfeng and Shafer, Padraic and Mion, Thomas R. and Tra, Vu Thanh and He, Qing and Kong, J. and Chuang, Y. -D. and Yang, W. L. and Graf, M. J. and Lin, J. -Y. and Chu, Y. -H. and Arenholz, E. and He, Rui -Hua},
abstractNote = {Recent developments in high-temperature superconductivity highlight a generic tendency of the cuprates to develop competing electronic (charge) supermodulations. While coupled with the lattice and showing different characteristics in different materials, these supermodulations themselves are generally conceived to be quasi-two-dimensional, residing mainly in individual CuO2 planes, and poorly correlated along the c axis. Here we observed with resonant elastic X-ray scattering a distinct type of electronic supermodulation in YBa2Cu3O7–x (YBCO) thin films grown epitaxially on La0.7Ca0.3MnO3 (LCMO). This supermodulation has a periodicity nearly commensurate with four lattice constants in-plane, eight out of plane, with long correlation lengths in three dimensions. It sets in far above the superconducting transition temperature and competes with superconductivity below this temperature for electronic states predominantly in the CuO2 plane. Our finding sheds light on the nature of charge ordering in cuprates as well as a reported long-range proximity effect between superconductivity and ferromagnetism in YBCO/LCMO heterostructures.},
doi = {10.1038/ncomms10852},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {2016},
month = {3}
}

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Works referenced in this record:

Charge ordering in La 1.8 x Eu 0.2 Sr x CuO 4 studied by resonant soft x-ray diffraction
journal, March 2009


Ubiquitous Interplay Between Charge Ordering and High-Temperature Superconductivity in Cuprates
journal, December 2013


Ferromagnetic/superconducting proximity effect in La 0.7 Ca 0.3 MnO 3 / YBa 2 Cu 3 O 7 δ superlattices
journal, June 2003


Long-range transfer of electron–phonon coupling in oxide superlattices
journal, July 2012

  • Driza, N.; Blanco-Canosa, S.; Bakr, M.
  • Nature Materials, Vol. 11, Issue 8
  • DOI: 10.1038/nmat3378

Interface control of bulk ferroelectric polarization
journal, May 2012

  • Yu, P.; Luo, W.; Yi, D.
  • Proceedings of the National Academy of Sciences, Vol. 109, Issue 25
  • DOI: 10.1073/pnas.1117990109

Colloquium : Theory of intertwined orders in high temperature superconductors
journal, May 2015

  • Fradkin, Eduardo; Kivelson, Steven A.; Tranquada, John M.
  • Reviews of Modern Physics, Vol. 87, Issue 2
  • DOI: 10.1103/RevModPhys.87.457

Competing charge, spin, and superconducting orders in underdoped YBa 2 Cu 3 O y
journal, August 2014


Resonant x-ray scattering study of charge-density wave correlations in YBa 2 Cu 3 O 6 + x
journal, August 2014


Oxygen Superstructures Throughout the Phase Diagram of ( Y , C a ) B a 2 C u 3 O 6 + x
journal, October 2004


Four-Unit-Cell Superstructure in the Optimally Doped Y B a 2 C u 3 O 6.92 Superconductor
journal, October 2004


Proximity induced metal-insulator transition in YBa 2 Cu 3 O 7 / La 2 / 3 Ca 1 / 3 MnO 3 superlattices
journal, February 2004


Magnetism at the interface between ferromagnetic and superconducting oxides
journal, April 2006

  • Chakhalian, J.; Freeland, J. W.; Srajer, G.
  • Nature Physics, Vol. 2, Issue 4
  • DOI: 10.1038/nphys272

Incipient charge order observed by NMR in the normal state of YBa2Cu3Oy
journal, March 2015

  • Wu, Tao; Mayaffre, Hadrien; Krämer, Steffen
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7438

Visualizing short-range charge transfer at the interfaces between ferromagnetic and superconducting oxides
journal, August 2013

  • Chien, Te Yu; Kourkoutis, Lena F.; Chakhalian, Jak
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3336

Quenched disorder and vestigial nematicity in the pseudogap regime of the cuprates
journal, May 2014

  • Nie, L.; Tarjus, G.; Kivelson, S. A.
  • Proceedings of the National Academy of Sciences, Vol. 111, Issue 22
  • DOI: 10.1073/pnas.1406019111

Charge Order Driven by Fermi-Arc Instability in Bi2Sr2-xLaxCuO6+ 
journal, December 2013


Long-Range Incommensurate Charge Fluctuations in (Y,Nd)Ba2Cu3O6+x
journal, July 2012


