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Title: High-Performance Polymer Solar Cells Based on a Wide-Bandgap Polymer Containing Pyrrolo[3,4- f ]benzotriazole-5,7-dione with a Power Conversion Efficiency of 8.63%

In article 1600032, an efficient new wide-bandgap polymer based on a novel moiety of pyrrolo[3,4-f]benzotriazole-5,7-dione (TZBI) is developed by Lei Ying, Feng Lui, Thomas P. Russel, Fei Huang, and co-workers. The new chemistry enables fine electronic structure tuning and solution-processed single-junction polymer solar cells provided a remarkable power conversion efficiency of 8.63%. Full electrical and structural characterization reveales that TZBI is a promising building block for the application in highly efficient organic photovoltaics.
Authors:
 [1] ;  [1] ;  [2] ;  [1] ;  [2] ;  [3] ;  [3] ;  [1] ;  [1]
  1. South China Univ. of Technology (SCUT), Guangzhou (China). Inst. of Polymer Optoelectronic Materials and Devices State Key Lab. of Luminescent Materials and Devices
  2. Peking Univ., Beijing (China). School of Physics, State Key Lab. for Artificial Microstructure and Mesoscopic Physics
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
Publication Date:
Grant/Contract Number:
AC02-05CH11231; 2014CB643501; 51303056; 21520102006; 51521002; 21490573; N00014-15-1-2244
Type:
Accepted Manuscript
Journal Name:
Advanced Science
Additional Journal Information:
Journal Volume: 3; Journal Issue: 9; Journal ID: ISSN 2198-3844
Publisher:
Wiley
Research Org:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); Natural Science Foundation of China; US Department of the Navy, Office of Naval Research (ONR)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 14 SOLAR ENERGY; polymer solar cells; pyrrolo[3,4-f]benzotriazole-5,7-dione; wide-bandgap polymer
OSTI Identifier:
1377457