Tricritical point of the f-electron antiferromagnet USb2 driven by high magnetic fields

Stillwell, R. L.; Liu, I. -L.; Harrison, Neil; Jaime, Marcelo; Jeffries, J. R.; Butch, N. P.

doi:10.1103/PhysRevB.95.014414

Title: Tricritical point of the $f$ -electron antiferromagnet $US b_{2}$ driven by high magnetic fields

Abstract

In pulsed magnetic fields up to 65 T and at temperatures below the Néel transition, our magnetization and magnetostriction measurements reveal a field-induced metamagneticlike transition that is suggestive of an antiferromagnetic to ferrimagnetic ordering. Our data also suggest a change in the nature of this metamagneticlike transition from second- to first-order-like near a tricritical point at T_tc ~ 145K and H_c ~ 52 T. At high fields for H > H_c we found a decreased magnetic moment roughly half of the moment determined by neutron powder diffraction. Lastly, we propose that the decreased moment and lack of saturation at high fields indicate the presence of a field-induced ferrimagnetic state above the tricritical point of the H-T phase diagram for USb₂.

Authors:

Stillwell, R. L. ^[1]; Liu, I. -L. ^[2];

^[3];

^[3]; Jeffries, J. R. ^[1]; Butch, N. P. ^[4]

Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of Maryland, College Park, MD (United States); National Institute of Science and Technology, Gaithersburg, MD (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
National Institute of Science and Technology, Gaithersburg, MD (United States); Univ. of Maryland, College Park, MD (United States)

Publication Date:: Thu Jan 12 00:00:00 EST 2017

Research Org.:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1343719

Alternate Identifier(s):: OSTI ID: 1339182; OSTI ID: 1377774

Report Number(s):: LA-UR-16-28417; LLNL-JRNL-702128
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1700992

Grant/Contract Number:: AC52-06NA25396; 14-ERD-041; AC52-07NA27344

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 95; Journal Issue: 1; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science

Citation Formats


                    Stillwell, R. L., Liu, I. -L., Harrison, Neil, Jaime, Marcelo, Jeffries, J. R., and Butch, N. P. Tricritical point of the f-electron antiferromagnet USb2 driven by high magnetic fields.  United States: N. p., 2017. 
Web.  doi:10.1103/PhysRevB.95.014414.

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                    Stillwell, R. L., Liu, I. -L., Harrison, Neil, Jaime, Marcelo, Jeffries, J. R., & Butch, N. P. Tricritical point of the f-electron antiferromagnet USb2 driven by high magnetic fields.  United States.  https://doi.org/10.1103/PhysRevB.95.014414

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                    Stillwell, R. L., Liu, I. -L., Harrison, Neil, Jaime, Marcelo, Jeffries, J. R., and Butch, N. P. Thu .  
"Tricritical point of the f-electron antiferromagnet USb2 driven by high magnetic fields".  United States.  https://doi.org/10.1103/PhysRevB.95.014414.  https://www.osti.gov/servlets/purl/1343719.

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@article{osti_1343719,

  title        = {Tricritical point of the f-electron antiferromagnet USb2 driven by high magnetic fields},

  author       = {Stillwell, R. L. and Liu, I. -L. and Harrison, Neil and Jaime, Marcelo and Jeffries, J. R. and Butch, N. P.},

  abstractNote = {In pulsed magnetic fields up to 65 T and at temperatures below the Néel transition, our magnetization and magnetostriction measurements reveal a field-induced metamagneticlike transition that is suggestive of an antiferromagnetic to ferrimagnetic ordering. Our data also suggest a change in the nature of this metamagneticlike transition from second- to first-order-like near a tricritical point at Ttc ~ 145K and Hc ~ 52 T. At high fields for H > Hc we found a decreased magnetic moment roughly half of the moment determined by neutron powder diffraction. Lastly, we propose that the decreased moment and lack of saturation at high fields indicate the presence of a field-induced ferrimagnetic state above the tricritical point of the H-T phase diagram for USb2.},

  doi          = {10.1103/PhysRevB.95.014414},

  journal      = {Physical Review B},

  number       = 1,

  volume       = 95,

  place        = {United States},

  year         = {Thu Jan 12 00:00:00 EST 2017},

  month        = {Thu Jan 12 00:00:00 EST 2017}

}

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High temperature singlet-based magnetism from Hund’s rule correlations
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Miao, Lin; Basak, Rourav; Ran, Sheng
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Tricritical point from high-field magnetoelastic and metamagnetic effects in UN
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Structure, elastic characteristic, ideal strengths, and phonon stability of binary uranium intermetallic UGe ₃ of AuCu ₃ -type
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High temperature singlet-based magnetism from Hund's rule correlations
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Miao, Lin; Basak, Rourav; Ran, Sheng
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Title: Tricritical point of the f -electron antiferromagnet US b 2 driven by high magnetic fields

Abstract

Citation Formats

High-Temperature Magnetic Investigations on Uranium Compounds journal, May 2005

Anisotropy of the physical properties of uniaxial antiferromagnetic USb2 journal, April 1992

Tricritical-Point Phase Diagram in Fe Cl 2 journal, October 1974

Angle-resolved photoemission study of USb 2 : The 5 f band structure journal, January 2004

Cylindrical Fermi surfaces formed by a fiat magnetic Brillouin zone in uranium dipnictides journal, August 2000