Comparison of charge modulations in La 1.875 Ba 0.125 CuO 4 and YBa 2 Cu 3 O 6.6
journal, July 2013


A ‘checkerboard’ electronic crystal state in lightly hole-doped Ca2-xNaxCuO2Cl2
journal, August 2004


Thickness effect on the structure and superconductivity of Nd 1.2 Ba 1.8 Cu 3 O z epitaxial films
journal, October 2005


Suppressed magnetization in La 0.7 Ca 0.3 MnO 3 YBa 2 Cu 3 O 7 δ superlattices
journal, October 2005


Direct spectroscopic evidence for phase competition between the pseudogap and superconductivity in Bi2Sr2CaCu2O8+δ
journal, November 2014

  • Hashimoto, Makoto; Nowadnick, Elizabeth A.; He, Rui-Hua
  • Nature Materials, Vol. 14, Issue 1
  • DOI: 10.1038/nmat4116

Magnetic-field-induced charge-stripe order in the high-temperature superconductor YBa2Cu3Oy
journal, September 2011

  • Wu, Tao; Mayaffre, Hadrien; Krämer, Steffen
  • Nature, Vol. 477, Issue 7363
  • DOI: 10.1038/nature10345

Proximity effects in superconductor-ferromagnet heterostructures
journal, September 2005


Spatially modulated 'Mottness' in La2-xBaxCuO4
journal, December 2005

  • Abbamonte, P.; Rusydi, A.; Smadici, S.
  • Nature Physics, Vol. 1, Issue 3
  • DOI: 10.1038/nphys178

Orbital Reconstruction and Covalent Bonding at an Oxide Interface
journal, November 2007


Inelastic X-ray scattering in YBa2Cu3O6.6 reveals giant phonon anomalies and elastic central peak due to charge-density-wave formation
journal, November 2013

  • Le Tacon, M.; Bosak, A.; Souliou, S. M.
  • Nature Physics, Vol. 10, Issue 1
  • DOI: 10.1038/nphys2805

Microscopic Coexistence of Superconductivity and Magnetism in Ba 1 x K x Fe 2 As 2
journal, November 2011


Coexistence of periodic modulation of quasiparticle states and superconductivity in Bi2Sr2CaCu2O8+ 
journal, August 2003

  • Howald, C.; Eisaki, H.; Kaneko, N.
  • Proceedings of the National Academy of Sciences, Vol. 100, Issue 17
  • DOI: 10.1073/pnas.1233768100

Charge ordering in the electron-doped superconductor Nd2-xCexCuO4
journal, January 2015


Charge stripe order near the surface of 12-percent doped La2−xSrxCuO4
journal, January 2012

  • Wu, H. -H.; Buchholz, M.; Trabant, C.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms2019

Direct observation of competition between superconductivity and charge density wave order in YBa2Cu3O6.67
journal, October 2012

  • Chang, J.; Blackburn, E.; Holmes, A. T.
  • Nature Physics, Vol. 8, Issue 12
  • DOI: 10.1038/nphys2456

Charge order and its connection with Fermi-liquid charge transport in a pristine high-Tc cuprate
journal, December 2014

  • Tabis, W.; Li, Y.; Tacon, M. Le
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6875

Coupling of superconductors through a half-metallic ferromagnet: Evidence for a long-range proximity effect
journal, June 2004


Charge-density-wave origin of cuprate checkerboard visualized by scanning tunnelling microscopy
journal, July 2008

  • Wise, W. D.; Boyer, M. C.; Chatterjee, Kamalesh
  • Nature Physics, Vol. 4, Issue 9
  • DOI: 10.1038/nphys1021

Giant superconductivity-induced modulation of the ferromagnetic magnetization in a cuprate–manganite superlattice
journal, February 2009

  • Hoppler, J.; Stahn, J.; Niedermayer, Ch.
  • Nature Materials, Vol. 8, Issue 4, p. 315-319
  • DOI: 10.1038/nmat2383

Resonant elastic soft x-ray scattering in oxygen-ordered YBa 2 Cu 3 O 6 + δ
journal, August 2011


Attenuation of superconductivity in manganite/cuprate heterostructures by epitaxially-induced CuO intergrowths
journal, July 2013

  • Zhang, H.; Gauquelin, N.; Botton, G. A.
  • Applied Physics Letters, Vol. 103, Issue 5
  • DOI: 10.1063/1.4813840

Evidence for stripe correlations of spins and holes in copper oxide superconductors
journal, June 1995

  • Tranquada, J. M.; Sternlieb, B. J.; Axe, J. D.
  • Nature, Vol. 375, Issue 6532
  • DOI: 10.1038/375561a0