Uncovering the deactivation mechanism of Au catalyst with operando high spatial resolution IR and X-ray microspectroscopy measurements
- Authors:
- Publication Date:
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1378137
- Resource Type:
- Publisher's Accepted Manuscript
- Journal Name:
- Surface Science
- Additional Journal Information:
- Journal Name: Surface Science Journal Volume: 648 Journal Issue: C; Journal ID: ISSN 0039-6028
- Publisher:
- Elsevier
- Country of Publication:
- Netherlands
- Language:
- English
Citation Formats
Gross, Elad. Uncovering the deactivation mechanism of Au catalyst with operando high spatial resolution IR and X-ray microspectroscopy measurements. Netherlands: N. p., 2016.
Web. doi:10.1016/j.susc.2015.11.007.
Gross, Elad. Uncovering the deactivation mechanism of Au catalyst with operando high spatial resolution IR and X-ray microspectroscopy measurements. Netherlands. https://doi.org/10.1016/j.susc.2015.11.007
Gross, Elad. Wed .
"Uncovering the deactivation mechanism of Au catalyst with operando high spatial resolution IR and X-ray microspectroscopy measurements". Netherlands. https://doi.org/10.1016/j.susc.2015.11.007.
@article{osti_1378137,
title = {Uncovering the deactivation mechanism of Au catalyst with operando high spatial resolution IR and X-ray microspectroscopy measurements},
author = {Gross, Elad},
abstractNote = {},
doi = {10.1016/j.susc.2015.11.007},
journal = {Surface Science},
number = C,
volume = 648,
place = {Netherlands},
year = {Wed Jun 01 00:00:00 EDT 2016},
month = {Wed Jun 01 00:00:00 EDT 2016}
}
Free Publicly Available Full Text
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https://doi.org/10.1016/j.susc.2015.11.007
https://doi.org/10.1016/j.susc.2015.11.007
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Cited by: 10 works
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Works referenced in this record:
Reaction Kinetics and Polarization-Modulation Infrared Reflection Absorption Spectroscopy (PM-IRAS) Investigation of CO Oxidation over Supported Pd−Au Alloy Catalysts
journal, February 2010
- Gao, Feng; Wang, Yilin; Goodman, D. Wayne
- The Journal of Physical Chemistry C, Vol. 114, Issue 9
Spectroscopic Study of Platinum and Rhodium Dendrimer (PAMAM G4OH) Compounds: Structure and Stability
journal, February 2011
- Borodko, Yuri; Thompson, Christopher M.; Huang, Wenyu
- The Journal of Physical Chemistry C, Vol. 115, Issue 11
The Impact of Nanoscience on Heterogeneous Catalysis
journal, March 2003
- Bell, A. T.
- Science, Vol. 299, Issue 5613
Magnetic resonance imaging methods for in situ studies in heterogeneous catalysis
journal, January 2010
- Lysova, Anna A.; Koptyug, Igor V.
- Chemical Society Reviews, Vol. 39, Issue 12
Time-resolved observations of water oxidation intermediates on a cobalt oxide nanoparticle catalyst
journal, February 2014
- Zhang, Miao; de Respinis, Moreno; Frei, Heinz
- Nature Chemistry, Vol. 6, Issue 4
Heterogeneities of individual catalyst particles in space and time as monitored by spectroscopy
journal, October 2012
- Buurmans, Inge L. C.; Weckhuysen, Bert M.
- Nature Chemistry, Vol. 4, Issue 11
High-resolution Fourier-transform infrared chemical imaging with multiple synchrotron beams
journal, March 2011
- Nasse, Michael J.; Walsh, Michael J.; Mattson, Eric C.