High resolution magnetostriction measurements in pulsed magnetic fields using fiber Bragg gratings journal, March 2010

Heavy-fermion systems journal, October 1984

Magnetic anisotropy of single crystals of rocksalttype uranium compounds journal, November 1978

Neutron diffraction study of UAs in high magnetic fields journal, December 1979

Field-induced phases in UPt 2 Si 2 journal, February 2012

Magnetostriction and magnetic texture to 100.75 Tesla in frustrated SrCu2(BO3)2 journal, July 2012

Crystal Growth and Cylindrical Fermi Surfaces of USb 2 journal, July 1999

Exploration of magnetic excitation behaviour of actinide compounds with neutron scattering journal, February 1983

Magnetization of UBe 13 to 60 T journal, January 2000

Interplay between quantum fluctuations and reentrant superconductivity with a highly enhanced upper critical field in URhGe journal, May 2016

Metamagnetic transition in single-crystal Bi 4 Cu 3 V 2 O 14 journal, August 2010

Nature of the 5 f states in actinide metals journal, February 2009

Metamagnetism of Ni ( N O 3 ) 2 .2 H 2 O journal, March 1970

Neutron-Diffraction Study of Antiferromagnetism in USb2 and UBi2 journal, January 1967

Shubnikov-de Haas effect study of cylindrical Fermi surfaces in UAs 2 journal, February 2000

Incommensurate-Commensurate Magnetic Phase Transitions of the Ising-5 f System UPd 2 Si 2 : the H - T Phase Diagram and Mean-Field Analyses journal, March 1998

Electronic properties of UNiAl in high magnetic fields journal, April 1994

Successive Field Induced Magnetic Phase Transitions of Heavy Fermion Compound CeRh 2 Si 2 journal, August 1997

Magnetic and magnetoelastic properties of UCo 2 Si 2 as studied by high-field magnetization and ultrasound measurements journal, June 2013

Emergent ferromagnetism and T -linear scattering in USb 2 at high pressure journal, May 2016

Crystal field interpretation of the magnetic properties of UX2 compounds (X = P, As, Sb, Bi) journal, March 1984

Magnetism and structural distortions in uranium sulfide under pressure journal, June 2013

Susceptibility anisotropy in the (Ce,La)Ru2Si2 system journal, October 1992

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Spin-lattice effects in selected antiferromagnetic materials (Review Article) journal, February 2014

A single-solenoid pulsed-magnet system for single-crystal scattering studies journal, March 2012

High-field magnetism and magnetoacoustics in uranium intermetallic antiferromagnets journal, October 2012

Antiferromagnetisme Dans Un Champ Magnetique I. Traitement De Champ Moleculaire journal, January 1967

Dependence of ordering temperature on pressure, carrier density and U-U distance in uranium pnictides; pressure and hall effects examinations of UP2 and USb2 journal, September 1991

Collapse of Ferromagnetism and Fermi Surface Instability near Reentrant Superconductivity of URhGe journal, July 2016

High field magnetization measurements on UP single crystals journal, October 1980

Magnetic and transport properties of UBi 2 and USb 2 single crystals journal, April 2006

Actinide pnictides and chalcogenides. I. study of magnetic ordering and ordered moments in uranium monochalcogenides by neutron diffraction journal, October 1972

Distinct magnetic spectra in the hidden order and antiferromagnetic phases in URu 2 − x Fe x Si 2 journal, November 2016

First-order magnetization process as a tool of magnetic-anisotropy determination: Application to the uranium-based intermetallic U 3 C u 4 G e 4 journal, February 2016

High-field metamagnetism in the antiferromagnet CeRh 2 Si 2 journal, March 2010

Field-induced magnetostructural transition in Gd 5 Ge 4 studied by pulsed magnetic fields journal, May 2008

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Structure, elastic characteristic, ideal strengths, and phonon stability of binary uranium intermetallic UGe 3 of AuCu 3 -type journal, January 2020

Magnetotransport as a probe of phase transformations in metallic antiferromagnets: The case of UIrS i 3 journal, July 2019

Microscopic mechanism for the unusual antiferromagnetic order and the pressure-induced transition to ferromagnetism in USb 2 journal, January 2018

Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion journal, October 2019

Fiber Bragg Grating Dilatometry in Extreme Magnetic Field and Cryogenic Conditions journal, November 2017

Orbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion text, January 2019

High temperature singlet-based magnetism from Hund's rule correlations text, January 2019

Title: Tricritical point of the $f$ -electron antiferromagnet $US b_{2}$ driven by high magnetic fields

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High temperature singlet-based magnetism from Hund’s rule correlations
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Tricritical point from high-field magnetoelastic and metamagnetic effects in UN
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Structure, elastic characteristic, ideal strengths, and phonon stability of binary uranium intermetallic UGe ₃ of AuCu ₃ -type
journal, January 2020

Magnetotransport as a probe of phase transformations in metallic antiferromagnets: The case of $UIrS i_{3}$
journal, July 2019

Microscopic mechanism for the unusual antiferromagnetic order and the pressure-induced transition to ferromagnetism in ${USb}_{2}$
journal, January 2018

Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
journal, October 2019

Fiber Bragg Grating Dilatometry in Extreme Magnetic Field and Cryogenic Conditions
journal, November 2017

Orbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion
text, January 2019

High temperature singlet-based magnetism from Hund's rule correlations
text, January 2019