Role of band filling in tuning the high-field phases of URu2Si2

Wartenbe, M. R.; Chen, K. -W.; Gallagher, A.; Harrison, N.; McDonald, R. D.; Boebinger, G. S.; Baumbach, R. E.

doi:10.1103/PhysRevB.96.085141

Title: Role of band filling in tuning the high-field phases of ${URu}_{2} {Si}_{2}$

Abstract

We present a detailed study of the low temperature and high magnetic eld phases in the chemical substitution series URu₂Si_2-xPx using electrical transport and magnetization in pulsed magnetic elds up to 65T. Within the hidden order x-regime (0 < x ≲ 0.035) the eld induced ordering that was earlier seen for x = 0 is robust, even as the hidden order temperature is suppressed. Earlier work shows that for 0.035 ≲ x ≲ 0.26 there is a Kondo lattice with a no-ordered state that is replaced by antiferromagnetism for 0.26 ≲ x ≲ 0.5. We observe a simpli ed continuation of the eld induced order in the no-order x-regime and an enhancement of the field induced order upon the destruction of the antiferromagnetism with magnetic field. These results closely resemble what is seen for URu_2-xRhxSi₂ a, from which we infer that charge tuning dominantly controls the ground state of URu₂Si₂, regardless of whether s/p or d-electrons are replaced. Contraction of the unit cell volume may also play a role at large x. This provides guidance for determining the specific factors that lead to hidden order versus magnetism in this family of materials and constrains possible models for hidden order.

Authors:

Wartenbe, M. R. ^[1]; Chen, K. -W. ^[1]; Gallagher, A. ^[1]; Harrison, N. ^[2]; McDonald, R. D. ^[2]; Boebinger, G. S. ^[1]; Baumbach, R. E. ^[1]

Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Publication Date:: Mon Aug 28 00:00:00 EDT 2017

Research Org.:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1412913

Alternate Identifier(s):: OSTI ID: 1377122

Report Number(s):: LA-UR-17-30079
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1800411

Grant/Contract Number:: AC52-06NA25396

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 96; Journal Issue: 8; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science

Citation Formats


                    Wartenbe, M. R., Chen, K. -W., Gallagher, A., Harrison, N., McDonald, R. D., Boebinger, G. S., and Baumbach, R. E. Role of band filling in tuning the high-field phases of URu2Si2.  United States: N. p., 2017. 
Web.  doi:10.1103/PhysRevB.96.085141.

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                    Wartenbe, M. R., Chen, K. -W., Gallagher, A., Harrison, N., McDonald, R. D., Boebinger, G. S., & Baumbach, R. E. Role of band filling in tuning the high-field phases of URu2Si2.  United States.  https://doi.org/10.1103/PhysRevB.96.085141

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                    Wartenbe, M. R., Chen, K. -W., Gallagher, A., Harrison, N., McDonald, R. D., Boebinger, G. S., and Baumbach, R. E. Mon .  
"Role of band filling in tuning the high-field phases of URu2Si2".  United States.  https://doi.org/10.1103/PhysRevB.96.085141.  https://www.osti.gov/servlets/purl/1412913.

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@article{osti_1412913,

  title        = {Role of band filling in tuning the high-field phases of URu2Si2},

  author       = {Wartenbe, M. R. and Chen, K. -W. and Gallagher, A. and Harrison, N. and McDonald, R. D. and Boebinger, G. S. and Baumbach, R. E.},

  abstractNote = {We present a detailed study of the low temperature and high magnetic eld phases in the chemical substitution series URu2Si2-xPx using electrical transport and magnetization in pulsed magnetic elds up to 65T. Within the hidden order x-regime (0 < x ≲ 0.035) the eld induced ordering that was earlier seen for x = 0 is robust, even as the hidden order temperature is suppressed. Earlier work shows that for 0.035 ≲ x ≲ 0.26 there is a Kondo lattice with a no-ordered state that is replaced by antiferromagnetism for 0.26 ≲ x ≲ 0.5. We observe a simpli ed continuation of the eld induced order in the no-order x-regime and an enhancement of the field induced order upon the destruction of the antiferromagnetism with magnetic field. These results closely resemble what is seen for URu2-xRhxSi2 a, from which we infer that charge tuning dominantly controls the ground state of URu2Si2, regardless of whether s/p or d-electrons are replaced. Contraction of the unit cell volume may also play a role at large x. This provides guidance for determining the specific factors that lead to hidden order versus magnetism in this family of materials and constrains possible models for hidden order.},