- Nature Methods, Vol. 8, Issue 5
Multistep continuous-flow synthesis of (R)- and (S)-rolipram using heterogeneous catalysts
journal, April 2015
- Tsubogo, Tetsu; Oyamada, Hidekazu; Kobayashi, Shū
- Nature, Vol. 520, Issue 7547
Gold(I)-Catalyzed Synthesis of Dihydropyrans
journal, June 2006
- Sherry, Benjamin D.; Maus, Lisa; Laforteza, Brian Ngo
- Journal of the American Chemical Society, Vol. 128, Issue 25
Monitoring surface metal oxide catalytic active sites with Raman spectroscopy
journal, January 2010
- Wachs, Israel E.; Roberts, Charles A.
- Chemical Society Reviews, Vol. 39, Issue 12
Dendrimer Templated Synthesis of One Nanometer Rh and Pt Particles Supported on Mesoporous Silica: Catalytic Activity for Ethylene and Pyrrole Hydrogenation
journal, July 2008
- Huang, Wenyu; Kuhn, John N.; Tsung, Chia-Kuang
- Nano Letters, Vol. 8, Issue 7
Infrared and Raman imaging of heterogeneous catalysts
journal, January 2010
- Stavitski, Eli; Weckhuysen, Bert M.
- Chemical Society Reviews, Vol. 39, Issue 12
Exploring catalytic solid/liquid interfaces by in situ attenuated total reflection infrared spectroscopy
journal, January 2010
- Andanson, Jean-Michel; Baiker, Alfons
- Chemical Society Reviews, Vol. 39, Issue 12
Furfuraldehyde Hydrogenation on Titanium Oxide-Supported Platinum Nanoparticles Studied by Sum Frequency Generation Vibrational Spectroscopy: Acid–Base Catalysis Explains the Molecular Origin of Strong Metal–Support Interactions
journal, August 2012
- Baker, L. Robert; Kennedy, Griffin; Van Spronsen, Matthijs
- Journal of the American Chemical Society, Vol. 134, Issue 34
Frontiers of surface science
journal, October 2007
- Somorjai, Gabor A.; Park, Jeong Y.
- Physics Today, Vol. 60, Issue 10
Deciding Whether To Go with the Flow: Evaluating the Merits of Flow Reactors for Synthesis
journal, June 2011
- Hartman, Ryan L.; McMullen, Jonathan P.; Jensen, Klavs F.
- Angewandte Chemie International Edition, Vol. 50, Issue 33
In Situ Surface and Reaction Probe Studies with Model Nanoparticle Catalysts
journal, September 2012
- Alayoglu, Selim; Krier, James M.; Michalak, William D.
- ACS Catalysis, Vol. 2, Issue 11
Reaction-Driven Restructuring of Rh-Pd and Pt-Pd Core-Shell Nanoparticles
journal, November 2008
- Tao, F.; Grass, M. E.; Zhang, Y.
- Science, Vol. 322, Issue 5903
Steam reforming of methanol on PdZn near-surface alloys on Pd(111) and Pd foil studied by in-situ XPS, LEIS and PM-IRAS
journal, November 2010
- Rameshan, Christoph; Weilach, Christian; Stadlmayr, Werner
- Journal of Catalysis, Vol. 276, Issue 1
Direct Observation of Kinetically Competent Surface Intermediates upon Ethylene Hydroformylation over Rh/Al 2 O 3 under Reaction Conditions by Time-Resolved Fourier Transform Infrared Spectroscopy
journal, March 2011
- Sivasankar, N.; Frei, H.
- The Journal of Physical Chemistry C, Vol. 115, Issue 15
Dual Visible Light Photoredox and Gold-Catalyzed Arylative Ring Expansion
journal, April 2014
- Shu, Xing-zhong; Zhang, Miao; He, Ying
- Journal of the American Chemical Society, Vol. 136, Issue 16
A Pt-Cluster-Based Heterogeneous Catalyst for Homogeneous Catalytic Reactions: X-ray Absorption Spectroscopy and Reaction Kinetic Studies of Their Activity and Stability against Leaching
journal, August 2011
- Li, Yimin; Liu, Jack Hung-Chang; Witham, Cole A.
- Journal of the American Chemical Society, Vol. 133, Issue 34
Break-Up of Stepped Platinum Catalyst Surfaces by High CO Coverage
journal, February 2010
- Tao, F.; Dag, S.; Wang, L. -W.