  doi          = {10.1103/PhysRevB.96.085141},

  journal      = {Physical Review B},

  number       = 8,

  volume       = 96,

  place        = {United States},

  year         = {Mon Aug 28 00:00:00 EDT 2017},

  month        = {Mon Aug 28 00:00:00 EDT 2017}

}

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Works referencing / citing this record:

Instability of the f -electron state in URu 2 Si 2 − x P x probed using high magnetic fields
journal, June 2019

Huang, K.; Chen, K. -W.; Gallagher, A.
Physical Review B, Vol. 99, Issue 23
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Title: Role of band filling in tuning the high-field phases of URu 2 Si 2

Abstract

Citation Formats

Sequential Spin Polarization of the Fermi Surface Pockets in URu 2 Si 2 and Its Implications for the Hidden Order journal, April 2011

Absence of a static in-plane magnetic moment in the ‘hidden-order’ phase of URu 2 Si 2 journal, May 2013

Phase diagram and thermal expansion measurements on the system URu 2− x Fe x Si 2 journal, November 2016

Chemical pressure tuning of URu 2 Si 2 via isoelectronic substitution of Ru with Fe journal, February 2015

High Magnetic Field Studies of the Hidden Order Transition in U R u 2 S i 2 journal, December 2002

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

Metamagnetic Behavior and Effect of Pressure on the Electronic State in Heavy-Fermion Compound YbRh 2 Zn 20 journal, August 2013

Unfolding the physics of URu2Si2 through silicon to phosphorus substitution journal, February 2016

Hybridization model for the magnetic-ordering behavior of uranium- and cerium-based 1:2:2 intermetallic compounds journal, October 1993

Temperature-pressure phase diagram of U Ru 2 Si 2 from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting journal, March 2008

Nature of the 5 f states in actinide metals journal, February 2009

Effect of pressure on competing electronic correlations in the heavy-electron system URu 2 Si 2 journal, January 1987

NMR investigation of antiferromagnetism and coherence in URu 2 Si 2 − x P x journal, January 2017

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2 journal, June 1986

High purity specimens of URu 2 Si 2 produced by a molten metal flux technique journal, April 2014

Effect of transition-metal substitutions on competing electronic transitions in the heavy-electron compound URu 2 Si 2 journal, February 1990

Magnetic properties of the ternary compounds CeT2Si2 and UT2Si2 journal, February 1986

Magnetic Structure of Phase II in U ( Ru 0.96 Rh 0.04 ) 2 Si 2 Determined by Neutron Diffraction under Pulsed High Magnetic Fields journal, May 2013

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of URu 2 Si 2 journal, November 2010

Enhancement of the hidden order/large moment antiferromagnetic transition temperature in the URu 2− x Os x Si 2 system journal, April 2014

Ferromagnetic instability in the heavy-electron compound URu 2 Si 2 doped with Re or Tc journal, February 1989

Field-induced spin-density wave beyond hidden order in URu2Si2 journal, October 2016

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Nexus between Quantum Criticality and Phase Formation in U ( R u 1 − x R h x ) 2 S i 2 journal, November 2004

Magnetic-Field-Induced Quantum Critical Point and Competing Order Parameters in U R u 2 S i 2 journal, December 2003

Hidden order behaviour in URu 2 Si 2 (A critical review of the status of hidden order in 2014) journal, May 2014

The suppression of hidden order and the onset of ferromagnetism in URu 2 Si 2 via Re substitution journal, March 2010

Field Reentrance of the Hidden Order State of URu 2 Si 2 under Pressure journal, May 2009

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu 2 − x Fe x Si 2 system journal, December 2011

Interplay of magnetism, Fermi surface reconstructions, and hidden order in the heavy-fermion material URu 2 Si 2 journal, March 2012

Thermodynamic and electrical transport investigation of URu 2 Si 2− x P x journal, November 2016

Specific heat of URu 2 Si 2 in fields up to 42 T: Clues to the hidden order journal, January 2003

Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7 journal, October 2001

Instability of the f -electron state in URu 2 Si 2 − x P x probed using high magnetic fields journal, June 2019

Title: Role of band filling in tuning the high-field phases of ${URu}_{2} {Si}_{2}$

Sequential Spin Polarization of the Fermi Surface Pockets in ${URu}_{2} {Si}_{2}$ and Its Implications for the Hidden Order
journal, April 2011

Absence of a static in-plane magnetic moment in the ‘hidden-order’ phase of URu ₂ Si ₂
journal, May 2013

Phase diagram and thermal expansion measurements on the system URu _{2− x} Fe _x Si ₂
journal, November 2016

Chemical pressure tuning of ${URu}_{2} {Si}_{2}$ via isoelectronic substitution of Ru with Fe
journal, February 2015

High Magnetic Field Studies of the Hidden Order Transition in ${U R u}_{2} {S i}_{2}$
journal, December 2002

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

Metamagnetic Behavior and Effect of Pressure on the Electronic State in Heavy-Fermion Compound YbRh ₂ Zn ₂₀
journal, August 2013

Unfolding the physics of URu2Si2 through silicon to phosphorus substitution
journal, February 2016

Hybridization model for the magnetic-ordering behavior of uranium- and cerium-based 1:2:2 intermetallic compounds
journal, October 1993

Temperature-pressure phase diagram of $U {Ru}_{2} {Si}_{2}$ from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting
journal, March 2008

Nature of the $5 f$ states in actinide metals
journal, February 2009

Effect of pressure on competing electronic correlations in the heavy-electron system ${URu}_{2}$ ${Si}_{2}$
journal, January 1987

NMR investigation of antiferromagnetism and coherence in ${URu}_{2} {Si}_{2 - x} P_{x}$
journal, January 2017

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2
journal, June 1986

High purity specimens of URu ₂ Si ₂ produced by a molten metal flux technique
journal, April 2014

Effect of transition-metal substitutions on competing electronic transitions in the heavy-electron compound ${URu}_{2}$ ${Si}_{2}$
journal, February 1990

Magnetic properties of the ternary compounds CeT2Si2 and UT2Si2
journal, February 1986

Magnetic Structure of Phase II in $U ({Ru}_{0.96} {Rh}_{0.04})_{2} {Si}_{2}$ Determined by Neutron Diffraction under Pulsed High Magnetic Fields
journal, May 2013

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of ${URu}_{2} {Si}_{2}$
journal, November 2010

Enhancement of the hidden order/large moment antiferromagnetic transition temperature in the URu _{2− x} Os _x Si ₂ system
journal, April 2014

Ferromagnetic instability in the heavy-electron compound ${URu}_{2}$ ${Si}_{2}$ doped with Re or Tc
journal, February 1989

Field-induced spin-density wave beyond hidden order in URu2Si2
journal, October 2016

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Nexus between Quantum Criticality and Phase Formation in $U ({R u}_{1 - x} {R h}_{x})_{2} {S i}_{2}$
journal, November 2004

Magnetic-Field-Induced Quantum Critical Point and Competing Order Parameters in ${U R u}_{2} {S i}_{2}$
journal, December 2003

Hidden order behaviour in URu ₂ Si ₂ (A critical review of the status of hidden order in 2014)
journal, May 2014

The suppression of hidden order and the onset of ferromagnetism in URu ₂ Si ₂ via Re substitution
journal, March 2010

Field Reentrance of the Hidden Order State of URu ₂ Si ₂ under Pressure
journal, May 2009

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu $_{2 - x}$ Fe $_{x}$ Si $_{2}$ system
journal, December 2011

Interplay of magnetism, Fermi surface reconstructions, and hidden order in the heavy-fermion material URu $_{2}$ Si $_{2}$
journal, March 2012

Thermodynamic and electrical transport investigation of URu ₂ Si _{2− x} P _x
journal, November 2016

Specific heat of ${URu}_{2} {Si}_{2}$ in fields up to 42 T: Clues to the hidden order
journal, January 2003

Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7
journal, October 2001

Instability of the f -electron state in URu 2 Si 2 − x P x probed using high magnetic fields
journal, June 2019