- Science, Vol. 327, Issue 5967
In Situ IR and X-ray High Spatial-Resolution Microspectroscopy Measurements of Multistep Organic Transformation in Flow Microreactor Catalyzed by Au Nanoclusters
journal, February 2014
- Gross, Elad; Shu, Xing-Zhong; Alayoglu, Selim
- Journal of the American Chemical Society, Vol. 136, Issue 9
Snapshots of a working catalyst: possibilities and limitations of in situ spectroscopy in the field of heterogeneous catalysis
journal, January 2002
- Weckhuysen, Bert M.
- Chemical Communications, Issue 2
Detection of Carbocationic Species in Zeolites: Large Crystals Pave the Way
journal, July 2010
- Stavitski, Eli; Pidko, Evgeny A.; Kox, Marianne H. F.
- Chemistry - A European Journal, Vol. 16, Issue 31
2D-Mapping of the Catalyst Structure Inside a Catalytic Microreactor at Work: Partial Oxidation of Methane over Rh/Al 2 O 3
journal, May 2006
- Grunwaldt, Jan-Dierk; Hannemann, Stefan; Schroer, Christian G.
- The Journal of Physical Chemistry B, Vol. 110, Issue 17
Molecular Factors of Catalytic Selectivity
journal, November 2008
- Somorjai, Gabor A.; Park, Jeong Y.
- Angewandte Chemie International Edition, Vol. 47, Issue 48
Control of selectivity in heterogeneous catalysis by tuning nanoparticle properties and reactor residence time
journal, September 2012
- Gross, Elad; Liu, Jack Hung-Chang; Toste, F. Dean
- Nature Chemistry, Vol. 4, Issue 11
Nanocatalysis in continuous flow: supported iron oxide nanoparticles for the heterogeneous aerobic oxidation of benzyl alcohol
journal, January 2013
- Obermayer, David; Balu, Alina M.; Romero, Antonio A.
- Green Chemistry, Vol. 15, Issue 6
Selective Amplification of CO Bond Hydrogenation on Pt/TiO 2 : Catalytic Reaction and Sum-Frequency Generation Vibrational Spectroscopy Studies of Crotonaldehyde Hydrogenation
journal, February 2014
- Kennedy, Griffin; Baker, L. Robert; Somorjai, Gabor A.
- Angewandte Chemie International Edition, Vol. 53, Issue 13
Polymer-Encapsulated Metallic Nanoparticles as a Bridge Between Homogeneous and Heterogeneous Catalysis
journal, November 2014
- Gross, Elad; Dean Toste, F.; Somorjai, Gabor A.
- Catalysis Letters, Vol. 145, Issue 1
In Situ Synchrotron-Based IR Microspectroscopy To Study Catalytic Reactions in Zeolite Crystals
journal, April 2008
- Stavitski, Eli; Kox, Marianne H. F.; Swart, Ingmar
- Angewandte Chemie International Edition, Vol. 47, Issue 19
Converting homogeneous to heterogeneous in electrophilic catalysis using monodisperse metal nanoparticles
journal, November 2009
- Witham, Cole A.; Huang, Wenyu; Tsung, Chia-Kuang
- Nature Chemistry, Vol. 2, Issue 1
Asymmetric Catalysis at the Mesoscale: Gold Nanoclusters Embedded in Chiral Self-Assembled Monolayer as Heterogeneous Catalyst for Asymmetric Reactions
journal, March 2013
- Gross, Elad; Liu, Jack H.; Alayoglu, Selim
- Journal of the American Chemical Society, Vol. 135, Issue 10
Label-Free Chemical Imaging of Catalytic Solids by Coherent Anti-Stokes Raman Scattering and Synchrotron-Based Infrared Microscopy
journal, November 2009
- Kox, Marianne���H. ���F.; Domke, Katrin���F.; Day, James���P. ���R.
- Angewandte Chemie International Edition, Vol. 48, Issue 47